Abstract. China has been experiencing severe air pollution in recent decades. Although ambient air quality monitoring network for criteria pollutants has been constructed in over 100 cities since 2013 in China, the temporal and spatial characteristics of some important pollutants, such as particulate matter (PM) components, remain unknown, limiting further studies investigating potential air pollution control strategies to improve air quality and associating human health outcomes with air pollution exposure. In this study, a yearlong (2013) air quality simulation using the Weather Research & Forecasting model (WRF) and the Community Multi-scale Air Quality model (CMAQ) was conducted to provide detailed temporal and spatial information of ozone (O3), PM2.5 total and chemical components. Multi-resolution Emission Inventory for China (MEIC) was used for anthropogenic emissions and observation data obtained from the national air quality monitoring network were collected to validate model performance. The model successfully reproduces the O3 and PM2.5 concentrations at most cities for most months, with model performance statistics meeting the performance criteria. However, over-prediction of O3 generally occurs at low concentration range while under-prediction of PM2.5 happens at low concentration range in summer. Spatially, the model has better performance in Southern China than in Northern, Central and Sichuan basin. Strong seasonal variations of PM2.5 exist and wind speed and direction play important roles in high PM2.5 events. Secondary components have more boarder distribution than primary components. Sulfate (SO42−), nitrate (NO3−), ammonium (NH4+), and primary organic aerosol (POA) are the most important PM2.5 components. All components have the highest concentrations in winter except secondary organic aerosol (SOA). This study proves the ability of CMAQ model in reproducing severe air pollution in China, identifies the directions where improvements are needed, and provides information for human exposure to multiple pollutants for assessing health effects.
A data-driven approach for optimal design of integrated air quality monitoring network in a chemical cluster
