scholarly journals Production Cross-Section Measurements for Terbium Radionuclides of Medical Interest Produced in Tantalum Targets Irradiated by 0.3 to 1.7 GeV Protons and Corresponding Thick Target Yield Calculations

2021 ◽  
Vol 8 ◽  
Author(s):  
Charlotte Duchemin ◽  
Thomas E. Cocolios ◽  
Kristof Dockx ◽  
Gregory J. Farooq-Smith ◽  
Olaf Felden ◽  
...  

This work presents the production cross-sections of Ce, Tb and Dy radionuclides produced by 300 MeV to 1.7 GeV proton-induced spallation reactions in thin tantalum targets as well as the related Thick Target production Yield (TTY) values and ratios. The motivation is to optimise the production of terbium radionuclides for medical applications and to find out at which energy the purity of the collection by mass separation would be highest. For that purpose, activation experiments were performed using the COSY synchrotron at FZ Jülich utilising the stacked-foils technique and γ spectrometry with high-purity germanium detectors. The Al-27(p,x)Na-24 reaction has been used as monitor reaction. All experimental data have been systematically compared with the existing literature.

Instruments ◽  
2019 ◽  
Vol 3 (2) ◽  
pp. 29 ◽  
Author(s):  
Mateusz Sitarz ◽  
Jerzy Jastrzębski ◽  
Férid Haddad ◽  
Tomasz Matulewicz ◽  
Katarzyna Szkliniarz ◽  
...  

In this work, we present an attempt to estimate the reaction excitation function based on the measurements of thick target yield. We fit a function to experimental data points and then use three fitting parameters to calculate the cross-section. We applied our approach to 43Ca(p,n)43Sc, 44Ca(p,n)44gSc, 44Ca(p,n)44mSc, 48Ca(p,2n)47Sc and 48Ca(p,n)48Sc reactions. A general agreement was observed between the reconstructions and the available cross-section data. The algorithm described here can be used to roughly estimate cross-section values, but it requires improvements.


2004 ◽  
Vol 734 ◽  
pp. 221-224 ◽  
Author(s):  
J. Pereira ◽  
P. Armbruster ◽  
J. Benlliure ◽  
M. Bernas ◽  
A. Boudard ◽  
...  

1983 ◽  
Vol 61 (4) ◽  
pp. 754-756 ◽  
Author(s):  
Seiichi Shibata ◽  
Paul J. Karol

An unknown γ-ray of energy 112.5 keV was found in zirconium fractions chemically extracted from isotopically enriched molybdenum targets bombarded with 500 and 800 MeV protons. All evidence suggests that the γ-ray is identifiable with the decay of 84Zr to 84Y. A half-life of 25.7 ± 0.5 min was obtained for 84Zr, which is considerably longer than previously reported half-lives. The absolute abundance of the 112.5 keV γ-ray was also determined. Relative production cross sections for 84Zr were calculated using these results and were consistent with the values interpolated from isotopic distribution curves for spallation reactions.


1972 ◽  
Vol 6 (3) ◽  
pp. 1257-1257 ◽  
Author(s):  
Knud Taulbjerg ◽  
Peter Sigmund

2019 ◽  
Vol 127 (5) ◽  
pp. 53001
Author(s):  
Y. Wu ◽  
Z. Y. Zhang ◽  
X. G. Xia ◽  
M. X. Xu ◽  
C. H. Chang ◽  
...  

2013 ◽  
Vol 899 ◽  
pp. 116-132 ◽  
Author(s):  
L. Giot ◽  
J.A. Alcántara-Núñez ◽  
J. Benlliure ◽  
D. Pérez-Loureiro ◽  
L. Audouin ◽  
...  

Instruments ◽  
2022 ◽  
Vol 6 (1) ◽  
pp. 3
Author(s):  
Sergio J. C. do Carmo ◽  
Francisco Alves

The present work describes a method to determine excitation function curves and, therefore, cross-sections, making use of the irradiation of liquid targets at distinct energies in a biomedical cyclotron. The method relies on the derivative of experimentally measured thick target yield curves to determine the corresponding excitation function curves. The technique is presented as a valid and practical alternative to the commonly used activation method combined with the stack monitor technique, whose implementation in liquid targets offers practical difficulties. The working principle is exemplified by presenting the results obtained for the clinically relevant 68Zn(p,n)68Ga and the 64Zn(p,α)61Cu nuclear reactions, obtained though the irradiation of liquid targets containing dissolved natural zinc.


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