Promoting Hot Carrier Extraction in Zn-Ag-In-Te Nanocrystals By Irradiation of High-Energy Light

2020 ◽  
Vol MA2020-02 (27) ◽  
pp. 1880-1880
Author(s):  
Tatsuya Kameyama ◽  
Kota Sugiura ◽  
Susumu Kuwabata ◽  
Tomoki Okuhata ◽  
Naoto Tamai ◽  
...  
2021 ◽  
Author(s):  
Mohammad Eskandari ◽  
Azeez Barzinjy ◽  
Ali Rostami ◽  
Ghasem Rostami ◽  
Mahboubeh Dolatyari

Abstract High-energy coming photons can be absorbed and lead to generate hot carriers. In normal solar cells, these carriers are scattered, by electron-electron and electron-lattice mechanisms, and rapidly lose extra energy then approach the conduction band energy edge. This event in addition to other loss mechanisms causes the efficiency reduction in the solar cells to a limited value, theoretically 33%. Accordingly, the efficiency of solar cells can be enhanced considerably, if one makes the possibility for carriers that can be extracted rapidly before scattering and releasing extra energy to the lattice. This type of solar cell is called hot carrier solar cells (HCSCs). To this end, to improve the conversional efficiency, multilevel energy selective contacts (ESCs) as a new concept and new mechanism in solar cells can be utilized. In the other words, several appropriate energy levels as carrier extraction contacts in the conduction band are introduced. Here, we use multilevel ESCs, and based on our simulation it is shown that the maximum efficiency of 75% is achievable for low bandgap materials. For a typical material such as Si, the maximum efficiency is increased to 60% using ten ESCs.


Author(s):  
Jianfeng Yang ◽  
Yu Feng ◽  
Robert Patterson ◽  
Shujuan Huang ◽  
Santosh Shrestha ◽  
...  

Nanophotonics ◽  
2020 ◽  
Vol 9 (2) ◽  
pp. 453-471 ◽  
Author(s):  
Jacob B. Khurgin

AbstractThe evolution of non-equilibrium carriers excited in the process of decay of surface plasmon polaritons (SPPs) in metal is described for each step – from the generation of carriers to their extraction from the metal. The relative importance of various carrier-generating mechanisms is discussed. It is shown that both the generation of carriers and their decay are inherently quantum processes as, for realistic illumination conditions, no more than a single SPP per nanoparticle exists at a given time. As a result, the distribution of non-equilibrium carriers cannot be described by a single temperature. It is also shown that the originally excited carriers that have not undergone a single electron-electron scattering event are practically the only ones that contribute to the injection. The role of momentum conservation in carrier extraction is discussed, and it is shown that, if all the momentum conservation rules are relaxed, it is the density of states in the semiconductor/dielectric that determines the ultimate injection efficiency. A set of recommendations aimed at improving the efficiency of plasmonic-assisted photodetection and (to a lesser degree) photocatalysis is made in the end.


Author(s):  
Yukihiro Harada ◽  
Naoto Iwata ◽  
Daiki Watanabe ◽  
Shigeo Asahi ◽  
Takashi Kita

2013 ◽  
Vol 411 ◽  
pp. 122-125
Author(s):  
Wei Yu ◽  
Xinzhan Wang ◽  
Wanlei Dai ◽  
Yumei Liu ◽  
Yanmei Xu ◽  
...  

2001 ◽  
Vol 15 (17n19) ◽  
pp. 692-695
Author(s):  
G. FONTHAL ◽  
L. E. TOBÓN ◽  
J. QUINTERO ◽  
N. PIRAQUIVE ◽  
H. ARIZA-CALDERÓN

We analyzed the photoluminescence (PL) spectra on heavily doped GaAs:Sn samples by Kane's theory including a Lorentzian, a Gaussian and the hot carrier temperature. The band gap, the Fermi level, and the Urbach tail were the fitting parameters. Good results were obtained when the theoretical and experimental values were compared for the three parameters. The Urbach energy magnitude and the topological disorder parameter increased when the impurity concentration augment. The average phononic participation was very close with the tabulated values. New information about a shoulder in the high energy side was obtained, too.


Nano Letters ◽  
2016 ◽  
Vol 16 (12) ◽  
pp. 8036-8036
Author(s):  
Roberto Urcuyo ◽  
Dinh Loc Duong ◽  
Patrick Sailer ◽  
Marko Burghard ◽  
Klaus Kern

Author(s):  
Andris Šutka ◽  
Martins Zubkins ◽  
Artis Linarts ◽  
Linards Lapčinskis ◽  
Kaspars Ma̅lnieks ◽  
...  

2019 ◽  
Vol 214 ◽  
pp. 387-397 ◽  
Author(s):  
Jorge U. Salmón-Gamboa ◽  
Mayela Romero-Gómez ◽  
Diane J. Roth ◽  
Matthew J. Barber ◽  
Pan Wang ◽  
...  

Plasmonic heterostructures were designed to optimize hot carrier extraction by controlling nanoparticle surface states.


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