Perturbative calculation of the ac Stark effect by the complex rotation method

1991 ◽  
Vol 43 (11) ◽  
pp. 6272-6283 ◽  
Author(s):  
Liwen Pan ◽  
K. T. Taylor ◽  
Charles W. Clark
2001 ◽  
Vol 79 (2-3) ◽  
pp. 533-545 ◽  
Author(s):  
W L Meerts ◽  
I Ozier ◽  
J T Hougen

An unusual type of nonresonant absorption signal produced by the ac Stark effect has been observed in a two-level avoided-crossing system. The theory for these anomalous transitions has been developed. The nonresonant signals have been shown to be caused by the perturbation by the oscillating field of the dephasing of the two-level system at the avoided crossing. A series of measurements of these anomalous transitions has been carried out using the avoided-crossing molecular-beam electric-resonance technique. In addition, different types of resonant multiphoton transitions have been investigated. Results are reported for the AE-barrier anticrossing with J = 1 in CH3SiH3. The experimental findings are in good agreement with the theory developed. PACS Nos.: 33.20Bx, 33.80Be, 42.50Hz


2012 ◽  
Vol 20 (13) ◽  
pp. 13762 ◽  
Author(s):  
S. Ya. Tochitsky ◽  
J. J. Pigeon ◽  
D. J. Haberberger ◽  
C. Gong ◽  
C. Joshi
Keyword(s):  

1988 ◽  
Vol 13 (5) ◽  
pp. 354 ◽  
Author(s):  
J. Coutts ◽  
J. Cooper ◽  
K. Burnett

1994 ◽  
Vol 72 (11-12) ◽  
pp. 1273-1283 ◽  
Author(s):  
A. F. Linskens ◽  
N. Dam ◽  
J. R. Reuss ◽  
B. Sartakov

A system is described in which a real molecular state is tuned into and out of resonance with the intermediate level of a two-photon transition, by the laser-induced ac-Stark effect. Two narrow-band CO2 wave-guide lasers are utilized to induce rovibrational transitions in the ν3 ladder of SF6. A weak probe laser monitors the absorption for the [Formula: see text] two-photon transition. Simultaneously, a strong pump laser is in resonance with the [Formula: see text] one-photon transition. The ac-Stark splitting is observed and quantum interferences between two-photon amplitudes involving different intermediate states occur. It is demonstrated that destructive interference allows suppression of the two-photon excitation for an appropriate pump laser power. Simulations based on the Dressed State Picture and the optical Bloch equations show a satisfactory agreement with the experiment.


1989 ◽  
Vol 62 (10) ◽  
pp. 1189-1192 ◽  
Author(s):  
W. H. Knox ◽  
D. S. Chemla ◽  
D. A. B. Miller ◽  
J. B. Stark ◽  
S. Schmitt-Rink

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