Plasmonic Properties of Al2O3 Nanoshell with a Metallic Core

2021 ◽  
Vol 13 ◽  
Author(s):  
Jyoti Katyal

Background: Al is the promising candidate for the deep UV and longer wavelength range plasmonic applications. But it is difficult to have the pure Aluminium nanostructure as it is easily oxidized forming a thin layer of Al2O3. In this paper we have evaluated the field enhancement of oxide layer on metallic shell (Al-Al2O3 and Au- Al2O3) for single and dimer core-shell configuration and shown potential of oxide layer in SERS. Methods: The Finite Difference Time Domain (FDTD) has been used to evaluated the LSPR and field enhancement of single and dimer Al-Al2O3 and Au- Al2O3 nanostructure. Results: The results exhibit the tunable plasmon resonance on varying the inner and outer radii of the Al2O3 shell. A redshift and decrease in enhancement were observed as shell thickness increases whereas on increasing the core size the enhancement gets increased in the case of Au-Al2O3 and gets a decrease in Al-Al2O3 due to quadrupole contribution. But on comparing the Au-Al2O3 with Al-Al2O3 for the same particle size, Al-Al2O3 shows larger enhancement because Au has to compete with its inter band transition. Conclusion: By optimizing the thickness of the shell and core size, it can be concluded that an ultrathin shell of Al2O3 can give higher enhancement. With Al as a core metal the enhancement increases as compared to Au-Al2O3. Since a single Al-Al2O3 nanoshell has shown a huge enhancement we have considered the multimer configuration of two identical nanoshell. Due to coupling between two nanoshell a huge increase in enhancement factor ~1012 was observed for Al-Al2O3 dimer nanoshell in the UV region.

Crystals ◽  
2021 ◽  
Vol 11 (4) ◽  
pp. 420
Author(s):  
Ang Deng ◽  
Wonkeun Chang

We numerically investigate the effect of scaling two key structural parameters in antiresonant hollow-core fibers—dielectric wall thickness of the cladding elements and core size—in view of low-loss mid-infrared beam delivery. We demonstrate that there exists an additional resonance-like loss peak in the long-wavelength limit of the first transmission band in antiresonant hollow-core fibers. We also find that the confinement loss in tubular-type hollow-core fibers depends strongly on the core size, where the degree of the dependence varies with the cladding tube size. The loss scales with the core diameter to the power of approximately −5.4 for commonly used tubular-type hollow-core fiber designs.


2008 ◽  
Vol 1142 ◽  
Author(s):  
Feng Jin ◽  
Yan Liu ◽  
Scott A Little ◽  
Chris M Day

ABSTRACTWe have created a thermionic cathode structure that consists of a thin tungsten ribbon; carbon nanotubes (CNTs) on the ribbon surface; and a thin layer of low work function barium strontium oxide coating on the CNTs. This oxide coated CNT cathode was designed to combine the benefits from the high field enhancement factor from CNTs and the low work function from the emissive oxide coating. The field emission and thermionic emission properties of the cathode have been characterized. A field enhancement factor of 266 and a work function of 1.9 eV were obtained. At 1221 K, a thermionic emission current density of 1.22A/cm2 in an electric field of 1.1 V/μm was obtained, which is four orders of magnitude greater than the emission current density from the uncoated CNT cathode at the same temperature. The high emission current density at such a modest temperature is among the best ever reported for an oxide cathode.


2005 ◽  
Vol 484 (1-2) ◽  
pp. 379-381 ◽  
Author(s):  
Guang Yuan ◽  
Hang Song ◽  
Yixin Jin ◽  
Hidenori Mimura ◽  
Kuniyoshi Yokoo

2010 ◽  
Vol 21 (35) ◽  
pp. 358001 ◽  
Author(s):  
A I Zhbanov ◽  
Yong-Gu Lee ◽  
E G Pogorelov ◽  
Yia-Chung Chang

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Bao-xin Yan ◽  
Yan-ying Zhu ◽  
Yong Wei ◽  
Huan Pei

AbstractIn this paper, the surface enhanced Raman scattering (SERS) characteristics of Au and Au@Al2O3 nanoparticle dimers were calculated and analyzed by using finite element method (3D-FEM). Firstly, the electric field enhancement factors of Au nanoparticles at the dimer gap were optimized from three aspects: the incident angle of the incident light, the radius of nanoparticle and the distance of the dimer. Then, aluminum oxide is wrapped on the Au dimer. What is different from the previous simulation is that Al2O3 shell and Au core are regarded as a whole and the total radius of Au@Al2O3 dimer is controlled to remain unchanged. By comparing the distance of Au nucleus between Au and Au@Al2O3 dimer, it is found that the electric field enhancement factor of Au@Al2O3 dimer is much greater than that of Au dimer with the increase of Al2O3 thickness. The peak of electric field of Au@Al2O3 dimer moves towards the middle of the resonance peak of the two materials, and it is more concentrated than that of the Au dimer. The maximum electric field enhancement factor 583 is reached at the shell thickness of 1 nm. Our results provide a theoretical reference for the design of SERS substrate and the extension of the research scope.


2017 ◽  
Vol 5 (4) ◽  
pp. 490-528 ◽  
Author(s):  
KAESER M. SABRIN ◽  
CONSTANTINE DOVROLIS

AbstractMany hierarchically modular systems are structured in a way that resembles an hourglass. This “hourglass effect” means that the system generates many outputs from many inputs through a relatively small number of intermediate modules that are critical for the operation of the entire system, referred to as the waist of the hourglass. We investigate the hourglass effect in general, not necessarily layered, hierarchical dependency networks. Our analysis focuses on the number of source-to-target dependency paths that traverse each vertex, and it identifies the core of a dependency network as the smallest set of vertices that collectively cover almost all dependency paths. We then examine if a given network exhibits the hourglass property or not, comparing its core size with a “flat” (i.e., non-hierarchical) network that preserves the source dependencies of each target in the original network. As a possible explanation for the hourglass effect, we propose the Reuse Preference model that captures the bias of new modules to reuse intermediate modules of similar complexity instead of connecting directly to sources or low complexity modules. We have applied the proposed framework in a diverse set of dependency networks from technological, natural, and information systems, showing that all these networks exhibit the general hourglass property but to a varying degree and with different waist characteristics.


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