scholarly journals Однородные и неоднородные ширины линий в оптических спектрах кристалла Y-=SUB=-2-=/SUB=-SiO-=SUB=-5-=/SUB=- : -=SUP=-171-=/SUP=-Yb-=SUP=-3+-=/SUP=-

2022 ◽  
Vol 130 (1) ◽  
pp. 23
Author(s):  
Eloise Lafitte-Houssat ◽  
Alban Ferrier ◽  
Mikael Afzelius ◽  
Perrine Berger ◽  
Loic Morvan ◽  
...  
Keyword(s):  
Rare Earth ◽  
Ground State ◽  
Spin Systems ◽  
Rare Earth Ions ◽  
Zero Magnetic Field ◽  
Unusual Property ◽  
Nuclear Spins ◽  
Spin Coherence ◽  
Slowing Down ◽  
State Spin

Rare earth ions are actively investigated as optically addressable spin systems for quantum technologies thanks to their long optical and spin coherence lifetimes. 171Yb3+, which has 1/2 electron and nuclear spins, recently raised interest for its simple hyperfine structure that moreover can result in long coherence lifetimes at zero magnetic field, an unusual property for paramagnetic rare earth ions. Here, we report on the optical inhomogeneous and homogeneous linewidths in 171Yb3+:Y2SiO5 (site 2) for different doping concentrations. While inhomogeneous linewidth is not correlated to 171Yb3+ concentration, the homogeneous one strongly decreases between 10 and 2 ppm doping level, reaching 255 Hz at 3 K. This is attributed to a slowing down of 171Yb3+ ground state spin flip-flops.

scholarly journals Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Kuppusamy Senthil Kumar ◽  
Diana Serrano ◽  
Aline M. Nonat ◽  
Benoît Heinrich ◽  
Lydia Karmazin ◽  
...  
Keyword(s):  
Ground State ◽  
Quantum Information Processing ◽  
Optical Transition ◽  
Molecular Engineering ◽  
Coherent Light ◽  
Nuclear Spins ◽  
Rare Earth Ion ◽  
Molecular Systems ◽  
Homogeneous Linewidth ◽  
State Spin

AbstractThe success of the emerging field of solid-state optical quantum information processing (QIP) critically depends on the access to resonant optical materials. Rare-earth ion (REI)-based molecular systems, whose quantum properties could be tuned taking advantage of molecular engineering strategies, are one of the systems actively pursued for the implementation of QIP schemes. Herein, we demonstrate the efficient polarization of ground-state nuclear spins—a fundamental requirement for all-optical spin initialization and addressing—in a binuclear Eu(III) complex, featuring inhomogeneously broadened 5D0 → 7F0 optical transition. At 1.4 K, long-lived spectral holes have been burnt in the transition: homogeneous linewidth (Γh) = 22 ± 1 MHz, which translates as optical coherence lifetime (T2opt) = 14.5 ± 0.7 ns, and ground-state spin population lifetime (T1spin) = 1.6 ± 0.4 s have been obtained. The results presented in this study could be a progressive step towards the realization of molecule-based coherent light-spin QIP interfaces.

scholarly journals Electron Spin Coherence in Optically Excited States of Rare-Earth Ions for Microwave to Optical Quantum Transducers

2019 ◽  
Vol 122 (24) ◽  
Author(s):  
Sacha Welinski ◽  
Philip J. T. Woodburn ◽  
Nikolai Lauk ◽  
Rufus L. Cone ◽  
Christoph Simon ◽  
...  
Keyword(s):  
Rare Earth ◽  
Excited States ◽  
Electron Spin ◽  
Rare Earth Ions ◽  
Spin Coherence

Cross-Relaxation Depletion of the Ground State of Rare-Earth Ions in Crystals

1991 ◽  
Author(s):  
M. A. Noginov ◽  
G. K. Sarkissian ◽  
V. A. Smirnov ◽  
I. A. Shcherbakov
Keyword(s):  
Rare Earth ◽  
Ground State ◽  
Cross Relaxation ◽  
Rare Earth Ions

scholarly journals Long spin coherence times in the ground state and in an optically excited state of Er3+167:Y2SiO5 at zero magnetic field

2020 ◽  
Vol 101 (18) ◽  
Author(s):  
Jelena V. Rakonjac ◽  
Yu-Hui Chen ◽  
Sebastian P. Horvath ◽  
Jevon J. Longdell
Keyword(s):  
Magnetic Field ◽  
Excited State ◽  
Ground State ◽  
Zero Magnetic Field ◽  
Spin Coherence

NMR studies of singlet-ground-state rare-earth ions in high-T c superconductors

1992 ◽  
Vol 3 (3-4) ◽  
pp. 613-640 ◽  
Author(s):  
O. N. Bakharev ◽  
A. V. Dooglav ◽  
A. V. Egorov ◽  
H. Lütgemeier ◽  
M. P. Rodionova ◽  
...  
Keyword(s):  
Rare Earth ◽  
Ground State ◽  
Rare Earth Ions ◽  
Singlet Ground State ◽  
Nmr Studies

A Bernasconi model for constructing ground-state spin systems

2014 ◽  
Vol 78 (3) ◽  
pp. 207-209 ◽  
Author(s):  
A. N. Leukhin ◽  
A. S. Shuvalov ◽  
E. N. Potekhin
Keyword(s):  
Ground State ◽  
Spin Systems ◽  
Ground State Spin ◽  
State Spin

Magnetic anisotropy and ground state of the rare-earth ions in PrMnO3 and NdMnO3

2001 ◽  
Vol 226-230 ◽  
pp. 1139-1141 ◽  
Author(s):  
A.A Mukhin ◽  
V.Yu Ivanov ◽  
V.D Travkin ◽  
A.M Balbashov
Keyword(s):  
Rare Earth ◽  
Magnetic Anisotropy ◽  
Ground State ◽  
Rare Earth Ions ◽  
The Rare Earth

ChemInform Abstract: NMR Studies of Singlet-Ground-State Rare-Earth Ions in High-Tc Superconductors

ChemInform ◽  
2010 ◽  
Vol 24 (14) ◽  
pp. no-no
Author(s):  
O. N. BAKHAREV ◽  
A. V. DOOGLAV ◽  
A. V. EGOROV ◽  
H. LUETGEMEIER ◽  
M. P. RODIONOVA ◽  
...  
Keyword(s):  
Rare Earth ◽  
Ground State ◽  
Rare Earth Ions ◽  
Singlet Ground State ◽  
High Tc Superconductors ◽  
Nmr Studies ◽  
High Tc

Luminescence of Er3+/Nd3+ Co-Doped Lithium Niobate Tellurite Glass

2016 ◽  
Vol 846 ◽  
pp. 131-136
Author(s):  
Nurhafizah Hasim ◽  
Md Supar Rohani ◽  
Md Rahim Sahar ◽  
Sib Krishna Ghoshal
Keyword(s):  
Rare Earth ◽  
Lithium Niobate ◽  
Excited States ◽  
Ground State ◽  
Emission Spectra ◽  
Green Emission ◽  
Volume Density ◽  
Rare Earth Ions ◽  
Luminescence Spectra ◽  
Co Doped

Achieving tuneable photoluminescence via controlled co-doping of rare earth ions in lithium niobate based glasses are challenging. A series of Er3+/ Nd3+ co-doped tellurite glasses of composition (70-x-y) TeO2 – 15 Li2CO3 – 15 Nb2O5 – (x) Er2O3 – (y) Nd2O3 with x = 0; 1.0 mol % and 0 ≤ y ≤ 1.0 mol % are prepared using melt quenching technique. The influence of co-dopants on the emission properties is analyzed and discussed using partial energy level diagram of rare earth ions. The dopants concentration dependent physical properties such as refractive index, molar volume, density, polarizability and molar refractions are determined. The down-converted luminescence spectra for 2G9/2 à4I9/2 transition reveal a strong green emission band centred at 497 nm is attributed to the energy transfer from erbium to neodymium ion. The emission spectra exhibit five prominent peaks centred at 497, 539, 553, 616 and 634 nm corresponding to the transitions from 2H11/2, 4S3/2 and 4F9/2 excited states to the ground state of Er3+ ion and the transitions from 2G9/2, 2G7/2, 2H11/2 and 4F9/2 excited states to ground state of Nd3+ ion. The highest intensity is achieved for x = y = 1.0 mol%. The excellent luminescence response suggests that our glasses may be nominated for solid state lasers and other photonic applications.

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