An aerothermochemical analysis of solid carbon combustion in the stagnation flow accompanied by homogeneous CO oxidation

1987 ◽  
Vol 70 (1) ◽  
pp. 79-99 ◽  
Author(s):  
K. Matsui ◽  
H. Tsuji
Catalysts ◽  
2019 ◽  
Vol 9 (5) ◽  
pp. 484 ◽  
Author(s):  
Jianfeng Zhou ◽  
Sebastian Matera ◽  
Sebastian Pfaff ◽  
Sara Blomberg ◽  
Edvin Lundgren ◽  
...  

A stagnation flow reactor has been designed and characterized for both experimental and modeling studies of single-crystal model catalysts in heterogeneous catalysis. Using CO oxidation over a Pd(100) single crystal as a showcase, we have employed planar laser-induced fluorescence (PLIF) to visualize the CO2 distribution over the catalyst under reaction conditions and subsequently used the 2D spatially resolved gas phase data to characterize the stagnation flow reactor. From a comparison of the experimental data and the stagnation flow model, it was found that characteristic stagnation flow can be achieved with the reactor. Furthermore, the combined stagnation flow/PLIF/modeling approach makes it possible to estimate the turnover frequency (TOF) of the catalytic surface from the measured CO2 concentration profiles above the surface and to predict the CO2, CO and O2 concentrations at the surface under reaction conditions.


1989 ◽  
Vol 75 (3-4) ◽  
pp. 281-295 ◽  
Author(s):  
F. Méndez ◽  
C. Treviño ◽  
A. Liñán

1996 ◽  
Vol 100 (3) ◽  
pp. 1048-1054 ◽  
Author(s):  
Tsuyoshi Sueyoshi ◽  
Takehiko Sasaki ◽  
Yasuhiro Iwasawa

2013 ◽  
Vol 133 (12) ◽  
pp. 642-647 ◽  
Author(s):  
Hitomi Kawakami ◽  
Akinori Zukeran ◽  
Koji Yasumoto ◽  
Yoshiyasu Ehara ◽  
Toshiaki Yamamoto

2004 ◽  
Vol 40 (1) ◽  
pp. 8
Author(s):  
N. Dzyuban ◽  
E. S. Bikbulatov ◽  
E. M. Bikbulatova ◽  
I. A. Kuznetsova

Author(s):  
І. О. Пеняк ◽  
Б. В. Гнатів ◽  
М. В. Токарчук

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