scholarly journals Suppressing defects through the synergistic effect of a Lewis base and a Lewis acid for highly efficient and stable perovskite solar cells

2018 ◽  
Vol 11 (12) ◽  
pp. 3480-3490 ◽  
Author(s):  
Fei Zhang ◽  
Dongqin Bi ◽  
Norman Pellet ◽  
Chuanxiao Xiao ◽  
Zhen Li ◽  
...  
Keyword(s):  
Solar Cells ◽  
Synergistic Effect ◽  
Lewis Acid ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Lewis Base ◽  
Highly Efficient ◽  
Synergistic Combination

The synergistic combination of a Lewis base and a Lewis acid enables perovskite solar cells with high efficiency and stability.

scholarly journals A general approach to high-efficiency perovskite solar cells by any antisolvent

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Alexander D. Taylor ◽  
Qing Sun ◽  
Katelyn P. Goetz ◽  
Qingzhi An ◽  
Tim Schramm ◽  
...  
Keyword(s):  
Solar Cells ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Precursor Solution ◽  
Microstructural Characterization ◽  
Application Rate ◽  
Perovskite Layer ◽  
Highly Efficient ◽  
Application Procedure ◽  
Wide Range

AbstractDeposition of perovskite films by antisolvent engineering is a highly common method employed in perovskite photovoltaics research. Herein, we report on a general method that allows for the fabrication of highly efficient perovskite solar cells by any antisolvent via manipulation of the antisolvent application rate. Through detailed structural, compositional, and microstructural characterization of perovskite layers fabricated by 14 different antisolvents, we identify two key factors that influence the quality of the perovskite layer: the solubility of the organic precursors in the antisolvent and its miscibility with the host solvent(s) of the perovskite precursor solution, which combine to produce rate-dependent behavior during the antisolvent application step. Leveraging this, we produce devices with power conversion efficiencies (PCEs) that exceed 21% using a wide range of antisolvents. Moreover, we demonstrate that employing the optimal antisolvent application procedure allows for highly efficient solar cells to be fabricated from a broad range of precursor stoichiometries.

Toward high-efficiency, hysteresis-less, stable perovskite solar cells: unusual doping of a hole-transporting material using a fluorine-containing hydrophobic Lewis acid

2018 ◽  
Vol 11 (8) ◽  
pp. 2035-2045 ◽  
Author(s):  
Junsheng Luo ◽  
Jianxing Xia ◽  
Hua Yang ◽  
Lingling Chen ◽  
Zhongquan Wan ◽  
...  
Keyword(s):  
Solar Cells ◽  
Lewis Acid ◽  
High Efficiency ◽  
State Of The Art ◽  
Perovskite Solar Cells ◽  
Hole Transporting ◽  
Hole Transporting Material ◽  
Effective Dopant

A fluorine-containing hydrophobic Lewis acid is employed as an effective dopant for PTAA to replace state-of-the-art Li-TFSI/t-BP in PSCs.

High‐Efficiency Tin Halide Perovskite Solar Cells: The Chemistry of Tin (II) Compounds and Their Interaction with Lewis Base Additives during Perovskite Film Formation

Solar RRL ◽  
2020 ◽  
pp. 2000606
Author(s):  
Muhammad. Abdel-Shakour ◽  
Towhid H. Chowdhury ◽  
Kiyoto Matsuishi ◽  
Idriss Bedja ◽  
Yutaka Moritomo ◽  
...  
Keyword(s):  
Solar Cells ◽  
High Efficiency ◽  
Film Formation ◽  
Perovskite Solar Cells ◽  
Lewis Base ◽  
Halide Perovskite

scholarly journals Facile all-dip-coating deposition of highly efficient (CH3)3NPbI3−xClx perovskite materials from aqueous non-halide lead precursor

RSC Advances ◽  
2020 ◽  
Vol 10 (48) ◽  
pp. 29010-29017 ◽  
Author(s):  
Muhammad Adnan ◽  
Zobia Irshad ◽  
Jae Kwan Lee
Keyword(s):  
Solar Cells ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Precursor Solution ◽  
Dip Coating ◽  
Coating Deposition ◽  
Highly Efficient ◽  
Perovskite Materials ◽  
Halide Solution

Sequential all-dip-coating processed perovskite materials was conducted in an aqueous non-halide lead precursor solution, which was followed by that in a mixed halide solution for high-efficiency perovskite solar cells.

Lewis Acid–Base Adduct Approach for High Efficiency Perovskite Solar Cells

2016 ◽  
Vol 49 (2) ◽  
pp. 311-319 ◽  
Author(s):  
Jin-Wook Lee ◽  
Hui-Seon Kim ◽  
Nam-Gyu Park
Keyword(s):  
Solar Cells ◽  
Lewis Acid ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Acid Base

scholarly journals Engineering the underlying surface to manipulate the growth of 2D perovskites for highly efficient solar cells

2019 ◽  
Vol 7 (23) ◽  
pp. 14027-14032 ◽  
Author(s):  
Shuoxun Tian ◽  
Jiehuan Chen ◽  
Xiaomei Lian ◽  
Yaqin Wang ◽  
Yingzhu Zhang ◽  
...  
Keyword(s):  
Solar Cells ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Underlying Surface ◽  
Highly Efficient

High efficiency (12.78%) 2D perovskite solar cells are realized by engineering the substrate to manipulate the growth of 2D perovskites.

The synergistic effect of cooperating solvent vapor annealing for high-efficiency planar inverted perovskite solar cells

2019 ◽  
Vol 7 (48) ◽  
pp. 27267-27277 ◽  
Author(s):  
Ahra Yi ◽  
Sangmin Chae ◽  
Hanbin Lee ◽  
Hyo Jung Kim
Keyword(s):  
Solar Cells ◽  
Synergistic Effect ◽  
Treatment Process ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Solvent Vapor ◽  
Vapor Annealing ◽  
Solvent Vapor Annealing ◽  
Post Treatment Process

We propose co-solvent vapor annealing (SVA) as an effective post-treatment process to improve the quality of crystals and grains for high-efficiency perovskite solar cells.

Dopant-free polymeric hole transport materials for highly efficient and stable perovskite solar cells

2016 ◽  
Vol 9 (7) ◽  
pp. 2326-2333 ◽  
Author(s):  
Guan-Woo Kim ◽  
Gyeongho Kang ◽  
Jinseck Kim ◽  
Gang-Young Lee ◽  
Hong Il Kim ◽  
...  
Keyword(s):  
Solar Cells ◽  
Solar Cell ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Perovskite Solar Cell ◽  
Hole Transport ◽  
Highly Efficient

A dopant–free polymeric hole transport material (HTM), RCP, based on benzo[1,2-b:4,5:b′]dithiophene and 2,1,3-benzothiadiazole exhibited a high efficiency of 17.3% in a perovskite solar cell and maintained its initial efficiency for over 1400 hours.

Achieving high efficiency and improved stability in large-area ITO-free perovskite solar cells with thiol-functionalized self-assembled monolayers

2016 ◽  
Vol 4 (20) ◽  
pp. 7903-7913 ◽  
Author(s):  
Chih-Yu Chang ◽  
Yu-Chia Chang ◽  
Wen-Kuan Huang ◽  
Wen-Chi Liao ◽  
Hung Wang ◽  
...  
Keyword(s):  
Solar Cells ◽  
High Efficiency ◽  
Perovskite Solar Cells ◽  
Self Assembled Monolayers ◽  
Large Area ◽  
Highly Efficient ◽  
Interfacial Modification ◽  
Assembled Monolayers ◽  
Improved Stability ◽  
Self Assembled

A promising approach towards highly efficient and stable large-area ITO-free perovskite solar cells is demonstrated by employing thiol-functionalized self-assembled monolayers as interfacial modification layers.

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