Hierarchical porous nitrogen-doped carbon materials derived from one-step carbonization of polyimide for efficient CO2 adsorption and separation

2016 ◽  
Vol 24 (3) ◽  
pp. 583-589 ◽  
Author(s):  
Yurong Liu ◽  
Yaqin Chen ◽  
Liangliang Tian ◽  
Rong Hu
Materials ◽  
2019 ◽  
Vol 12 (8) ◽  
pp. 1207 ◽  
Author(s):  
Ruiping Wei ◽  
Xingchao Dai ◽  
Feng Shi

Nitrogen-doped carbon materials with enhanced CO2 adsorption were prepared by the salt and base co-activation method. First, resorcinol-formaldehyde resin was synthesized with a certain salt as an additive and used as a precursor. Next, the resulting precursor was mixed with KOH and subsequently carbonized under ammonia flow to finally obtain the nitrogen-doped carbon materials. A series of samples, with and without the addition of different salts, were prepared, characterized by XRD (X-ray powder diffraction), elemental analysis, BET (N2-adsorption-desorption analysis), XPS (X-ray photoelectron spectroscopy) and SEM (Scanning electron microscopy) and tested for CO2 adsorption. The results showed that the salt and base co-activation method has a remarkable enhancing effect on the CO2 capture capacity. The combination of KCl and KOH was proved to be the best combination, and 167.15 mg CO2 could be adsorbed with 1 g nitrogen-doped carbon at 30 °C under 1 atm pressure. The materials characterizations revealed that the introduction of the base and salt could greatly increase the content of doped nitrogen, the surface area and the amount of formed micropore, which led to enhanced CO2 absorption of the carbon materials.


2021 ◽  
Author(s):  
Chengfeng Yi ◽  
Lushuang Zhang ◽  
Ganghua Xiang ◽  
Xiaoyan Chen ◽  
Na Cheng ◽  
...  

Nitrogen–doped carbon materials with hierarchical porous structures have attracted mountainous attentions in the field of catalysis owing to their special structures and properties in the past decades. In this study,...


2019 ◽  
Vol 7 (21) ◽  
pp. 13154-13163 ◽  
Author(s):  
Yuntong Li ◽  
Ling Liu ◽  
Yuzhe Wu ◽  
Tong Wu ◽  
Haiyang Wu ◽  
...  

Hierarchical porous nitrogen-doped carbon materials possess an outstanding supercapacitance performance in both acidic and alkaline electrolytes.


2014 ◽  
Vol 2 (30) ◽  
pp. 11666-11671 ◽  
Author(s):  
Xiaojun Zhao ◽  
Huanyu Zhao ◽  
Tingting Zhang ◽  
Xuecheng Yan ◽  
Ye Yuan ◽  
...  

In this work, a series of microporous nitrogen-doped carbon catalysts are reported through a convenient preparation route, and exhibit excellent performance for oxygen reduction reaction.


2020 ◽  
Vol 39 ◽  
pp. 101164
Author(s):  
Jinsong Shi ◽  
Hongmin Cui ◽  
Jianguo Xu ◽  
Nanfu Yan ◽  
Yuewei Liu ◽  
...  

RSC Advances ◽  
2021 ◽  
Vol 11 (15) ◽  
pp. 8628-8635
Author(s):  
Chang Ki Kim ◽  
Jung-Min Ji ◽  
M. Aftabuzzaman ◽  
Hwan Kyu Kim

The incorporation of the Te element into nitrogen-doped carbon-based nanomaterials is a good strategy to improve the capacitive performance of carbon materials and the incorporation of two types of atoms improves the overall capacitive performance of the materials due to a synergetic effect.


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