Simulation of radiation induced dissolution of spent nuclear fuel using the steady-state approach. A comparison to experimental data

2008 ◽  
Vol 374 (1-2) ◽  
pp. 286-289 ◽  
Author(s):  
Fredrik Nielsen ◽  
Ella Ekeroth ◽  
Trygve E. Eriksen ◽  
Mats Jonsson
Author(s):  
James A. Fort ◽  
Judith M. Cuta ◽  
Chris S. Bajwa ◽  
Emilio Baglietto

In the United States, commercial spent nuclear fuel is typically moved from spent fuel pools to outdoor dry storage pads within a transfer cask system that provides radiation shielding to protect personnel and the surrounding environment. The transfer casks are cylindrical steel enclosures with integral gamma and neutron radiation shields. Since the transfer cask system must be passively cooled, decay heat removal from the spent nuclear fuel canister is limited by the rate of heat transfer through the cask components, and natural convection from the transfer cask surface. The primary mode of heat transfer within the transfer cask system is conduction, but some cask designs incorporate a liquid neutron shield tank surrounding the transfer cask structural shell. In these systems, accurate prediction of natural convection within the neutron shield tank is an important part of assessing the overall thermal performance of the transfer cask system. The large-scale geometry of the neutron shield tank, which is typically an annulus approximately 2 meters in diameter but only 10–15 cm in thickness, and the relatively small scale velocities (typically less than 5 cm/s) represent a wide range of spatial and temporal scales that contribute to making this a challenging problem for computational fluid dynamics (CFD) modeling. Relevant experimental data at these scales are not available in the literature, but some recent modeling studies offer insights into numerical issues and solutions. However, the geometries in these studies, and for the experimental data in the literature at smaller scales, all have large annular gaps that are not prototypic of the transfer cask neutron shield. This paper proposes that there may be reliable CFD approaches to the transfer cask problem, specifically coupled steady-state solvers or unsteady simulations; however, both of these solutions take significant computational effort. Segregated (uncoupled) steady state solvers that were tested did not accurately capture the flow field and heat transfer distribution in this application. Mesh resolution, turbulence modeling, and the tradeoff between steady state and transient solutions are addressed. Because of the critical nature of this application, the need for new experiments at representative scales is clearly demonstrated.


2013 ◽  
Vol 92 ◽  
pp. 80-86 ◽  
Author(s):  
Åsa Björkbacka ◽  
Saman Hosseinpour ◽  
Magnus Johnson ◽  
Christofer Leygraf ◽  
Mats Jonsson

2017 ◽  
Vol 57 (1) ◽  
pp. 42-53 ◽  
Author(s):  
Vytenis Barkauskas ◽  
Rita Plukienė ◽  
Artūras Plukis ◽  
Vidmantas Remeikis

Depletion of RBMK-1500 spent nuclear fuel (SNF) with and without an erbium burnable absorber was modelled, and one-group burn-up dependent cross-section libraries for Origen-ARP were created. Depletion calculations for the generation of cross-section libraries were performed using the SCALE 6.1 code package with the TRITON control module, which employs the NEWT deterministic 2D transport code with the 238-group energy library based on the ENDF-B VII library and the ORIGEN-S nuclide composition calculation code. Concentrations of the most important actinides for criticality safety were calculated using the created libraries and were compared with the available experimental data and the newest modelling results. Available experimental data of fission products (Nd and Cs isotopes) were also compared to the modelling results. Composition differences were evaluated for several fuel enrichments and water densities. The comparison shows an acceptable agreement between the values obtained using new one-group cross-section libraries and experimental data except for238Pu and241Am, as well as the causes of discrepancy are discussed. It has been found that the enrichment and presence of the burnable absorber play an important role in the SNF composition. At the highest evaluated burn-up (29 GWd/tU) isotopic composition differences between 2% enrichment fuel and 2.8% burn-up for actinides important to burn-up credit (BUC) applications varied from 11 to 52%.


2021 ◽  
Author(s):  
Ghada El Jamal ◽  
Thomas Gouder ◽  
Rachel Eloirdi ◽  
Mats Jonsson

Thin UO2 films exposed to water plasma under UHV conditions have been shown to be interesting models for radiation induced oxidative dissolution of spent nuclear fuel. This is partly attributed...


2008 ◽  
Vol 1107 ◽  
Author(s):  
Melody L. Carter ◽  
E. R. Vance

AbstractThis paper illustrates the benefits of hot isostatically pressed (HIPed) tailored ceramic waste forms for the immobilisation of Cs and Sr separated from spent nuclear fuel. Experimental data on microstructure and aqueous durability are presented for Cs- and Sr-bearing hollanditerich tailored ceramics prepared with 12-18 wt% waste (on an oxide basis). MCC-1 type leach testing, on the sample containing 12 wt% waste at 90°C for 28 days revealed extremely low normalised 7-28-day Cs and Sr release rates of 0.003 and 0.004 g/m2day respectively.


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