A New Beamline For Time Resolved And Extreme Conditions X-Ray Absorption Spectroscopy

Author(s):  
Olivier Mathon ◽  
Trevor Mairs ◽  
Sakura Pascarelli ◽  
R. Garrett ◽  
I. Gentle ◽  
...  
2016 ◽  
Vol 23 (1) ◽  
pp. 353-368 ◽  
Author(s):  
S. Pascarelli ◽  
O. Mathon ◽  
T. Mairs ◽  
I. Kantor ◽  
G. Agostini ◽  
...  

The European Synchrotron Radiation Facility has recently made available to the user community a facility totally dedicated to Time-resolved and Extreme-conditions X-ray Absorption Spectroscopy – TEXAS. Based on an upgrade of the former energy-dispersive XAS beamline ID24, it provides a unique experimental tool combining unprecedented brilliance (up to 1014 photons s−1on a 4 µm × 4 µm FWHM spot) and detection speed for a full EXAFS spectrum (100 ps per spectrum). The science mission includes studies of processes down to the nanosecond timescale, and investigations of matter at extreme pressure (500 GPa), temperature (10000 K) and magnetic field (30 T). The core activities of the beamline are centered on new experiments dedicated to the investigation of extreme states of matter that can be maintained only for very short periods of time. Here the infrastructure, optical scheme, detection systems and sample environments used to enable the mission-critical performance are described, and examples of first results on the investigation of the electronic and local structure in melts at pressure and temperature conditions relevant to the Earth's interior and in laser-shocked matter are given.


2004 ◽  
Vol 75 (1) ◽  
pp. 24-30 ◽  
Author(s):  
Melanie Saes ◽  
Frank van Mourik ◽  
Wojciech Gawelda ◽  
Maik Kaiser ◽  
Majed Chergui ◽  
...  

1997 ◽  
Vol 7 (C2) ◽  
pp. C2-31-C2-38 ◽  
Author(s):  
J. P. Itié ◽  
A. Polian ◽  
D. Martinez ◽  
V. Briois ◽  
A. Di Cicco ◽  
...  

2022 ◽  
Vol 29 (1) ◽  
Author(s):  
Yujin Kim ◽  
Daewoong Nam ◽  
Rory Ma ◽  
Sangsoo Kim ◽  
Myung-jin Kim ◽  
...  

Understanding the ultrafast dynamics of molecules is of fundamental importance. Time-resolved X-ray absorption spectroscopy (TR-XAS) is a powerful spectroscopic technique for unveiling the time-dependent structural and electronic information of molecules that has been widely applied in various fields. Herein, the design and technical achievement of a newly developed experimental apparatus for TR-XAS measurements in the tender X-ray range with X-ray free-electron lasers (XFELs) at the Pohang Accelerator Laboratory XFEL (PAL-XFEL) are described. Femtosecond TR-XAS measurements were conducted at the Ru L 3-edge of well known photosensitizer tris(bipyridine)ruthenium(II) chloride ([Ru(bpy)3]2+) in water. The results indicate ultrafast photoinduced electron transfer from the Ru center to the ligand, which demonstrates that the newly designed setup is applicable for monitoring ultrafast reactions in the femtosecond domain.


2009 ◽  
Vol 96 (1) ◽  
pp. 11-18 ◽  
Author(s):  
G. Gavrila ◽  
K. Godehusen ◽  
C. Weniger ◽  
E. T. J. Nibbering ◽  
T. Elsaesser ◽  
...  

2019 ◽  
Vol 100 (18) ◽  
Author(s):  
Silvia Boccato ◽  
Raffaella Torchio ◽  
Paola D'Angelo ◽  
Angela Trapananti ◽  
Innokenty Kantor ◽  
...  

2019 ◽  
Vol 216 ◽  
pp. 414-433 ◽  
Author(s):  
Johannes Mahl ◽  
Stefan Neppl ◽  
Friedrich Roth ◽  
Mario Borgwardt ◽  
Catherine Saladrigas ◽  
...  

Laser-induced energy deposition and heat transport in CuO is studied by picosecond time-resolved X-ray absorption spectroscopy.


2020 ◽  
Vol 56 (71) ◽  
pp. 10329-10332 ◽  
Author(s):  
Paulo F. M. de Oliveira ◽  
Adam A. L. Michalchuk ◽  
Ana Guilherme Buzanich ◽  
Ralf Bienert ◽  
Roberto M. Torresi ◽  
...  

A new tandem approach combines XRD and XANES for time-resolved in situ monitoring of the mechanochemical synthesis of gold nanoparticles.


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