scholarly journals Room-temperature single-photon emitters in titanium dioxide optical defects

2018 ◽  
Vol 9 ◽  
pp. 1085-1094 ◽  
Author(s):  
Kelvin Chung ◽  
Yu H Leung ◽  
Chap H To ◽  
Aleksandra B Djurišić ◽  
Snjezana Tomljenovic-Hanic

Fluorescence properties of crystallographic point defects within different morphologies of titanium dioxide were investigated. For the first time, room-temperature single-photon emission in titanium dioxide optical defects was discovered in thin films and commercial nanoparticles. Three-level defects were identified because the g (2) correlation data featured prominent shoulders around the antibunching dip. Stable and blinking photodynamics were observed for the single-photon emitters. These results reveal a new room-temperature single-photon source within a wide bandgap semiconductor.

Nanophotonics ◽  
2020 ◽  
Vol 9 (11) ◽  
pp. 3557-3565
Author(s):  
Guorui Zhang ◽  
Ying Gu ◽  
Qihuang Gong ◽  
Jianjun Chen

AbstractDue to small optical mode volumes and linear polarizations of surface-plasmon-polariton (SPP) resonant modes in metallic antennas, it is very difficult to obtain complex emission patterns and polarizations for single-photon emitters. Herein, nonresonant enhancement in a silver nanowire is used to both enhance emission rates and extract a z-oriented dipole, and then the symmetry of metallic nanostructures is proposed to tailor the patterns and polarizations of single-photon emission. The emission pattern of a quantum dot located close to a metallic nanostructure with a symmetric axis is split into multiple flaps. The number of splitting flaps is equal to the order of the symmetric axis. Moreover, the electric vectors of the emitted photons become centrally symmetric about the symmetric axis. The above phenomena are well explained by both a simulation and an image dipole model. The structural-symmetry-tailoring mechanism may open up a new avenue in the design of multifunctional and novel quantum-plasmonic devices.


2017 ◽  
Vol 29 (12) ◽  
pp. 1605092 ◽  
Author(s):  
Amanuel M. Berhane ◽  
Kwang-Yong Jeong ◽  
Zoltán Bodrog ◽  
Saskia Fiedler ◽  
Tim Schröder ◽  
...  

2011 ◽  
Vol 99 (25) ◽  
pp. 251106 ◽  
Author(s):  
A. Lohrmann ◽  
S. Pezzagna ◽  
I. Dobrinets ◽  
P. Spinicelli ◽  
V. Jacques ◽  
...  

Nanophotonics ◽  
2017 ◽  
Vol 6 (1) ◽  
pp. 269-278 ◽  
Author(s):  
Kelvin Chung ◽  
Timothy J. Karle ◽  
Asma Khalid ◽  
Amanda N. Abraham ◽  
Ravi Shukla ◽  
...  

AbstractZinc oxide (ZnO) is a promising semiconductor that is suitable for bioimaging applications due to its intrinsic defect fluorescence. However, ZnO generally suffers from poor photostability. We report room-temperature single-photon emission from optical defects found in ZnO nanoparticles (NPs) formed by ion implantation followed by thermal oxidation in a silica substrate. We conduct a thorough investigation into the photophysics of a particularly bright defect and identify other single emitters within the NPs. Photostability was observed when the NPs were removed from the growth substrate and taken up by skin cells for in vitro imaging.


2014 ◽  
Vol 105 (14) ◽  
pp. 141109 ◽  
Author(s):  
Saniya Deshpande ◽  
Thomas Frost ◽  
Arnab Hazari ◽  
Pallab Bhattacharya

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