Relationship between submicron particle formation and air mass history observed in the Asian continental outflow at Gosan, Korea, during 2008–2018

2020 ◽  
Author(s):  
Sang-Woo Kim ◽  
Junghwa Heo ◽  
Jong-Uk Park
Keyword(s):  
Particle Formation ◽  
Submicron Particle ◽  
Air Mass ◽  
Continental Outflow

scholarly journals Concentrations and fluxes of aerosol particles during the LAPBIAT measurement campaign at Värriö field station

2007 ◽  
Vol 7 (14) ◽  
pp. 3683-3700 ◽  
Author(s):  
T. M. Ruuskanen ◽  
M. Kaasik ◽  
P. P. Aalto ◽  
U. Hõrrak ◽  
M. Vana ◽  
...  
Keyword(s):  
Kola Peninsula ◽  
Aerosol Particle ◽  
Aerosol Particles ◽  
Particle Formation ◽  
Nucleation Event ◽  
New Particle Formation ◽  
Air Ions ◽  
Field Station ◽  
Air Mass ◽  
Measurement Campaign

Abstract. The LAPBIAT measurement campaign took place in the Värriö SMEAR I measurement station located in Eastern Lapland in the spring of 2003 between 26 April and 11 May. In this paper we describe the measurement campaign, concentrations and fluxes of aerosol particles, air ions and trace gases, paying special attention to an aerosol particle formation event broken by a air mass change from a clean Arctic air mass with new particle formation to polluted one approaching from industrial areas of Kola Peninsula, Russia, lacking new particle formation. Aerosol particle number flux measurements show strong downward fluxes during that time. Concentrations of coarse aerosol particles were high for 1–2 days before the nucleation event (i.e. 28–29 April), very low immediately before and during the observed aerosol particle formation event (30 April) and increased moderately from the moment of sudden break of the event. In general particle deposition measurements based on snow samples show the same changes. Measurements of the mobility distribution of air ions showed elevated concentrations of intermediate air ions during the particle formation event. We estimated the growth rates in the nucleation mode size range. For particles <10 nm, the growth rate increases with size on 30 April. Dispersion modelling made with model SILAM support the conclusion that the nucleation event was interrupted by an outbreak of sulphate-rich air mass in the evening of 30 April that originated from the industry at Kola Peninsula, Russia. The results of this campaign highlight the need for detailed research in atmospheric transport of air constituents for understanding the aerosol dynamics.

Characterization of new particle formation events at a background site in Southern Sweden: relation to air mass history

Tellus B ◽  
2008 ◽  
Vol 60 (3) ◽  
pp. 330-344 ◽  
Author(s):  
A. Kristensson ◽  
M. Dal Maso ◽  
E. Swietlicki ◽  
T. Hussein ◽  
J. Zhou ◽  
...  
Keyword(s):  
Particle Formation ◽  
New Particle Formation ◽  
Southern Sweden ◽  
Air Mass ◽  
Background Site

scholarly journals New particle formation in air mass transported between two measurement sites in Northern Finland

2005 ◽  
Vol 5 (6) ◽  
pp. 11929-11963 ◽  
Author(s):  
M. Komppula ◽  
S.-L. Sihto ◽  
H. Korhonen ◽  
H. Lihavainen ◽  
V.-M. Kerminen ◽  
...  
Keyword(s):  
Growth Rates ◽  
Particle Growth ◽  
Particle Formation ◽  
Distribution Data ◽  
New Particle Formation ◽  
Air Mass ◽  
Air Masses ◽  
Aerosol Dynamics ◽  
Almost All ◽  
Distinct Features

Abstract. This study covers four years of aerosol number size distribution data from Pallas and Värriö sites 250 km apart from each other in Northern Finland and compares new particle formation events between these sites. In eastern air masses almost all events were observed to start earlier at the eastern station Värriö, whereas in western air masses most of the events were observed to start earlier at the western station Pallas. This demonstrates that particle formation in a certain air mass type depends not only on the diurnal variation of the parameters causing the phenomenon (such as photochemistry) but also on some properties carried by the air mass itself. The correlation in growth rates between the two sites was relatively good, which suggests that the amount of condensable vapour causing the growth must have been at about the same level in both sites. The value of condensation sink was frequently much higher at the downwind station. It seems that secondary particle formation related to biogenic sources dominate in many cases over the particle sinks during the air mass transport between the sites. Two cases of transport from Pallas to Värriö were further analysed with an aerosol dynamics model. The model was able to reproduce the observed nucleation events 250 km down-wind at Värriö but revealed some differences between the two cases. The simulated nucleation rates were in both cases similar but the organic concentration profiles that best reproduced the observations were different in the two cases indicating that divergent formation reactions may dominate under different conditions. The simulations also suggested that organic compounds were the main contributor to new particle growth, which offers a tentative hypothesis to the distinct features of new particles at the two sites: Air masses arriving from Atlantic Ocean typically spent approximately only ten hours over land before arriving at Pallas, and thus the time for the organic vapours to accumulate in the air and to interact with the particles is relatively short. This can lead to low nucleation mode growth rates and even to suppression of detectable particle formation event due to efficient scavenging of newly formed clusters, as was observed in the case studies.

scholarly journals Measurement report: New particle formation characteristics at an urban and a mountain station in northern China

2021 ◽  
Vol 21 (23) ◽  
pp. 17885-17906
Author(s):  
Ying Zhou ◽  
Simo Hakala ◽  
Chao Yan ◽  
Yang Gao ◽  
Xiaohong Yao ◽  
...  
Keyword(s):  
Urban Areas ◽  
Formation Rate ◽  
Northern China ◽  
Particle Formation ◽  
Urban Site ◽  
New Particle Formation ◽  
Large Area ◽  
Air Mass ◽  
Mountain Site ◽  
Favorable Conditions

Abstract. Atmospheric new particle formation (NPF) events have attracted increasing attention for their contribution to the global aerosol number budget and therefore their effects on climate, air quality and human health. NPF events are regarded as a regional phenomenon, occurring over a large area. Most observations of NPF events in Beijing and its vicinity were conducted in populated areas, whereas observations of NPF events on mountaintops with low anthropogenic emissions are still rare in China. The spatial variation of NPF event intensity has not been investigated in detail by incorporating both urban areas and mountain measurements in Beijing. Here, we provide NPF event characteristics in summer 2018 and 2019 at urban Beijing and a comparison of NPF event characteristics – NPF event frequency, formation rate and growth rate – by comparing an urban Beijing site and a background mountain site separated by ∼80 km from 14 June to 14 July 2019, as well as giving insights into the connection between both locations. During parallel measurements at urban Beijing and mountain background areas, although the median condensation sink during the first 2 h of the common NPF events was around 0.01 s−1 at both sites, there were notable differences in formation rates between the two locations (median of 5.42 cm−3 s−1 at the urban site and 1.13 cm−3 s−1 at the mountain site during the first 2 h of common NPF events). In addition, the growth rates in the 7–15 nm range for common NPF events at the urban site (median of 7.6 nm h−1) were slightly higher than those at the mountain site (median of 6.5 nm h−1). To understand whether the observed events were connected, we compared air mass trajectories as well as meteorological conditions at both stations. Favorable conditions for the occurrence of regional NPF events were largely affected by air mass transport. Overall, our results demonstrate a clear inhomogeneity of regional NPF within a distance of ∼100 km, possibly due to the discretely distributed emission sources.

scholarly journals Spatial distribution and occurrence probability of regional new particle formation events in eastern China

2018 ◽  
Vol 18 (2) ◽  
pp. 587-599 ◽  
Author(s):  
Xiaojing Shen ◽  
Junying Sun ◽  
Niku Kivekäs ◽  
Adam Kristensson ◽  
Xiaoye Zhang ◽  
...  
Keyword(s):  
Spatial Distribution ◽  
Eastern China ◽  
Particle Formation ◽  
Spatial Extent ◽  
Occurrence Probability ◽  
New Particle Formation ◽  
Relative Probability ◽  
Air Mass ◽  
Air Masses ◽  
Rural Sites

Abstract. In this work, the spatial extent of new particle formation (NPF) events and the relative probability of observing particles originating from different spatial origins around three rural sites in eastern China were investigated using the NanoMap method, using particle number size distribution (PNSD) data and air mass back trajectories. The length of the datasets used were 7, 1.5, and 3 years at rural sites Shangdianzi (SDZ) in the North China Plain (NCP), Mt. Tai (TS) in central eastern China, and Lin'an (LAN) in the Yangtze River Delta region in eastern China, respectively. Regional NPF events were observed to occur with the horizontal extent larger than 500 km at SDZ and TS, favoured by the fast transport of northwesterly air masses. At LAN, however, the spatial footprint of NPF events was mostly observed around the site within 100–200 km. Difference in the horizontal spatial distribution of new particle source areas at different sites was connected to typical meteorological conditions at the sites. Consecutive large-scale regional NPF events were observed at SDZ and TS simultaneously and were associated with a high surface pressure system dominating over this area. Simultaneous NPF events at SDZ and LAN were seldom observed. At SDZ the polluted air masses arriving over the NCP were associated with higher particle growth rate (GR) and new particle formation rate (J) than air masses from Inner Mongolia (IM). At TS the same phenomenon was observed for J, but GR was somewhat lower in air masses arriving over the NCP compared to those arriving from IM. The capability of NanoMap to capture the NPF occurrence probability depends on the length of the dataset of PNSD measurement but also on topography around the measurement site and typical air mass advection speed during NPF events. Thus the long-term measurements of PNSD in the planetary boundary layer are necessary in the further study of spatial extent and the probability of NPF events. The spatial extent, relative probability of occurrence, and typical evolution of PNSD during NPF events presented in this study provide valuable information to further understand the climate and air quality effects of new particle formation.

Seasonality of new particle formation in Vienna, Austria – Influence of air mass origin and aerosol chemical composition

2015 ◽  
Vol 118 ◽  
pp. 118-126 ◽  
Author(s):  
Anna Wonaschütz ◽  
Anselm Demattio ◽  
Robert Wagner ◽  
Julia Burkart ◽  
Naděžda Zíková ◽  
...  
Keyword(s):  
Chemical Composition ◽  
Particle Formation ◽  
New Particle Formation ◽  
Air Mass ◽  
Air Mass Origin ◽  
Aerosol Chemical Composition

scholarly journals New particle formation and ultrafine charged aerosol climatology at a high altitude site in the Alps (Jungfraujoch, 3580 m a.s.l., Switzerland)

2010 ◽  
Vol 10 (19) ◽  
pp. 9333-9349 ◽  
Author(s):  
J. Boulon ◽  
K. Sellegri ◽  
H. Venzac ◽  
D. Picard ◽  
E. Weingartner ◽  
...  
Keyword(s):  
High Altitude ◽  
Particle Formation ◽  
Ion Source ◽  
Swiss Alps ◽  
Aerosol Size Distribution ◽  
New Particle Formation ◽  
Data Set ◽  
Air Mass ◽  
Air Masses ◽  
Charged Aerosol

Abstract. We investigate the formation and growth of charged aerosols clusters at Jungfraujoch, in the Swiss Alps (3580 m a.s.l.), the highest altitude site of the European EUCAARI project intensive campaign. Charged particles and clusters (0.5–1.8 nm) were measured from April 2008 to April 2009 and allowed the detection of nucleation events in this very specific environment (presence of free tropospheric air and clouds). We found that the naturally charged aerosol concentrations, which are dominated by the cluster size class, shows a strong diurnal pattern likely linked to valley breezes transporting surface layer ion precursors, presumably radon. Cosmic rays were found not to be the major ion source at the measurement site. However, at night, when air masses are more representative of free tropospheric conditions, we found that the cluster concentrations are still high. The charged aerosol size distribution and concentration are strongly influenced by the presence of clouds at the station. Clouds should be taken into account when deriving high altitude nucleation statistics. New particle formation occurs on average 17.5% of the measurement period and shows a weak seasonality with a minimum of frequency during winter, but this seasonality is enhanced when the data set is screened for periods when the atmospheric station is out of clouds. The role of ions in the nucleation process was investigated and we found that the ion-mediated nucleation explains 22.3% of the particle formation. The NPF events frequency is correlated with UV radiation but not with calculated H2SO4 concentrations, suggesting that other compounds such as organic vapors are involved in the nucleation and subsequently growth process. In fact, NPF events frequency also surprisingly increases with the condensational sink (CS), suggesting that at Jungfraujoch, the presence of condensing vapours probably coupled with high CS are driving the occurrence of NPF events. A strong link to the air mass path was also pointed out and events were observed to be frequently occurring in Eastern European air masses, which present the highest condensational sink. In these air masses, pre-existing cluster concentrations are more than three time larger than in other air masses during event days, and no new clusters formation is observed, contrarily to what is happening in other air mass types.

scholarly journals Concentrations and fluxes of aerosol particles during the LAPBIAT measurement campaign in Värriö field station

2007 ◽  
Vol 7 (1) ◽  
pp. 709-751
Author(s):  
T. M. Ruuskanen ◽  
M. Kaasik ◽  
P. P. Aalto ◽  
U. Hõrrak ◽  
M. Vana ◽  
...  
Keyword(s):  
Kola Peninsula ◽  
Aerosol Particle ◽  
Particle Deposition ◽  
Aerosol Particles ◽  
Particle Formation ◽  
Nucleation Event ◽  
Air Ions ◽  
Field Station ◽  
Air Mass ◽  
Measurement Campaign

Abstract. The LAPBIAT measurement campaign took place in the SMEAR I measurement station located in Eastern Lapland in the spring of 2003 between 26 April and 11 May. In this paper we describe the measurement campaign, concentrations and fluxes of aerosol particles, air ions and trace gases, paying special attention to an aerosol particle formation event broken by a polluted air mass approaching from industrial areas of Kola Peninsula, Russia. Aerosol particle number flux measurements show strong downward fluxes during that time. Concentrations of coarse aerosol particles were high for 1–2 days before the nucleation event (i.e. 28–29 April), very low immediately before and during the observed aerosol particle formation event (30 April) and increased moderately from the moment of sudden break of the event. In general particle deposition measurements based on snow samples show the same changes. Measurements of the mobility distribution of air ions showed elevated concentrations of intermediate air ions during the particle formation event. We estimated the growth rates in the nucleation mode size range. For particles <10 nm, the growth rate increases with size on 30 April. Dispersion modelling made with model SILAM support the conclusion that the nucleation event was interrupted by an outbreak of sulphate-rich air mass in the evening of 30 April that originated from the industry at Kola Peninsula, Russia. The results of this campaign highlight the need for detailed research in atmospheric transport of air constituents for understanding the aerosol dynamics.

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