scholarly journals Harmonic generation with multi-layer dielectric metasurfaces

Nanophotonics ◽  
2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Giuseppe Marino ◽  
Davide Rocco ◽  
Carlo Gigli ◽  
Grégoire Beaudoin ◽  
Konstantinos Pantzas ◽  
...  

Abstract Metasurfaces have recently gained extensive interest because of their extraordinary optical behavior as artificial material interfaces with ultrahigh compactness. In this framework, dielectric platforms have newly become very promising for nonlinear nanophotonics, providing opportunities, especially for ultrafast optical switching, and high harmonic generation, opening the research field of nonlinear metaoptics. Up to now, nonlinear metaoptics have been mostly explored using single metasurfaces. However, in a long-term vision, the stacking of optical metasurfaces, very challenging in terms of fabrication, is one key goal of this research field. Here, we demonstrate a three-layer metasurface in the AlGaAs-on-insulator platform, which improves the second harmonic generation efficiency by more than one order of magnitude with respect to its one-layer counterpart. Our achievement paves the way toward phase-shaping multilayer and multifunctional all-dielectric metasurfaces.

2020 ◽  
Vol 183 ◽  
pp. 108739
Author(s):  
Shivani ◽  
Ishpreet Kaur ◽  
Karthika Chemmanghattu ◽  
Paramjit Kaur ◽  
Kamaljit Singh

2021 ◽  
Vol 7 (21) ◽  
pp. eabe2265
Author(s):  
Tobias Helk ◽  
Emma Berger ◽  
Sasawat Jamnuch ◽  
Lars Hoffmann ◽  
Adeline Kabacinski ◽  
...  

The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties has limited the availability of nonlinear XUV and x-ray spectroscopies to free-electron lasers (FELs). Here, we demonstrate second harmonic generation (SHG) on a table-top XUV source by observing SHG near the Ti M2,3 edge with a high-harmonic seeded soft x-ray laser. Furthermore, this experiment represents the first SHG experiment in the XUV. First-principles electronic structure calculations suggest the surface specificity and separate the observed signal into its resonant and nonresonant contributions. The realization of XUV-SHG on a table-top source opens up more accessible opportunities for the study of element-specific dynamics in multicomponent systems where surface, interfacial, and bulk-phase asymmetries play a driving role.


2001 ◽  
Vol 15 (28n30) ◽  
pp. 3628-3632 ◽  
Author(s):  
M. Ashida ◽  
T. Ogasawara ◽  
N. Motoyama ◽  
H. Eisaki ◽  
S. Uchida ◽  
...  

The dimensionality dependence of optical nonlinearity in cuprates was investigated by sub-picosecond pump-probe transmission measurements in the near-infrared region. It was found that cuprates with one-dimensional Cu-O networks show nonlinearity one order of magnitude larger than that of conventional band semiconductors and picosecond relaxation of the excited state. In contrast, a two-dimensional cuprate shows one order of magnitude smaller nonlinearity and slower decay of the excited state, as well as picosecond relaxation. The possibility for application of the present material to all-optical switching devices is also discussed.


2020 ◽  
Vol 3 (1) ◽  
Author(s):  
Muhammad Khalid ◽  
Cristian Ciracì

AbstractSecond-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length scales, quantum mechanical effects come into play which could be crucial for an accurate description of plasmonic systems. In this article, we develop a theoretical model based on the quantum hydrodynamic description to study free-electron nonlinear dynamics in plasmonic systems. Our model predicts strong resonances induced by the spill-out of electron density at the metal surface. We show that these resonances can boost second-harmonic generation efficiency up to four orders of magnitude and can be arbitrarily tuned by controlling the electron spill-out at the metal surface with the aid of thin dielectric layers. These results offer a possibility to artificially increase nonlinear susceptibilities by engineering optical properties at the quantum level.


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