scholarly journals Aerosol properties and their influences on marine boundary layer cloud condensation nuclei at the ARM mobile facility over the Azores

2014 ◽  
Vol 119 (8) ◽  
pp. 4859-4872 ◽  
Author(s):  
Timothy Logan ◽  
Baike Xi ◽  
Xiquan Dong
Keyword(s):  
Boundary Layer ◽  
Marine Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Condensation Nuclei ◽  
Boundary Layer Cloud ◽  
Aerosol Properties ◽  
Layer Cloud

scholarly journals The relationship between cloud condensation nuclei (CCN) concentration and light extinction of dried particles: indications of underlying aerosol processes and implications for satellite-based CCN estimates

2015 ◽  
Vol 15 (13) ◽  
pp. 7585-7604 ◽  
Author(s):  
Y. Shinozuka ◽  
A. D. Clarke ◽  
A. Nenes ◽  
A. Jefferson ◽  
R. Wood ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Extinction Coefficient ◽  
Cloud Condensation Nuclei ◽  
Number Concentration ◽  
Light Extinction ◽  
Condensation Nuclei ◽  
Average Data ◽  
Boundary Layer Cloud ◽  
The Relationship ◽  
Layer Cloud

Abstract. We examine the relationship between the number concentration of boundary-layer cloud condensation nuclei (CCN) and light extinction to investigate underlying aerosol processes and satellite-based CCN estimates. For a variety of airborne and ground-based observations not dominated by dust, regression identifies the CCN (cm−3) at 0.4 ± 0.1% supersaturation with 100.3α +1.3σ0.75 where σ (Mm−1) is the 500 nm extinction coefficient by dried particles and α is the Angstrom exponent. The deviation of 1 km horizontal average data from this approximation is typically within a factor of 2.0. ∂logCCN / ∂logσ is less than unity because, among other explanations, growth processes generally make aerosols scatter more light without increasing their number. This, barring special meteorology–aerosol connections, associates a doubling of aerosol optical depth with less than a doubling of CCN, contrary to previous studies based on heavily averaged measurements or a satellite algorithm.

scholarly journals Marine boundary layer cloud regimes and POC formation in a CRM coupled to a bulk aerosol scheme

2013 ◽  
Vol 13 (24) ◽  
pp. 12549-12572 ◽  
Author(s):  
A. H. Berner ◽  
C. S. Bretherton ◽  
R. Wood ◽  
A. Muhlbauer
Keyword(s):  
Boundary Layer ◽  
Marine Boundary Layer ◽  
Three Dimensional ◽  
Two Dimensional ◽  
State Variables ◽  
Liquid Water Path ◽  
Modeling Framework ◽  
Boundary Layer Cloud ◽  
Cloud Regimes ◽  
Layer Cloud

Abstract. A cloud-resolving model (CRM) coupled to a new intermediate-complexity bulk aerosol scheme is used to study aerosol–boundary-layer–cloud–precipitation interactions and the development of pockets of open cells (POCs) in subtropical stratocumulus cloud layers. The aerosol scheme prognoses mass and number concentration of a single lognormal accumulation mode with surface and entrainment sources, evolving subject to processing of activated aerosol and scavenging of dry aerosol by clouds and rain. The CRM with the aerosol scheme is applied to a range of steadily forced cases idealized from a well-observed POC. The long-term system evolution is explored with extended two-dimensional (2-D) simulations of up to 20 days, mostly with diurnally averaged insolation and 24 km wide domains, and one 10 day three-dimensional (3-D) simulation. Both 2-D and 3-D simulations support the Baker–Charlson hypothesis of two distinct aerosol–cloud "regimes" (deep/high-aerosol/non-drizzling and shallow/low-aerosol/drizzling) that persist for days; transitions between these regimes, driven by either precipitation scavenging or aerosol entrainment from the free-troposphere (FT), occur on a timescale of ten hours. The system is analyzed using a two-dimensional phase plane with inversion height and boundary layer average aerosol concentrations as state variables; depending on the specified subsidence rate and availability of FT aerosol, these regimes are either stable equilibria or distinct legs of a slow limit cycle. The same steadily forced modeling framework is applied to the coupled development and evolution of a POC and the surrounding overcast boundary layer in a larger 192 km wide domain. An initial 50% aerosol reduction is applied to half of the model domain. This has little effect until the stratocumulus thickens enough to drizzle, at which time the low-aerosol portion transitions into open-cell convection, forming a POC. Reduced entrainment in the POC induces a negative feedback between the areal fraction covered by the POC and boundary layer depth changes. This stabilizes the system by controlling liquid water path and precipitation sinks of aerosol number in the overcast region, while also preventing boundary layer collapse within the POC, allowing the POC and overcast to coexist indefinitely in a quasi-steady equilibrium.

scholarly journals Contrasting characteristics of open- and closed- cellular stratocumulus cloud in the Eastern North Atlantic

2021 ◽  
Author(s):  
Michael P. Jensen ◽  
Virendra P. Ghate ◽  
Dié Wang ◽  
Diana K. Apoznanski ◽  
Mary J. Bartholomew ◽  
...  
Keyword(s):  
Boundary Layer ◽  
North Atlantic ◽  
Large Scale ◽  
Marine Boundary Layer ◽  
Open Cell ◽  
Cold Air ◽  
Closed Cell ◽  
Boundary Layer Cloud ◽  
Eastern North Atlantic ◽  
Layer Cloud

Abstract. Extensive regions of marine boundary layer cloud impact the radiative balance through their significant shortwave albedo while having little impact on outgoing longwave radiation. Despite this importance, these cloud systems remain poorly represented in large-scale models due to difficulty in representing the processes that drive their lifecycle and coverage. In particular, the mesoscale organization, and cellular structure of marine boundary clouds has important implications for the subsequent cloud feedbacks. In this study, we use long-term (2013–2018) observations from the Atmospheric Radiation Measurement (ARM) Facility's Eastern North Atlantic (ENA) site on Graciosa Island, Azores, Portugal to identify cloud cases with open- or closed-cellular organization. More than 500 hours of each organization type are identified. The ARM observations are combined with reanalysis and satellite products to quantify the cloud, precipitation, aerosol, thermodynamic and large-scale synoptic characteristics associated with these cloud types. Our analysis shows that both cloud organization populations occur during similar sea surface temperature conditions, but the open-cell cases are distinguished by stronger cold-air advection and large-scale subsidence compared to the closed-cell cases, consistent with their formation during cold-air outbreaks. We also find that the open-cell cases were associated with deeper boundary layers, stronger low-level winds, and higher-rain rates compared to their closed-cell counterparts. Finally, raindrops with diameters larger than one millimeter were routinely recorded at the surface during both populations, with a higher number of large drops during the open-cellular cases. The similarities and differences noted herein provide important insights into the environmental and cloud characteristics during varying marine boundary layer cloud mesoscale organization and will be useful for the evaluation of model simulations for ENA marine clouds.

scholarly journals Contrasting characteristics of open- and closed-cellular stratocumulus cloud in the eastern North Atlantic

2021 ◽  
Vol 21 (19) ◽  
pp. 14557-14571
Author(s):  
Michael P. Jensen ◽  
Virendra P. Ghate ◽  
Dié Wang ◽  
Diana K. Apoznanski ◽  
Mary J. Bartholomew ◽  
...  
Keyword(s):  
Boundary Layer ◽  
North Atlantic ◽  
Large Scale ◽  
Marine Boundary Layer ◽  
Open Cell ◽  
Cold Air ◽  
Closed Cell ◽  
Boundary Layer Cloud ◽  
Eastern North Atlantic ◽  
Layer Cloud

Abstract. Extensive regions of marine boundary layer cloud impact the radiative balance through their significant shortwave albedo while having little impact on outgoing longwave radiation. Despite this importance, these cloud systems remain poorly represented in large-scale models due to difficulty in representing the processes that drive their life cycle and coverage. In particular, the mesoscale organization and cellular structure of marine boundary clouds have important implications for the subsequent cloud feedbacks. In this study, we use long-term (2013–2018) observations from the Atmospheric Radiation Measurement (ARM) Facility's Eastern North Atlantic (ENA) site on Graciosa Island, Azores, Portugal, to identify cloud cases with open- or closed-cellular organization. More than 500 h of each organization type are identified. The ARM observations are combined with reanalysis and satellite products to quantify the cloud, precipitation, aerosol, thermodynamic, and large-scale synoptic characteristics associated with these cloud types. Our analysis shows that both cloud organization populations occur during similar sea surface temperature conditions, but the open-cell cases are distinguished by stronger cold-air advection and large-scale subsidence compared to the closed-cell cases, consistent with their formation during cold-air outbreaks. We also find that the open-cell cases were associated with deeper boundary layers, stronger low-level winds, and higher rain rates compared to their closed-cell counterparts. Finally, raindrops with diameters larger than 1 mm were routinely recorded at the surface during both populations, with a higher number of large drops during the open-cellular cases. The similarities and differences noted herein provide important insights into the environmental and cloud characteristics during varying marine boundary layer cloud mesoscale organization and will be useful for the evaluation of model simulations for ENA marine clouds.

scholarly journals Assessment of marine boundary layer cloud simulations in the CAM with CLUBB and updated microphysics scheme based on ARM observations from the Azores

2016 ◽  
Vol 121 (14) ◽  
pp. 8472-8492 ◽  
Author(s):  
X. Zheng ◽  
S. A. Klein ◽  
H.-Y. Ma ◽  
P. Bogenschutz ◽  
A. Gettelman ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Marine Boundary Layer ◽  
Microphysics Scheme ◽  
Boundary Layer Cloud ◽  
Layer Cloud

scholarly journals Intercomparisons of marine boundary layer cloud properties from the ARM CAP‐MBL campaign and two MODIS cloud products

2017 ◽  
Vol 122 (4) ◽  
pp. 2351-2365 ◽  
Author(s):  
Zhibo Zhang ◽  
Xiquan Dong ◽  
Baike Xi ◽  
Hua Song ◽  
Po‐Lun Ma ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Marine Boundary Layer ◽  
Cloud Properties ◽  
Boundary Layer Cloud ◽  
Layer Cloud

Shipboard Measurements of Aerosol Properties in the Coupled Ocean-Atmosphere System of the Northwest Tropical Atlantic

2020 ◽  
Author(s):  
Tim Bates ◽  
Patricia Quinn
Keyword(s):  
Solar Radiation ◽  
Marine Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Cloud Droplet ◽  
Lower Atmosphere ◽  
Radiation Balance ◽  
Tropical Atlantic ◽  
Shallow Convection ◽  
Condensation Nuclei ◽  
Aerosol Properties

<p>The fair-weather cumulus clouds, that cover much of the low-latitude oceans, affect the radiation balance of the planet by reflecting incoming solar radiation and absorbing outgoing longwave radiation.  These clouds also drive atmospheric circulation by mixing the lower atmosphere in a process called shallow convection.  This mixing, in turn, affects sea surface temperature and salinity by moderating the air-sea exchange of energy and moisture.  Marine boundary layer (MBL) atmospheric aerosols play a role in the processes described above by scattering and absorbing solar radiation and by serving as cloud condensation nuclei (CCN) thereby influencing cloud droplet concentrations and size; the extent, lifetime, and albedo of clouds; and the frequency and intensity of precipitation. Quantifying the role of aerosols over the Northwest Tropical Atlantic is critical to advance understanding of shallow convection and air-sea interactions.</p><p>MBL aerosol properties were measured aboard the RV Ronald H. Brown during the EUREC4A and ATOMIC field studies in January/February 2020.  Aerosols encountered during the study include background sulfate/sea spray particles and African dust/biomass burning particles.  Aerosol physical, chemical, optical and cloud condensation nuclei properties will be presented and their interaction with local and regional circulation.</p>

scholarly journals A global off-line model of size-resolved aerosol microphysics: II. Identification of key uncertainties

2005 ◽  
Vol 5 (12) ◽  
pp. 3233-3250 ◽  
Author(s):  
D. V. Spracklen ◽  
K. J. Pringle ◽  
K. S. Carslaw ◽  
M. P. Chipperfield ◽  
G. W. Mann
Keyword(s):  
Nucleation Rate ◽  
Marine Boundary Layer ◽  
Cloud Condensation Nuclei ◽  
Accommodation Coefficient ◽  
Sulfate Aerosol ◽  
Sea Salt ◽  
Condensation Nuclei ◽  
Microphysical Processes ◽  
Global Mean ◽  
Aerosol Properties

Abstract. We use the new GLOMAP model of global aerosol microphysics to investigate the sensitivity of modelled sulfate and sea salt aerosol properties to uncertainties in the driving microphysical processes and compare these uncertainties with those associated with aerosol and precursor gas emissions. Overall, we conclude that uncertainties in microphysical processes have a larger effect on global sulfate and sea salt derived condensation nuclei (CN) and cloud condensation nuclei (CCN) concentrations than uncertainties in present-day sulfur emissions. Our simulations suggest that uncertainties in predicted sulfate and sea salt CCN abundances due to poorly constrained microphysical processes are likely to be of a similar magnitude to long-term changes in sulfate and sea salt CCN due to changes in anthropogenic emissions. A microphysical treatment of the global sulfate aerosol allows the uncertainty in climate-relevant aerosol properties to be attributed to specific processes in a way that has not been possible with simpler aerosol schemes. In particular we conclude that: (1) changes in the binary H2SO4-H2O nucleation rate and condensation rate of gaseous H2SO4 cause a shift in the vertical location of the upper tropospheric CN layer by as much as 3 km, while the shape of the CN profile is essentially pre-served (2) uncertainties in the binary H2SO4-H2O nucleation rate have a relatively insignificant effect on marine boundary layer (MBL) aerosol properties; (3) emitting a fraction of anthropogenic SO2 as particulates (to represent production of sulfate particles in power plant plumes below the scale of the model grid (which is of the order of 300 km)) has the potential to change the global mean MBL sulfate-derived CN concentrations by up to 72%, and changes of up to a factor 20 can occur in polluted continental regions; (4) predicted global mean MBL sulfate and sea salt CCN concentrations change by 10 to 60% when several microphysical processes are changed within reasonable uncertainty ranges; (5) sulfate and sea salt derived CCN concentrations are particularly sensitive to primary particle emissions, with global mean MBL sulfate and sea salt CCN changing by up to 27% and local concentrations over continental regions changing by more than 100% when the percentage of anthropogenic SO2 emitted as particulates is changed from 0 to 5%; (6) large changes in sea spray flux have insignificant effects on global sulfate aerosol except when the mass accommodation coefficient of sulfuric acid on the salt particles is set unrealistically low.

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