Resonance mode analysis of DNA self-assembled metamolecules with an effective refractive index model

2022 ◽  
Author(s):  
Masashi Fukuhara ◽  
Yoshiaki Tachiiri
Author(s):  
Iltai (Isaac) Kim ◽  
Kenneth David Kihm

Innovative optical techniques based on nano-biophotonics such as surface plasmon resonance (SPR) imaging and R-G-B natural fringe mapping techniques are developed to characterize the transport and optical properties of nanofluids in situ, real-time, and full field manner. Recent results regarding the characterization of nanofluids are summarized and future research directions are presented. 47 nm Al2O3 nanoparticles are dispersed in water with various concentrations. Al2O3 nanofluids droplets are placed on substrates and evaporated in room temperature. In-situ visualization of evaporation-induced self-assembly is conducted to detect concentration, effective refractive index, and different self-assembled pattern including cavity with various nanofluids concentrations and surface hydrophobbicities with SPR and fringe mapping. During the evaporation, time-dependent and near-field nanoparticle concentrations are determined by correlating the SPR reflectance intensities with the effective refractive index (ERI) of the nanofluids. With increasing the concentrations of nanofluids, the existence of hidden complex cavities inside a self-assembled nanocrystalline structure or final dryout pattern is discovered in real-time. R-G-B natural fringe mapping allowed the reconstruction of the 3D cavity formation and crystallization processes quantitatively. The formation of the complex inner structure was found to be attributable to multiple cavity inceptions and their competing growth during the aquatic evaporation. Furthermore, the effect of surface hydrophobicity is examined in the formation of hidden complex cavities, taking place on three different substrates bearing different levels of hydrophobicity; namely, cover glass (CG), gold thin film (Au), and polystyrene dish (PS). These surface plamson resonance imaging and natural fringe mapping techniques are expected to provide a breakthrough in micro-nanoscale thermal fluids phenomena and nano-biochemical sensing when coupled with localized surface Plasmon and metamaterials techniques.


2007 ◽  
Author(s):  
Te-Hung Chang ◽  
Yu-Wen Yeh ◽  
Sheng-Hui Chen ◽  
Cheng-Chung Lee

2021 ◽  
Vol 13 (4) ◽  
pp. 723
Author(s):  
Hossain Zadhoush ◽  
Antonios Giannopoulos ◽  
Iraklis Giannakis

Estimating the permittivity of heterogeneous mixtures based on the permittivity of their components is of high importance with many applications in ground penetrating radar (GPR) and in electrodynamics-based sensing in general. Complex Refractive Index Model (CRIM) is the most mainstream approach for estimating the bulk permittivity of heterogeneous materials and has been widely applied for GPR applications. The popularity of CRIM is primarily based on its simplicity while its accuracy has never been rigorously tested. In the current study, an optimised shape factor is derived that is fine-tuned for modelling the dielectric properties of concrete. The bulk permittivity of concrete is expressed with respect to its components i.e., aggregate particles, cement particles, air-voids and volumetric water fraction. Different combinations of the above materials are accurately modelled using the Finite-Difference Time-Domain (FDTD) method. The numerically estimated bulk permittivity is then used to fine-tune the shape factor of the CRIM model. Then, using laboratory measurements it is shown that the revised CRIM model over-performs the default shape factor and provides with more accurate estimations of the bulk permittivity of concrete.


2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Pavel Malakhovsky ◽  
Dmitry Murausky ◽  
Dmitry Guzatov ◽  
Sergey Gaponenko ◽  
Mikhail Artemyev

Abstract We examined systematically how self-assembled monolayers (SAMs) of different mercaptoacids affect the spectral shift of the localized surface plasmon resonance in silver nanoplates and nanospheres. We observed a clear trend in the magnitude of a redshift with a molecular length or the SAM thickness within a homologous series of aliphatic mercaptoacids: the thicker shell the stronger the red shift. Using classic Mie theory for plasmonic core-dielectric shell spheres and oblate spheroids we developed the method for determination of a pseudo-refractive index in SAM of different molecules and obtained a good correlation with the reference refractive indices for bulk long-chain aliphatic acids, but only in case of silver nanoplates. Calculations for silver core–shell nanospheres gave overestimated values of refractive index perhaps due to restrictions of Mie theory on the minimum particle size.


2007 ◽  
Vol 21 (30) ◽  
pp. 5075-5089 ◽  
Author(s):  
HALA M. KHALIL ◽  
MOHAMMED M. SHABAT ◽  
SOFYAN A. TAYA ◽  
MAZEN M. ABADLA

In this work, we present an extensive theoretical analysis of nonlinear optical waveguide sensor. The waveguide under consideration consists of a thin dielectrica film surrounded by a self-focused nonlinear cladding and a linear substrate. The nonlinearity of the cladding is considered to be of Kerr-type. Both cases, when the effective refractive index is greater and when it is smaller than the index of the guiding layer, are discussed. The sensitivity of the effective refractive index to any change in the cladding index in evanescent optical waveguide sensor is derived for TM modes. Closed form analytical expressions and normalized charts are given to provide the conditions required for the sensor to exhibit its maximum sensitivity. The results are compared with those of the well-known linear evanescent waveguide sensors.


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