THE ABSOLUTE FISSION YIELDS OF TWENTY-EIGHT MASS CHAINS IN THE THERMAL NEUTRON FISSION OF U235

1955 ◽  
Vol 33 (11) ◽  
pp. 693-706 ◽  
Author(s):  
J. A. Petruska ◽  
H. G. Thode ◽  
R. H. Tomlinson
Keyword(s):  
Fine Structure ◽  
Isotope Dilution ◽  
Yield Curve ◽  
Mass Yield ◽  
Absolute Accuracy ◽  
Neutron Fission ◽  
Thermal Neutron Fission ◽  
The Absolute ◽  
Fission Yields ◽  
Better Than

Twenty-eight absolute fission yields totalling 78% of the heavy and 16% of the light fragments have been determined using the mass spectrometer and isotope dilution techniques. The precision of the values obtained is in most cases better than 2% and the absolute accuracy is estimated to be about 3%. Fine structure in the mass–yield curve is discussed in terms of structural preference and various chain branching mechanisms.

THE CUMULATIVE YIELDS OF THE KRYPTON AND XENON ISOTOPES PRODUCED IN THE FAST NEUTRON FISSION OF Th232

1957 ◽  
Vol 35 (8) ◽  
pp. 969-979 ◽  
Author(s):  
T. J. Kennett ◽  
H. G. Thode
Keyword(s):  
Fine Structure ◽  
Fast Neutron ◽  
Isotope Dilution ◽  
Yield Curve ◽  
Mass Yield ◽  
Neutron Fission ◽  
Xenon Isotopes ◽  
Induced Fission ◽  
The Absolute ◽  
Fission Yields

The relative fission yields for mass chains ending in stable krypton and xenon isotopes have been measured for the fast neutron-induced fission of Th232. Isotope dilution techniques were used to determine the krypton/xenon ratio to assist in obtaining the absolute fission yields for these mass chains. The absolute yields were determined by the use of two methods, both giving results which were in excellent agreement. The fine structure observed for the Th232 mass–yield curve is compared with that of heavier fissile nuclides.

CUMULATIVE YIELDS OF THE HEAVY FRAGMENTS IN THE THERMAL-NEUTRON FISSION OF 241Pu

1964 ◽  
Vol 42 (11) ◽  
pp. 2063-2079 ◽  
Author(s):  
H. Farrar ◽  
W. B. Clarke ◽  
H. G. Thode ◽  
R. H. Tomlinson
Keyword(s):  
Fine Structure ◽  
Thermal Neutron ◽  
Isotope Dilution ◽  
Yield Curve ◽  
Mass Spectrometric ◽  
Mass Yield ◽  
General Shape ◽  
Neutron Fission ◽  
Yield Curves ◽  
Thermal Neutron Fission

The relative yields of isotopes of xenon, cesium, barium, cerium, neodymium, and samarium formed by the thermal neutron fission of 241Pu have been obtained by mass spectrometric methods. The relative yields of the elements were normalized by means of the isotope dilution and isobaric techniques, and absolute cumulative yields were determined by summing the relative yields to 100%. The curve obtained for 241Pu is compared with other mass–yield curves. The general shape of this mass–yield curve is similar to that for 239Pu; yet the fine structure shows greater similarity to that for 235U thermal-neutron fission.

Cumulative yields of stable and long-lived isotopes of ruthenium and palladium in neutron-induced fission

1978 ◽  
Vol 56 (10) ◽  
pp. 1340-1352 ◽  
Author(s):  
Masako Shima ◽  
H. G. Thode ◽  
R. H. Tomlinson
Keyword(s):  
Thermal Neutron ◽  
Isotope Dilution ◽  
Yield Curve ◽  
Mass Region ◽  
Mass Yield ◽  
Neutron Fission ◽  
Significant Depression ◽  
Thermal Neutron Fission ◽  
Induced Fission ◽  
Fission Yields

The relative cumulative yields of nine stable and long-lived isotopes of ruthenium and palladium (masses 101 to 110) produced in the thermal neutron fission of 233U and in the thermal and epicadmium neutron fission of 235U and 239Pu have been measured using a solid source mass spectrometer and isotope dilution techniques. Absolute yields of these isotopes for the thermal neutron fission of 233U, 235U, and 239Pu are obtained using normalization procedures. These yields provide the first experimentally determined yields of the palladium masses 105, 106, 107, 108, and 110.In the thermal fission of 233U and 235U the ruthenium isotope yields obtained are in general agreement with previously determined values, although discrepancies exist of the order of 10% at masses 103, 104, and 106 for thermal fission of 235U.A plot of the ruthenium and palladium isotope mass yields together with the previously determined yields for the cadmium and tin isotopes indicate a significant depression in the mass yield curve at masses 111 and 114 for 233U and 235U thermal fission, respectively. In the 235U epicadmium fission, yields at even mass numbers are relatively higher than those at odd numbers, resulting in a zigzag yield curve in the 101 to 110 mass region.

CUMULATIVE YIELDS OF LIGHT FRAGMENTS IN U235 THERMAL NEUTRON FISSION

1962 ◽  
Vol 40 (8) ◽  
pp. 1017-1026 ◽  
Author(s):  
H. Farrar ◽  
H. R. Fickel ◽  
R. H. Tomlinson
Keyword(s):  
Thermal Neutron ◽  
Yield Curve ◽  
Mass Spectrometric Study ◽  
Detailed Examination ◽  
Mass Region ◽  
Mass Yield ◽  
Neutron Fission ◽  
Molybdenum Isotopes ◽  
Thermal Neutron Fission ◽  
Fission Yields

A mass spectrometric study of the relative yields of the strontium, yttrium, zirconium, and molybdenum isotopes formed in the thermal neutron fission of U235 has made possible a detailed examination of structure of the light mass region of the mass–yield curve. The relative yields of this work have been normalized to 5.77% for Sr90, and when literature and extrapolated values are taken for the remaining chains, the fission yields total 100.8%.

Fine structure in the region of symmetric mass distribution for cumulative fission yields

1969 ◽  
Vol 47 (3) ◽  
pp. 275-278 ◽  
Author(s):  
K. S. Thind ◽  
R. H. Tomlinson
Keyword(s):  
Fine Structure ◽  
Yield Curve ◽  
Neutron Emission ◽  
Central Peak ◽  
Mass Region ◽  
Mass Yield ◽  
Neutron Fission ◽  
Energy Neutron ◽  
Cumulative Mass ◽  
Fission Yields

It is predicted that there should be fine structure in the cumulative mass yield curve in the symmetric mass region where major discontinuities in the neutron emission vs. mass curve exist. In the case of low-energy neutron fission of 238U, this fine structure takes the form of a pronounced depression in the region of mass 125. Under similar conditions for 232Th, the fine structure may take the form of depressions in the region of mass 110 and 125 so that the cumulative mass yield curve appears to have a central peak.

STRUCTURE IN THE MASS–YIELD DISTRIBUTION FOR U235 FISSION

1962 ◽  
Vol 40 (8) ◽  
pp. 943-953 ◽  
Author(s):  
H. Farrar ◽  
R. H. Tomlinson
Keyword(s):  
Fine Structure ◽  
Neutron Yield ◽  
Yield Curve ◽  
Detailed Examination ◽  
Mass Yield ◽  
Neutron Fission ◽  
Fission Fragments ◽  
U235 Fission ◽  
Thermal Neutron Fission ◽  
Mass Yield Distribution

Recent measurements of the cumulative yields of essentially all the mass chains in the thermal neutron fission of U235 have enabled a detailed examination of the fine structure in the mass–yield curve. It has been found that most of the structure results from a slowly changing neutron yield as a function of the mass of the primary fission fragments.

THE THERMAL-NEUTRON FISSION YIELDS OF 229Th

1966 ◽  
Vol 44 (5) ◽  
pp. 1011-1019 ◽  
Author(s):  
J. W. Harvey ◽  
W. B. Clarke ◽  
H. G. Thode ◽  
R. H. Tomlinson
Keyword(s):  
Thermal Neutron ◽  
Isotope Dilution ◽  
Mass Spectrometric ◽  
Neutron Fission ◽  
Thermal Neutron Fission ◽  
Mass Group ◽  
The Absolute ◽  
Fission Yields ◽  
Mass Spectrometric Techniques

The relative cumulative yields for isotopes of the elements krypton, strontium, xenon, cesium, cerium, and neodymium formed in the thermal-neutron fission of 229Th have been determined by mass spectrometric techniques. Normalization of the relative yields by means of the isotope dilution and isobaric techniques has allowed estimates to be made of the absolute cumulative yields of the heavy-mass group by forcing the sum of the yields to total 100%.

THE FISSION YIELDS OF THE STABLE AND LONG-LIVED ISOTOPES OF XENON, CESIUM, AND KRYPTON IN NEUTRON FISSION OF U233

1954 ◽  
Vol 32 (8) ◽  
pp. 522-529 ◽  
Author(s):  
W. Fleming ◽  
R. H. Tomlinson ◽  
H. G. Thode
Keyword(s):  
Fine Structure ◽  
Mass Spectrometer ◽  
Yield Curve ◽  
Closed Shell ◽  
Mass Range ◽  
The Other ◽  
Mass Yield ◽  
Fission Yield ◽  
Neutron Fission ◽  
Fission Yields

The fission yields of Xe131, Xe132, Xe134, Xe136, Cs133, Cs135, Cs137, Kr83, Kr84, 10.27 year Kr85, and Kr86 in the neutron fission of U233 have been determined by mass spectrometer methods. The very pronounced fine structure in the mass yield curve in the mass range 131 to 137 found in U235 fission does not occur in the fission of U233. This disappearance of fine structure would not have been predicted by any of the mechanisms which have been suggested to explain the fine structure in U235 fission. The fission yield of the 10.27 year isomer of Kr85 relative to the other krypton isotopes is considerably higher in U233 fission than in U235 fission, indicating some fine structure in this mass range which may be related to the closed shell of 50 neutrons.

THE FISSION YIELDS OF THE CESIUM ISOTOPES FORMED IN THE THERMAL NEUTRON FISSION OF U235 AND THE NEUTRON ABSORPTION CROSS SECTION OF Xe135

1955 ◽  
Vol 33 (11) ◽  
pp. 640-649 ◽  
Author(s):  
J. A. Petruska ◽  
E. A. Melaika ◽  
R. H. Tomlinson
Keyword(s):  
Thermal Neutron ◽  
Cross Section ◽  
Isotope Dilution ◽  
Absorption Cross Section ◽  
Neutron Absorption ◽  
Absorption Cross ◽  
Neutron Fission ◽  
Thermal Neutron Fission ◽  
Fission Yields ◽  
Neutron Absorption Cross Section

The absolute fission yields of the cesium isotopes occurring in the thermal neutron fission of U235 have been determined with a mass spectrometer using isotope dilution techniques. Values of 6.59%, 6.41%, and 6.15% have been obtained for the yields of Cs133, Cs135, and Cs137 respectively. The neutron absorption cross section of Xe135 has also been measured to be 866 times greater than that of B10 for a Maxwellian distribution of neutron velocities corresponding to a neutron temperature of 57 °C. This ratio gives a thermal neutron absorption cross section of 3.47 × 106 barns for Xe135 assuming it is a 1/ν detector.

scholarly journals Relative Yields of Stable Tellurium Isotopes in Neutron-induced Fission

1982 ◽  
Vol 35 (4) ◽  
pp. 385 ◽  
Author(s):  
JR de Laeter ◽  
KJR Rosman ◽  
JW Boldeman
Keyword(s):  
Mass Spectrometry ◽  
Yield Curve ◽  
Mass Range ◽  
Neutron Fission ◽  
Significant Depression ◽  
Isotopic Abundances ◽  
Thermal Neutron Fission ◽  
First Time ◽  
Fission Yields ◽  
Good Agreement

The relative isotopic abundances of four isotopes of tellurium (125, 126, 128 and 130) produced in the thermal neutron fission of 233U and 23SU have been measured for the first time by solid source mass spectrometry. Samples of 233U and 23SU were irradiated in a reactor and chemically separated by ion exchange techniques to permit nanogram-sized samples of fission product tellurium to be analysed mass spectrometrically. The results for 23SU are in good agreement with published radiometric values, whereas our results for 233U are the first experimental measurements in this mass range. The cumulative fission yields determined by mass spectrometry for ruthenium, palladium, cadmium, tin and tellurium show a smooth mass distribution in the symmetric region for both 233U and 235U, except for a significant depression in the yield curve in the range 111-14.

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