EVIDENCE FOR AN (n, α) REACTION INDUCED IN O17 BY THERMAL NEUTRONS

1947 ◽  
Vol 25a (2) ◽  
pp. 77-87 ◽  
Author(s):  
A. N. May ◽  
E. P. Hincks

It can be shown from the masses involved that the reaction O17 (n, α) C14 should be exothermic by 1.72 Mev., and should therefore occur with thermal neutrons. As an attempt to detect the reaction an investigation was made of the pulse spectrum produced when an ionization chamber containing oxygen was placed in a flux of thermal neutrons. The pulses were amplified and then counted in a series of energy bands by means of a kicksorter. Two oxygen samples were compared, one being enriched (three times normal), and the other impoverished (0.5 times normal), in O17. Differences between runs with these two gases showed a considerable number of pulses between 1 and 2 Mev., with a maximum at 1.4 Mev. Reasons are given for assigning these pulses to the above reaction, including considerations of the possibility that other exothermic neutron reactions occur. By comparing the number of pulses with the number produced by N14 (n, p) C14 when the chamber contained air, a value of (1.9 ± 0.5) × 10−28 cm.2 for the cross-section for the O17 (n, α) C14 reaction in ordinary oxygen was deduced. This gives a cross-section of (0.46 ± 0.11) × 10−24 cm.2 per atom of the pure isotope O17. The effect measured is about 20% of the total thermal neutron capture cross-section that has been reported for ordinary oxygen.

1956 ◽  
Vol 34 (8) ◽  
pp. 1023-1026 ◽  
Author(s):  
L. P. Roy ◽  
L. Yaffe

The cross section of Ce142 has been determined by the activation method and found to be 0.95 ± 0.05 barns relative to a value of σCo59 = 36.3 barns. Disintegration rates were determined by a 4π counter. The value obtained agrees with that of Katcoff etal. (1949) also obtained by the activation method but differs markedly from that of Pomerance (1952).


1975 ◽  
Vol 15 (02) ◽  
pp. 161-168
Author(s):  
Arthur H. Youmans ◽  
Eric C. Hopkinson

Abstract Commercially available logging services provide a measurement of the lifetime of thermal neutrons in formations adjacent to a borehole. This lifetime provides a measure of the macroscopic thermal neutron-capture cross-section S of the formation. which in turn is functionally related to the abundance and constituency of the rock matrix and contained fluids. Because the measurement is extremely sensitive to an abundance of trace elements like boron and gadolinium, it is very difficult to find rock formations with an accurately known value of S, which is required for the accuracy of the measuring system to be experimentally tested. Various theoretical studies published suggest that errors in the determination of S may occur because of the influence of borehole parameters and the effects of neutron diffusion. Experimental results are reported that demonstrate that the design of the instrument is crucial to the validity of any theoretical treatment of the subject. The influence of neutron diffusion and borehole effects can be overcome by optimal selection of spacing and shielding parameters. INTRODUCTION The lifetime of thermal neutrons in formation materials is a measure of the thermal neutron-capture cross-section of the bulk materials comprising the formation. This parameter, S, is quantitatively related to the elemental constituency of the medium. As such, a log based on the measurement of neutron lifetime1 can be used for identifying fluids in porous rocks when there is a contrast between the values of S for the respective fluids. Where formation waters are saline, the log has been used with great success to detect and evaluate oil-bearing zones behind casing. If S is accurately measured, it may be used to compute an unknown parameter with commensurate accuracy using the following relations.2Equation 1 whereEquation 2 The basic assumption of the logging method is that a population of neutrons in a formation will obey the simple relation N = Noe−Svt if the medium is homogeneous. In a medium penetrated by a borehole, it is assumed that the same kind of relation holds true after some time t1:Equation 3 From this equation, the value of S may be derived by measuring N1 and N2 at two times, t1 and t2.Equation 4 This theory requires two assumptions: that neutrons die or disappear only because of capture in the formation, and that it is possible to measure N, the number of live neutrons at any given time (or rather, the ratio of N1 to N2). About 10 years of commercial logging experience have established that S is, to all intents and purposes, accurately and reliably measured3 by the Neutron Lifetime Log (NLL). * This is true even though the foregoing assumptions are not rigorously true. Neutrons do diffuse4 during the measurement interval, with the result that some leave the formation and enter the borehole where their remaining lifetime is dependent on borehole parameters rather than on the formation. Also, the problem of sampling the neutron population is complicated by the fact that the spatial distribution of neutrons changes during the measurement interval, so that any sampling technique designed to measure N is prone to error, or at least subject to doubt.


1953 ◽  
Vol 31 (3) ◽  
pp. 204-206 ◽  
Author(s):  
Rosalie M. Bartholomew ◽  
R. C. Hawkings ◽  
W. F. Merritt ◽  
L. Yaffe

The thermal neutron capture cross sections of Na23 and Mn55 have been determined using the activation method. The values are 0.53 ± 0.03 and 12.7 ± 0.3 barns respectively with respect to σAul97 = 93 barns. These agree well with recent pile oscillator results. The half-life for Mn56 is found to be 2.576 ± 0.002 hr.


1955 ◽  
Vol 33 (8) ◽  
pp. 457-465 ◽  
Author(s):  
R. E. Bell ◽  
R. L. Graham ◽  
L. Yaffe

The thermal neutron capture cross section of radioactive Au198 has been measured by the activation method as 26,000 ± 1200 barns, assuming 99 barns for the thermal neutron cross section of Au197. Metallic Au197 was bombarded in fluxes up to 9 × 1013 thermal neutrons cm.−2 sec.−1 to produce a mixture of Au198 and Au199 by the successive neutron capture reactions Au197(n, γ)Au198(n, γ)Au199. The ratio of the Au199 activity to Au198 activity so produced yields σc(Au197). In a preliminary experiment, the half-life of Au199 was measured as 3.148 ± 0.010 days.


2007 ◽  
Author(s):  
T. Belgya ◽  
O. Bouland ◽  
G. Noguere ◽  
A. Plompen ◽  
P. Schillebeeckx ◽  
...  

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