Observation of three resonances in the third harmonic generation spectrum of conjugated polymers: Evidence for the four‐level essential states model

1994 ◽  
Vol 100 (2) ◽  
pp. 1665-1672 ◽  
Author(s):  
S. Mazumdar ◽  
F. Guo
Keyword(s):  
Conjugated Polymers ◽  
Harmonic Generation ◽  
Third Harmonic Generation ◽  
Third Harmonic ◽  
Generation Spectrum ◽  
The Third

Nonlinear Optical Properties of Two Thiophene-Based Polyconjugated Systems: Photoinduced Absorption and Third Harmonic Generation Spectroscopy

1989 ◽  
Vol 173 ◽  
Author(s):  
R. Zamboni ◽  
C. Taliani ◽  
G. Ruani ◽  
A. J. Pal ◽  
F. Kajzar
Keyword(s):  
Optical Properties ◽  
Conjugated Polymers ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Third Harmonic Generation ◽  
Nonlinear Optical Properties ◽  
Photoinduced Absorption ◽  
Third Harmonic ◽  
Optical Gap ◽  
The Third

ABSTRACTNonlinear optical properties of two thiophene-based conjugated polymers (PTT and PDTB) were studied by the photoinduced absorption spectroscopy and the third harmonic generation spectroscopy. The results obtained with these two methods are used to estimate the value of χ(3) in these materials. Resonant χ(3) are (2.0 ± 0.2) × 10−11 e.s.u. and (1.0 ± 0.1) × 10−11 e.s.u. for PTT and PDTB, respectively. χ(3) is shown to be related to the width of the optical gap through a sixth-power law. In PTT a vibronic structure due to the C = C stretching mode appears in the χ(3) spectrum.

scholarly journals Ultrafast Third-Order Nonlinear Optical Response Excited by fs Laser Pulses at 1550 nm in GaN Crystals

Materials ◽  
2021 ◽  
Vol 14 (12) ◽  
pp. 3194
Author(s):  
Adrian Petris ◽  
Petronela Gheorghe ◽  
Tudor Braniste ◽  
Ion Tiginyanu
Keyword(s):  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Laser Pulses ◽  
Third Harmonic Generation ◽  
High Repetition Rate ◽  
Third Order ◽  
Third Harmonic ◽  
The Third ◽  
High Repetition ◽  
Gan Crystal

The ultrafast third-order optical nonlinearity of c-plane GaN crystal, excited by ultrashort (fs) high-repetition-rate laser pulses at 1550 nm, wavelength important for optical communications, is investigated for the first time by optical third-harmonic generation in non-phase-matching conditions. As the thermo-optic effect that can arise in the sample by cumulative thermal effects induced by high-repetition-rate laser pulses cannot be responsible for the third-harmonic generation, the ultrafast nonlinear optical effect of solely electronic origin is the only one involved in this process. The third-order nonlinear optical susceptibility of GaN crystal responsible for the third-harmonic generation process, an important indicative parameter for the potential use of this material in ultrafast photonic functionalities, is determined.

Enhancement of the third harmonic generation during interaction of several beams

2018 ◽  
Author(s):  
D.V. Mokrousova ◽  
G.E. Rizaev ◽  
A.V. Shalova ◽  
D.E. Shipilo ◽  
N.A. Panov ◽  
...  
Keyword(s):  
Harmonic Generation ◽  
Third Harmonic Generation ◽  
Third Harmonic ◽  
The Third

Third-Harmonic Generation in Special Parabolic Quantum Wells

2013 ◽  
Vol 760-762 ◽  
pp. 392-396
Author(s):  
You Bin Yu
Keyword(s):  
Quantum Well ◽  
Density Matrix ◽  
Quantum Wells ◽  
Harmonic Generation ◽  
Third Harmonic Generation ◽  
Third Harmonic ◽  
The Third ◽  
Compact Density ◽  
Asymmetric Quantum ◽  
Parabolic Quantum Wells

Third-harmonic generation in a special asymmetric quantum well is investigated. The third-harmonic generation coefficient is carried out by applying compact-density-matrix method. The numerical results are presented for a GaAs/AlGaAs asymmetric quantum well. The very large third-harmonic generation coefficient is obtained in this quantum well. Moreover, the third-harmonic generation coefficient dependents on the quantum well parameters are investigated, respectively.

Third-harmonic-generation spectroscopy of poly(p-phenylenevinylene): A comparison with oligomers and scaling laws for conjugated polymers

1996 ◽  
Vol 53 (8) ◽  
pp. 4367-4376 ◽  
Author(s):  
A. Mathy ◽  
K. Ueberhofen ◽  
R. Schenk ◽  
H. Gregorius ◽  
R. Garay ◽  
...  
Keyword(s):  
Conjugated Polymers ◽  
Harmonic Generation ◽  
Scaling Laws ◽  
Third Harmonic Generation ◽  
Third Harmonic
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