Role of Oxygen-Bound Reaction Intermediates in Selective Electrochemical CO2 Reduction

2021 ◽  
Author(s):  
Xing Zhi ◽  
Anthony Vasileff ◽  
Yao Zheng ◽  
Yan Jiao ◽  
Shizhang Qiao
Keyword(s):  
Co2 Reduction ◽  
Reduction Reaction ◽  
Reaction Pathways ◽  
Reaction Intermediates ◽  
Electrochemical Co2 Reduction ◽  
End Products ◽  
Co2 Reduction Reaction

The electrochemical CO2 reduction reaction (CRR) is intrinsically complex given the multiple possible reaction pathways and end products. Consequently, selectivity is a persistent challenge for the design and operation of...

Understanding the role of axial O in CO2 electroreduction on NiN4 single-atom catalysts via simulations in realistic electrochemical environment

2021 ◽  
Author(s):  
Xu Hu ◽  
Sai Yao ◽  
Letian Chen ◽  
Xu Zhang ◽  
Menggai Jiao ◽  
...  
Keyword(s):  
Sustainable Development ◽  
Heterogeneous Catalysis ◽  
Co2 Reduction ◽  
Reduction Reaction ◽  
Single Atom ◽  
Electrochemical Co2 Reduction ◽  
Co2 Electroreduction ◽  
Important Approach ◽  
Co2 Reduction Reaction

Electrochemical CO2 reduction reaction (CO2RR) is a very important approach to realize sustainable development. Single-atom catalysts show advantages in both homogeneous and heterogeneous catalysis, and considerable progress has been made...

Tandem catalysis in electrochemical CO2 reduction reaction

Nano Research ◽  
2021 ◽  
Author(s):  
Yating Zhu ◽  
Xiaoya Cui ◽  
Huiling Liu ◽  
Zhenguo Guo ◽  
Yanfeng Dang ◽  
...  
Keyword(s):  
Co2 Reduction ◽  
Reduction Reaction ◽  
Tandem Catalysis ◽  
Electrochemical Co2 Reduction ◽  
Co2 Reduction Reaction

Atomic regulation of metal-organic framework derived carbon-based single-atom catalysts for electrochemical CO2 reduction reaction

2021 ◽  
Author(s):  
Danni Zhou ◽  
Xinyuan Li ◽  
Huishan Shang ◽  
Fengjuan Qin ◽  
Wenxing Chen
Keyword(s):  
Active Sites ◽  
Metal Organic Framework ◽  
Co2 Reduction ◽  
Carbon Dioxide Reduction ◽  
Reduction Reaction ◽  
Single Atom ◽  
Electrochemical Co2 Reduction ◽  
Metal Organic ◽  
Co2 Reduction Reaction ◽  
Organic Framework

Metal-organic framework (MOF) derived single-atom catalysts (SACs), featured unique active sites and adjustable topological structures, exhibit high electrocatalytic performance on carbon dioxide reduction reactions (CO2RR). By modulating elements and atomic...

A Wide Range of CO : H2 Syngas Proportions Enabled by Tellurization-Induced Amorphous Telluride-Palladium Surface

2021 ◽  
Author(s):  
Kailei Cao ◽  
Yujin Ji ◽  
Shuxing Bai ◽  
Xiaoqing Huang ◽  
Youyong Li ◽  
...  
Keyword(s):  
Co2 Reduction ◽  
Reduction Reaction ◽  
Direct Production ◽  
Environmental Friendly ◽  
Electrochemical Co2 Reduction ◽  
Wide Range ◽  
Palladium Surface ◽  
Co2 Reduction Reaction

The direct production of syngas via electrochemical CO2 reduction reaction (CO2RR) is a highly potential process for its environmental-friendly and product adjustability advantages. However, it is challenging to synthesize syngas...

scholarly journals Optimizing the use of a “Zero-Gap” Gas Diffusion Electrode Setup for Electrochemical Reduction of CO2

2021 ◽  
Author(s):  
Shima Alinejad ◽  
Jonathan Quinson ◽  
Yao Li ◽  
Ying Kong ◽  
Sven Reichenberger ◽  
...  
Keyword(s):  
Co2 Reduction ◽  
Catalyst Layer ◽  
Gas Diffusion ◽  
Reduction Reaction ◽  
Gas Diffusion Electrode ◽  
Test Bed ◽  
Catalyst Screening ◽  
Electrochemical Co2 Reduction ◽  
Reduction Of Co2 ◽  
Co2 Reduction Reaction

The lack of a robust and standardized experimental test bed to investigate the performance of catalyst materials for the electrochemical CO2 reduction reaction (ECO2RR) is one of the major challenges in this field of research. To best reproduce and mimic commercially relevant conditions for catalyst screening and testing, gas diffusion electrode (GDE) setups attract a rising attention as an alternative to conventional aqueous-based setups such as the H-cell configuration. In particular a zero-gap design shows promising features for upscaling to the commercial scale. In this study, we develop further our recently introduced zero-gap GDE setup for the CO2RR using an Au electrocatalyst as model system and identify/report the key experimental parameters to control in the catalyst layer preparation in order to optimize the activity and selectivity of the catalyst.

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