scholarly journals Bacteria in the ECHAM5-HAM global climate model

2012 ◽  
Vol 12 (18) ◽  
pp. 8645-8661 ◽  
Author(s):  
A. Sesartic ◽  
U. Lohmann ◽  
T. Storelvmo
Keyword(s):  
Active Sites ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Ice Nucleation ◽  
Cloud Formation ◽  
Liquid Water Path ◽  
Water Path ◽  
Ice Nuclei ◽  
Ice Water

Abstract. Some bacteria are among the most active ice nuclei found in nature due to the ice nucleation active proteins on their surface, which serve as active sites for ice nucleation. Their potential impact on clouds and precipitation is not well known and needs to be investigated. Bacteria as a new aerosol species were introduced into the global climate model (GCM) ECHAM5-HAM. The inclusion of bacteria acting as ice nuclei in a GCM leads to only minor changes in cloud formation and precipitation on a global level, however, changes in the liquid water path and ice water path are simulated, specifically in the boreal regions where tundra and forests act as sources of bacteria. Although bacteria contribute to heterogeneous freezing, their impact is reduced by their low numbers compared to other heterogeneous IN. This result confirms the outcome of several previous studies.

scholarly journals Bacteria in the ECHAM5-HAM global climate model

2011 ◽  
Vol 11 (1) ◽  
pp. 1457-1488 ◽  
Author(s):  
A. Sesartic ◽  
U. Lohmann ◽  
T. Storelvmo
Keyword(s):  
Active Sites ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Ice Nucleation ◽  
Cloud Formation ◽  
Liquid Water Path ◽  
Water Path ◽  
Ice Nuclei ◽  
Ice Water

Abstract. Bacteria are the most active naturally occuring ice nuclei (IN) due to the ice nucleation active proteins on their surface, which serve as active sites for ice nucleation. Their potential impact on clouds and precipitation is not well known and needs to be investigated. Bacteria as a new aerosol species were introduced into the global climate model (GCM) ECHAM5-HAM. The inclusion of bacteria acting as IN in a GCM leads to only minor changes in cloud formation and precipitation on a global level, however, changes in the liquid water path and ice water path can be observed, specifically in the boreal regions where tundra and forests act as sources of bacteria.

scholarly journals A Classical-Theory-Based Parameterization of Heterogeneous Ice Nucleation by Mineral Dust, Soot, and Biological Particles in a Global Climate Model

2010 ◽  
Vol 67 (8) ◽  
pp. 2483-2503 ◽  
Author(s):  
Corinna Hoose ◽  
Jón Egill Kristjánsson ◽  
Jen-Ping Chen ◽  
Anupam Hazra
Keyword(s):  
Climate Model ◽  
Mineral Dust ◽  
Global Climate ◽  
Global Climate Model ◽  
Ice Nucleation ◽  
Nucleation Theory ◽  
Ice Formation ◽  
Biological Particles ◽  
Ice Nuclei ◽  
Immersion Freezing

Abstract An ice nucleation parameterization based on classical nucleation theory, with aerosol-specific parameters derived from experiments, has been implemented into a global climate model—the Community Atmosphere Model (CAM)-Oslo. The parameterization treats immersion, contact, and deposition nucleation by mineral dust, soot, bacteria, fungal spores, and pollen in mixed-phase clouds at temperatures between 0° and −38°C. Immersion freezing is considered for insoluble particles that are activated to cloud droplets, and deposition and contact nucleation are only allowed for uncoated, unactivated aerosols. Immersion freezing by mineral dust is found to be the dominant ice formation process, followed by immersion and contact freezing by soot. The simulated biological aerosol contribution to global atmospheric ice formation is marginal, even with high estimates of their ice nucleation activity, because the number concentration of ice nucleation active biological particles in the atmosphere is low compared to other ice nucleating aerosols. Because of the dominance of mineral dust, the simulated ice nuclei concentrations at temperatures below −20°C are found to correlate with coarse-mode aerosol particle concentrations. The ice nuclei (IN) concentrations in the model agree well overall with in situ continuous flow diffusion chamber measurements. At individual locations, the model exhibits a stronger temperature dependence on IN concentrations than what is observed. The simulated IN composition (77% mineral dust, 23% soot, and 10−5% biological particles) lies in the range of observed ice nuclei and ice crystal residue compositions.

scholarly journals A comparison of ship and satellite measurements of cloud properties with global climate model simulations in the southeast Pacific stratus deck

2010 ◽  
Vol 10 (14) ◽  
pp. 6527-6536 ◽  
Author(s):  
M. A. Brunke ◽  
S. P. de Szoeke ◽  
P. Zuidema ◽  
X. Zeng
Keyword(s):  
Diurnal Cycle ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Cloud Fraction ◽  
Cloud Base ◽  
Liquid Water Path ◽  
Cloud Properties ◽  
Southeast Pacific ◽  
Cloud Thickness

Abstract. Here, liquid water path (LWP), cloud fraction, cloud top height, and cloud base height retrieved by a suite of A-train satellite instruments (the CPR aboard CloudSat, CALIOP aboard CALIPSO, and MODIS aboard Aqua) are compared to ship observations from research cruises made in 2001 and 2003–2007 into the stratus/stratocumulus deck over the southeast Pacific Ocean. It is found that CloudSat radar-only LWP is generally too high over this region and the CloudSat/CALIPSO cloud bases are too low. This results in a relationship (LWP~h9) between CloudSat LWP and CALIPSO cloud thickness (h) that is very different from the adiabatic relationship (LWP~h2) from in situ observations. Such biases can be reduced if LWPs suspected to be contaminated by precipitation are eliminated, as determined by the maximum radar reflectivity Zmax>−15 dBZ in the apparent lower half of the cloud, and if cloud bases are determined based upon the adiabatically-determined cloud thickness (h~LWP1/2). Furthermore, comparing results from a global model (CAM3.1) to ship observations reveals that, while the simulated LWP is quite reasonable, the model cloud is too thick and too low, allowing the model to have LWPs that are almost independent of h. This model can also obtain a reasonable diurnal cycle in LWP and cloud fraction at a location roughly in the centre of this region (20° S, 85° W) but has an opposite diurnal cycle to those observed aboard ship at a location closer to the coast (20° S, 75° W). The diurnal cycle at the latter location is slightly improved in the newest version of the model (CAM4). However, the simulated clouds remain too thick and too low, as cloud bases are usually at or near the surface.

scholarly journals Cirrus clouds in a global climate model with a statistical cirrus cloud scheme

2010 ◽  
Vol 10 (12) ◽  
pp. 5449-5474 ◽  
Author(s):  
M. Wang ◽  
J. E. Penner
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Lower Troposphere ◽  
Circulation Model ◽  
Cirrus Clouds ◽  
Cloud Formation ◽  
Cirrus Cloud ◽  
Ice Crystal ◽  
Homogeneous Freezing

Abstract. A statistical cirrus cloud scheme that accounts for mesoscale temperature perturbations is implemented in a coupled aerosol and atmospheric circulation model to better represent both subgrid-scale supersaturation and cloud formation. This new scheme treats the effects of aerosol on cloud formation and ice freezing in an improved manner, and both homogeneous freezing and heterogeneous freezing are included. The scheme is able to better simulate the observed probability distribution of relative humidity compared to the scheme that was implemented in an older version of the model. Heterogeneous ice nuclei (IN) are shown to decrease the frequency of occurrence of supersaturation, and improve the comparison with observations at 192 hPa. Homogeneous freezing alone can not reproduce observed ice crystal number concentrations at low temperatures (<205 K), but the addition of heterogeneous IN improves the comparison somewhat. Increases in heterogeneous IN affect both high level cirrus clouds and low level liquid clouds. Increases in cirrus clouds lead to a more cloudy and moist lower troposphere with less precipitation, effects which we associate with the decreased convective activity. The change in the net cloud forcing is not very sensitive to the change in ice crystal concentrations, but the change in the net radiative flux at the top of the atmosphere is still large because of changes in water vapor. Changes in the magnitude of the assumed mesoscale temperature perturbations by 25% alter the ice crystal number concentrations and the net radiative fluxes by an amount that is comparable to that from a factor of 10 change in the heterogeneous IN number concentrations. Further improvements on the representation of mesoscale temperature perturbations, heterogeneous IN and the competition between homogeneous freezing and heterogeneous freezing are needed.

Understanding the Extratropical Liquid Water Path Feedback in Mixed-Phase Clouds with an Idealized Global Climate Model

2022 ◽  
pp. 1-48
Author(s):  
Yi Ming
Keyword(s):  
Water Content ◽  
Liquid Water ◽  
Climate Model ◽  
Global Climate Model ◽  
Cloud Water ◽  
Mixed Phase ◽  
Liquid Water Path ◽  
Water Path ◽  
Cloud Water Content ◽  
Mixed Phase Clouds

Abstract A negative shortwave cloud feedback associated with higher extratropical liquid water content in mixed-phase clouds is a common feature of global warming simulations, and multiple mechanisms have been hypothesized. A set of process-level experiments performed with an idealized global climate model (a dynamical core with passive water and cloud tracers and full Rotstayn-Klein single-moment microphysics) show that the common picture of the liquid water path (LWP) feedback in mixed-phase clouds being controlled by the amount of ice susceptible to phase change is not robust. Dynamic condensate processes—rather than static phase partitioning—directly change with warming, with varied impacts on liquid and ice amounts. Here, three principal mechanisms are responsible for the LWP response, namely higher adiabatic cloud water content, weaker liquid-to-ice conversion through the Bergeron-Findeisen process, and faster melting of ice and snow to rain. Only melting is accompanied by a substantial loss of ice, while the adiabatic cloud water content increase gives rise to a net increase in ice water path (IWP) such that total cloud water also increases without an accompanying decrease in precipitation efficiency. Perturbed parameter experiments with a wide range of climatological LWP and IWP demonstrate a strong dependence of the LWP feedback on the climatological LWP and independence from the climatological IWP and supercooled liquid fraction. This idealized setup allows for a clean isolation of mechanisms and paints a more nuanced picture of the extratropical mixed-phase cloud water feedback than simple phase change.

scholarly journals Global 3D modelling of Martian CO2 clouds

2021 ◽  
Author(s):  
Christophe Mathé ◽  
Anni Määttänen ◽  
Joachim Audouard ◽  
Constantino Listowski ◽  
Ehouarn Millour ◽  
...  
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Martian Atmosphere ◽  
Cloud Formation ◽  
Polar Regions ◽  
Northern Latitudes ◽  
1D Model ◽  
Mesospheric Clouds ◽  
Microphysical Processes

&lt;p&gt;In the Martian atmosphere, carbon dioxide (CO&lt;sub&gt;2&lt;/sub&gt;) clouds have been revealed by numerous instruments around Mars from the beginning of the XXI century. These observed clouds can be distinguished by two kinds involving different formation processes: those formed during the winter in polar regions located in the troposphere, and those formed during the Martian year at low- and mid-northern latitudes located in the mesosphere (M&amp;#228;&amp;#228;att&amp;#228;nen et al, 2013). Microphysical processes of the formation of these clouds are still not fully understood. However, modeling studies revealed processes necessary for their formation: the requirement of waves that perturb the atmosphere leading to a temperature below the condensation of CO&lt;sub&gt;2&lt;/sub&gt; (transient planetary waves for tropospheric clouds (Kuroda et al., 20123), thermal tides (Gonzalez-Galindo et al., 2011) and gravity waves for mesospheric clouds (Spiga et al., 2012)). In the last decade, a state-of-the-art microphysical column (1D) model for CO&lt;sub&gt;2&lt;/sub&gt; clouds in a Martian atmosphere was developed at Laboratoire Atmosph&amp;#232;res, Observations Spatiales (LATMOS) (Listowski et al., 2013, 2014). We use our full microphysical model of CO&lt;sub&gt;2&lt;/sub&gt; cloud formation to investigate the occurrence of these CO&lt;sub&gt;2&lt;/sub&gt; clouds by coupling it with the Global Climate Model (GCM) of the Laboratoire de M&amp;#233;t&amp;#233;orologie Dynamique (LMD) (Forget et al., 1999). We recently activated the radiative impact of CO&lt;sub&gt;2&lt;/sub&gt; clouds in the atmosphere. Last modeling results on Martian CO&lt;sub&gt;2&lt;/sub&gt; clouds properties and their impacts on the atmosphere will be presented and be compared to observational data.&lt;/p&gt;

The effect of the photomineralization mechanism on ambient organic aerosols' cloud condensation nuclei and ice nucleation abilities

2020 ◽  
Author(s):  
Silvan Müller ◽  
Nadine Borduas-Dedekind
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Cloud Condensation Nuclei ◽  
Global Climate Model ◽  
Complex Mixture ◽  
Substantial Effect ◽  
Ice Nucleation ◽  
Anthropogenic Sources ◽  
Wood Smoke ◽  
Condensation Nuclei

&lt;p&gt;Organic aerosol (OA) is an important component of the atmospheric submicron particulate mass, consisting of a complex mixture of organic compounds from natural and anthropogenic sources. During its lifetime of approximately one week in the atmosphere, OA is exposed to sunlight and thus undergoes atmospheric processing through photochemistry. This photochemical aging mechanism is thought to have a substantial effect on the propensity of OA to participate in cloud-forming processes by increasing its cloud condensation nuclei (CCN) activity. However, this effect is not well-constrained, and the influence of photochemistry on the ice nucleation (IN) activity of OA is uncertain. In this study, we aim to better understand how the photomineralization mechanism changes the cloud-forming properties of OA by measuring the CCN and IN abilities of photochemically aged OA of different sources: (1) Laboratory-generated ammonium sulfate-methylglyoxal (a proxy for secondary OA), and ambient OA bulk solutions collected from (2) wood smoke and (3) urban particulate matter in Padua (Italy). The solutions are exposed to UV-B radiation in a photoreactor for up to 25 hour and subsequently analyzed for their IN ability and, following aerosolization, for their CCN ability. To correlate changes in cloud-forming properties with changes in chemical composition due to photomineralization, we measure total organic carbon, UV-Vis absorbance, and CO, CO&lt;sub&gt;2&lt;/sub&gt;, acetic acid, formic acid, pyruvic acid and oxalic acid production. Indeed, preliminary data of wood smoke OA highlights photomineralization as an important atmospheric aging process that modifies the CCN ability of OA. By characterizing both the CCN and IN abilities of photochemically aged OA, our study may thus provide important insights into the atmospheric evolution and cloud-forming properties of OA, potentially establishing photomineralization of OA as an important mechanism to consider in regional and global climate model predictions.&lt;/p&gt;

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