Recent Progress in Improving the Performance of Infrared Photodetectors via Optical Field Manipulations

Benefiting from the inherent capacity for detecting longer wavelengths inaccessible to human eyes, infrared photodetectors have found numerous applications in both military and daily life, such as individual combat weapons, automatic driving sensors and night-vision devices. However, the imperfect material growth and incomplete device manufacturing impose an inevitable restriction on the further improvement of infrared photodetectors. The advent of artificial microstructures, especially metasurfaces, featuring with strong light field enhancement and multifunctional properties in manipulating the light–matter interactions on subwavelength scale, have promised great potential in overcoming the bottlenecks faced by conventional infrared detectors. Additionally, metasurfaces exhibit versatile and flexible integration with existing detection semiconductors. In this paper, we start with a review of conventionally bulky and recently emerging two-dimensional material-based infrared photodetectors, i.e., InGaAs, HgCdTe, graphene, transition metal dichalcogenides and black phosphorus devices. As to the challenges the detectors are facing, we further discuss the recent progress on the metasurfaces integrated on the photodetectors and demonstrate their role in improving device performance. All information provided in this paper aims to open a new way to boost high-performance infrared photodetectors.

Theoretical Comparison of Optothermal Absorption in Transmissive Metalenses Composed of Nanobricks and Nanoholes

Background: Optical components with high damage thresholds are very desirable in intense-light systems. Metalenses, being composed of phase-control nanostructures with peculiar properties, are one of the important component candidates in future optical systems. However, the optothermal mechanism in metalenses is still not investigated adequately. Methods: In this study, the optothermal absorption in transmissive metalenses made of silicon nanobricks and nanoholes is investigated comparatively to address this issue. Results: The geometrical dependencies of nanostructures’ transmittance, phase difference, and field distribution are calculated numerically via simulations. To demonstrate the optothermal mechanism in metalenses, the mean absorption efficiencies of the selected unit-cells, which would constitute metalenses, are analyzed. The results show that the electric field in the silicon zone would lead to an obvious thermal effect, and the enhancement of the localized electric field also results in the strong absorption of optical energy. Then, two typical metalenses are designed based on these nanobricks and nanoholes. The optothermal simulations show that the nanobrick-based metalens can handle a power density of 0.15 W/µm2, and the density of the nanohole-based design is 0.12 W/µm2. Conclusions: The study analyzes and compares the optothermal absorption in nanobricks and nanoholes, which shows that the electric-field distribution in absorbent materials and the localized-field enhancement are the two key effects that lead to optothermal absorption. This study provides an approach to improve the anti-damage potentials of transmissive metalenses for intense-light systems.

Optical Dielectrophoretic (DEP) Manipulation of Oil-Immersed Aqueous Droplets on a Plasmonic-Enhanced Photoconductive Surface

We present a plasmonic-enhanced dielectrophoretic (DEP) phenomenon to improve optical DEP performance of a floating electrode optoelectronic tweezers (FEOET) device, where aqueous droplets can be effectively manipulated on a light-patterned photoconductive surface immersed in an oil medium. To offer device simplicity and cost-effectiveness, recent studies have utilized a polymer-based photoconductive material such as titanium oxide phthalocyanine (TiOPc). However, the TiOPc has much poorer photoconductivity than that of semiconductors like amorphous silicon (a-Si), significantly limiting optical DEP applications. The study herein focuses on the FEOET device for which optical DEP performance can be greatly enhanced by utilizing plasmonic nanoparticles as light scattering elements to improve light absorption of the low-quality TiOPc. Numerical simulation studies of both plasmonic light scattering and electric field enhancement were conducted to verify wide-angle scattering light rays and an approximately twofold increase in electric field gradient with the presence of nanoparticles. Similarly, a spectrophotometric study conducted on the absorption spectrum of the TiOPc has shown light absorption improvement (nearly twofold) of the TiOPc layer. Additionally, droplet dynamics study experimentally demonstrated a light-actuated droplet speed of 1.90 mm/s, a more than 11-fold improvement due to plasmonic light scattering. This plasmonic-enhanced FEOET technology can considerably improve optical DEP capability even with poor-quality photoconductive materials, thus providing low-cost, easy-fabrication solutions for various droplet-based microfluidic applications.

Significant Near Field Enhancement Over Large Volumes Around Metal Nanorods via Strong Coupling of Surface Lattice Resonances and Fabry-Pérot Resonance

Metal nanoparticles supporting plasmons are widely used to enhance electromagnetic fields, resulting in strong light-matter interactions at the nanoscale in a diverse range of applications. Recently, it has been shown that when metal nanorods are periodically arranged with proper lattice periods, surface lattice resonances (SLRs) can be excited and near fields can be greatly enhanced over extended volumes. In this work, we report significant near field enhancement over even larger volumes by placing the metal nanorod array within a Fabry-Pérot (F-P) microcavity. Results show that taking advantage of strong coupling between the SLR and the photonic F-P resonances, the electric field intensity of the bonding split mode can be enhanced by up to 1935 times, which is about three times of the enhancement of the SLR, and the greatly enhanced field can extend over most of the F-P microcavity. We further show that the F-P resonances of both odd and even orders can strongly couple to the SLR by varying the nanorods position from the middle of the microcavity. We expect that the proposed plasmonic-photonic coupling system will find promising applications in nanolasers, nonlinear optics and sensing.

Electromagnetic Field Enhancement of Nanostructured TiN Electrodes Probed with Surface-Enhanced Raman Spectroscopy

We present a facile approach for the determination of the electromagnetic field enhancement of nanostructured TiN electrodes. As model system, TiN with partially collapsed nanotube structure obtained from nitridation of TiO2 nanotube arrays was used. Using surface-enhanced Raman scattering (SERS) spectroscopy, the electromagnetic field enhancement factors (EFs) of the substrate across the optical region were determined. The non-surface binding SERS reporter group azidobenzene was chosen, for which contributions from the chemical enhancement effect can be minimized. Derived EFs correlated with the electronic absorption profile and reached 3.9 at 786 nm excitation. Near-field enhancement and far-field absorption simulated with rigorous coupled wave analysis showed good agreement with the experimental observations. The major optical activity of TiN was concluded to originate from collective localized plasmonic modes at ca. 700 nm arising from the specific nanostructure.

Unveiling radial breathing mode in a particle-on-mirror plasmonic nanocavity

Plasmonic radial breathing mode (RBM), featured with radially oscillating charge density, arises from the surface plasmon waves confined in the flat nanoparticles. The zero net dipole moment endows the RBM with an extremely low radiation yet a remarkable intense local field. On the other hand, owing to the dark mode nature, the RBMs routinely escape from the optical measurements, severely preventing their applications in optoelectronics and nanophotonics. Here, we experimentally demonstrate the existence of RBM in a hexagonal Au nanoplate-on-mirror nanocavity using a far-field linear-polarized light source. The polarization-resolved scattering measurements cooperated with the full-wave simulations elucidate that the RBM originates from the standing plasmon waves residing in the Au nanoplate. Further numerical analysis shows the RBM possesses the remarkable capability of local field enhancement over the other dark modes in the same nanocavity. Moreover, the RBM is sensitive to the gap and nanoplate size of the nanocavity, providing a straightforward way to tailor the wavelength of RBM from the visible to near-infrared region. Our approach provides a facile optical path to access to the plasmonic RBMs and may open up a new route to explore the intriguing applications of RBM, including surface-enhanced Raman scattering, enhanced nonlinear effects, nanolasers, biological and chemical sensing.

Gold Coated VO2 Nanogratings Based Plasmonic Switches

This paper presents 2 dimensional (2D) and 1 dimensional (1D) gold (Au) coated VO2 (Vanadium Dioxide) nanogratings based tunable plasmonic switch. VO2 is a phase changing material and hence exhibits phase transition from semiconductor to metallic phase approximately at 67 ºC or 340 K (critical temperature) which can be achieved by exposure to IR radiation, application of voltage, heating, etc. and there is a huge contrast between optical properties of its metallic and insulating phases and hence that can be utilized to implement VO2 based optical switches. These VO2 based gratings couple the incident optical radiation to plasmonic waveguide modes which in turn leads to high electromagnetic field enhancement in the gaps between the nanogratings. The proposed Au coated VO2 nanogratings can be fabricated by using current state of art fabrication techniques and provides switchability of the order of femtoseconds. Hence the optical switching explained in our paper can be used fast switching applications. For an optimum switch our aim is to maximize its differential reflectance spectra between the 2 states of VO2, i.e., metallic and semiconductor phases. Rigorous Coupled Wave Analysis (RCWA) reveals that wavelengths for maximum differential reflectance can be optimized over a large spectral regime by varying various parameters of nanogratings for example groove height (h), width (w), gap (g) between the gratings, and thickness (t) of Au coating over VO2 by simulation using RCWA for maximum differential reflectance between VO2 metal and semiconductor phase, i.e., the switching wavelengths can be tuned by varying grating parameters and thus we can have optimum optical switch.

Gold Enhanced Graphene-Based Photodetector on Optical Fiber with Ultrasensitivity over Near-Infrared Bands

Graphene has been widely used in photodetectors; however its photoresponsivity is limited due to the intrinsic low absorption of graphene. To enhance the graphene absorption, a waveguide structure with an extended interaction length and plasmonic resonance with light field enhancement are often employed. However, the operation bandwidth is narrowed when this happens. Here, a novel graphene-based all-fiber photodetector (AFPD) was demonstrated with ultrahigh responsivity over a full near-infrared band. The AFPD benefits from the gold-enhanced absorption when an interdigitated Au electrode is fabricated onto a Graphene-PMMA film covered over a side-polished fiber (SFP). Interestingly, the AFPD shows a photoresponsivity of >1 × 104 A/W and an external quantum efficiency of >4.6 × 106% over a broadband region of 980–1620 nm. The proposed device provides a simple, low-cost, efficient, and robust way to detect optical fiber signals with intriguing capabilities in terms of distributed photodetection and on-line power monitoring, which is highly desirable for a fiber-optic communication system.