scholarly journals Spatio-temporal variations of nitric acid total columns from 9 years of IASI measurements – a driver study

2018 ◽  
Vol 18 (7) ◽  
pp. 4403-4423 ◽  
Author(s):  
Gaétane Ronsmans ◽  
Catherine Wespes ◽  
Daniel Hurtmans ◽  
Cathy Clerbaux ◽  
Pierre-François Coheur

Abstract. This study aims to understand the spatial and temporal variability of HNO3 total columns in terms of explanatory variables. To achieve this, multiple linear regressions are used to fit satellite-derived time series of HNO3 daily averaged total columns. First, an analysis of the IASI 9-year time series (2008–2016) is conducted based on various equivalent latitude bands. The strong and systematic denitrification of the southern polar stratosphere is observed very clearly. It is also possible to distinguish, within the polar vortex, three regions which are differently affected by the denitrification. Three exceptional denitrification episodes in 2011, 2014 and 2016 are also observed in the Northern Hemisphere, due to unusually low arctic temperatures. The time series are then fitted by multivariate regressions to identify what variables are responsible for HNO3 variability in global distributions and time series, and to quantify their respective influence. Out of an ensemble of proxies (annual cycle, solar flux, quasi-biennial oscillation, multivariate ENSO index, Arctic and Antarctic oscillations and volume of polar stratospheric clouds), only the those defined as significant (p value < 0.05) by a selection algorithm are retained for each equivalent latitude band. Overall, the regression gives a good representation of HNO3 variability, with especially good results at high latitudes (60–80 % of the observed variability explained by the model). The regressions show the dominance of annual variability in all latitudinal bands, which is related to specific chemistry and dynamics depending on the latitudes. We find that the polar stratospheric clouds (PSCs) also have a major influence in the polar regions, and that their inclusion in the model improves the correlation coefficients and the residuals. However, there is still a relatively large portion of HNO3 variability that remains unexplained by the model, especially in the intertropical regions, where factors not included in the regression model (such as vegetation fires or lightning) may be at play.

2017 ◽  
Author(s):  
Gaétane Ronsmans ◽  
Catherine Wespes ◽  
Daniel Hurtmans ◽  
Cathy Clerbaux ◽  
Pierre-François Coheur

Abstract. This study aims at understanding the spatial and temporal variability of HNO3 total columns in terms of explanatory variables. To achieve this, multiple linear regressions are used to fit satellite-derived time series of HNO3 daily averaged total columns. First, an analysis of the IASI 9-year time series (2008–2016) is conducted based on various equivalent latitude bands. The strong and systematic denitrification of the southern polar stratosphere is observed very clearly. It is also possible to distinguish, within the polar vortex, three regions wich are differently affected by the denitrification. Three exceptional denitrification episodes in 2011, 2014 and 2016 are also observed in the northern hemisphere, due to unusually low arctic temperatures. The time series are then fitted by multivariate regressions to identify what variables are responsible for HNO3 variability in global distributions and time series, and to quantify their respective influence. Out of an ensemble of proxies (annual cycle, solar flux, quasi-biennial oscillation, multivariate ENSO index, Arctic and Antarctic oscillations and volume of polar stratospheric clouds), only the ones defined as significant (p-value 


2020 ◽  
Vol 12 (18) ◽  
pp. 2898
Author(s):  
Filipe Lisboa ◽  
Vanda Brotas ◽  
Filipe Duarte Santos ◽  
Sakari Kuikka ◽  
Laura Kaikkonen ◽  
...  

Monitoring lakes in high-latitude areas can provide a better understanding of freshwater systems sensitivity and accrete knowledge on climate change impacts. Phytoplankton are sensitive to various conditions: warmer temperatures, earlier ice-melt and changing nutrient sources. While satellite imagery can monitor phytoplankton biomass using chlorophyll a (Chl) as a proxy over large areas, detection of Chl in small lakes is hindered by the low spatial resolution of conventional ocean color satellites. The short time-series of the newest generation of space-borne sensors (e.g., Sentinel-2) is a bottleneck for assessing long-term trends. Although previous studies have evaluated the use of high-resolution sensors for assessing lakes’ Chl, it is still unclear how the spatial and temporal variability of Chl concentration affect the performance of satellite estimates. We discuss the suitability of Landsat (LT) 30 m resolution imagery to assess lakes’ Chl concentrations under varying trophic conditions, across extensive high-latitude areas in Finland. We use in situ data obtained from field campaigns in 19 lakes and generate remote sensing estimates of Chl, taking advantage of the long-time span of the LT-5 and LT-7 archives, from 1984 to 2017. Our results show that linear models based on LT data can explain approximately 50% of the Chl interannual variability. However, we demonstrate that the accuracy of the estimates is dependent on the lake’s trophic state, with models performing in average twice as better in lakes with higher Chl concentration (>20 µg/L) in comparison with less eutrophic lakes. Finally, we demonstrate that linear models based on LT data can achieve high accuracy (R2 = 0.9; p-value < 0.05) in determining lakes’ mean Chl concentration, allowing the mapping of the trophic state of lakes across large regions. Given the long time-series and high spatial resolution, LT-based estimates of Chl provide a tool for assessing the impacts of environmental change.


2004 ◽  
Vol 219 ◽  
pp. 552-556 ◽  
Author(s):  
R. Knaack ◽  
J. O. Stenflo

We have investigated the temporal evolution of the solar magnetic field during solar cycles 20, 21 and 22 by means of spherical harmonic decomposition and subsequent time series analysis. A 33 yr and a 25 yr time series of daily magnetic maps of the solar photosphere, recorded at the Mt. Wilson and NSO/Kitt Peak observatories respectively, were used to calculate the spherical coefficients of the radial magnetic field. Fourier and wavelet analysis were then applied to deduce the temporal variations. We compare the results of the two datasets and present examples of zonal modes which show significant variations, e. g. with a period of approx. 2.0—2.5 years. We provide evidence that this quasi-biennial oscillation originates mainly from the southern hemisphere. Furthermore, we show that low degree modes with odd l — m exhibit periods of 29.2 and 28.1 days while modes with even l — m show a dominant period of 26.9 days. A resonant modal structure of the solar magnetic field (apart from the 22 yr cycle) has not been found.


2007 ◽  
Vol 7 (19) ◽  
pp. 5207-5228 ◽  
Author(s):  
M. C. Pitts ◽  
L. W. Thomason ◽  
L. R. Poole ◽  
D. M. Winker

Abstract. The role of polar stratospheric clouds in polar ozone loss has been well documented. The CALIPSO satellite mission offers a new opportunity to characterize PSCs on spatial and temporal scales previously impossible. A PSC detection algorithm based on a single wavelength threshold approach has been developed for CALIPSO. The method appears to accurately detect PSCs of all opacities, including tenuous clouds, with a very low rate of false positives and few missed clouds. We applied the algorithm to CALIOP data acquired during the 2006 Antarctic winter season from 13 June through 31 October. The spatial and temporal distribution of CALIPSO PSC observations is illustrated with weekly maps of PSC occurrence. The evolution of the 2006 PSC season is depicted by time series of daily PSC frequency as a function of altitude. Comparisons with "virtual" solar occultation data indicate that CALIPSO provides a different view of the PSC season than attained with previous solar occultation satellites. Measurement-based time series of PSC areal coverage and vertically-integrated PSC volume are computed from the CALIOP data. The observed area covered with PSCs is significantly smaller than would be inferred from the commonly used temperature-based proxy TNAT but is similar in magnitude to that inferred from TSTS. The potential of CALIOP measurements for investigating PSC composition is illustrated using combinations of lidar backscatter and volume depolarization for two CALIPSO PSC scenes.


2020 ◽  
Author(s):  
Yoshio Kawatani ◽  
Toshihiko Hirooka ◽  
Kevin Hamilton ◽  
Anne K. Smith ◽  
Masatomo Fujiwara

Abstract. This paper reports on a project to compare the representation of the semiannual oscillation (SAO) in the equatorial stratosphere and lower mesosphere among six major global atmospheric reanalysis datasets and with recent satellite SABER and MLS observations. All reanalyses have a good representation of the quasi-biennial oscillation (QBO) in the equatorial lower and middle stratosphere and each displays a clear SAO centered near the stratopause. However, the differences among reanalyses are much more substantial in the SAO region than in the QBO dominated region. The degree of disagreement among the reanalyses is characterized by the standard deviation (SD) of the monthly-mean zonal wind and temperature; this depends on latitude, longitude, height, and time. The zonal wind SD displays a prominent equatorial maximum that increases with height, while the temperature SD is minimum near the equator and largest in the polar regions. Along the equator the zonal wind SD is smallest around the longitude of Singapore where consistently high-quality near-equatorial radiosonde observations are available. Interestingly the near-Singapore minimum in SD is evident to at least ~ 3 hPa, i.e. considerably higher than the usual ~ 10 hPa ceiling for in situ radiosonde observations. Our measurement of the agreement among the reanalyses shows systematic improvement over the period considered (1980–2016), up to near the stratopause. Characteristics of the SAO at 1 hPa, such as its detailed time variation and the displacement off the equator of the zonal wind SAO amplitude maximum, differ significantly among the reanalyses. Disagreement among the reanalyses becomes still greater above 1 hPa. One of the reanalyses in our study also has a version produced without assimilating satellite observations and a comparison of the SAO in these two versions demonstrates the very great importance of satellite derived temperatures in the realistic analysis of the tropical upper stratospheric circulation.


2020 ◽  
Author(s):  
Florent Tencé ◽  
Julien Jumelet ◽  
Alain Sarkissian ◽  
Slimane Bekki ◽  
Philippe Keckhut

&lt;p&gt;&lt;span&gt;Polar Stratospheric Clouds (PSCs) play a primary role in polar stratospheric ozone depletion processes. &lt;/span&gt;&lt;span&gt;Aside from recent improvements in both spaceborne PSCs monitoring as well as investigations on PSCs microphysics and modeling, there are still uncertainties associated to solid particle formation and their denitrification potential. In that regard, groundbased instruments deliver detailed and valuable measurements that complement the global spaceborne coverage.&lt;/span&gt;&lt;/p&gt;&lt;p&gt;Operated since 1989 at the French antarctic station Dumont d&amp;#8217;Urville (DDU) in the frame of the international Network for the Detection of Atmospheric Composition Change (NDACC), the Rayleigh/Mie/Raman lidar provides over the years a solid dataset to feed both process and classification studies, by monitoring cloud and aerosol occurrences in the upper troposphere and lower stratosphere. Located on antarctic shore (66&amp;#176;S - 140&amp;#176;E), the station has a privileged access to polar vortex dynamics. Measurements are weather-dependent with a yearly average of 130 nights of monitoring. Expected PSC formation temperatures are used to evaluate the whole PSC season occurrences.&lt;/p&gt;&lt;p&gt;We hereby present a consolidated dataset from 10 years of lidar measurements using the 532nm backscatter ratio, the aerosol depolarisation and local atmospheric conditions to help in building an aerosol/cloud classification. Using the different PSC classes and associated optical properties thresholds established in the recent PSC CALIOP classification, we build a picture of the 2007-2019 events, from march to october.&lt;/p&gt;&lt;p&gt;Overall, the DDU PSC pattern is very consistent with expected typical temperature controlled microphysical calculations. Outside of background sulfate aerosols and anomalies related to volcanic activity (like in 2015), Supercooled Ternary Solution (STS) particles are the most observed particle type, closely followed by Nitric Acid Trihydrate (NAT). ICE clouds are less but regularly observed. ICE clouds also have to be cleary separated from cirrus clouds, raising the issue of accurate dynamics tropopause calculations.&lt;/p&gt;&lt;p&gt;&lt;span&gt;Validation of the spaceborne measurements as well as multiple signatures of volcanic or even biomass originated aerosol plumes strengthens the need for groundbased monitoring &lt;/span&gt;&lt;span&gt;especially in polar regions where instrumental facilities remain sparse.&lt;/span&gt;&lt;/p&gt;


2020 ◽  
Vol 20 (14) ◽  
pp. 9115-9133
Author(s):  
Yoshio Kawatani ◽  
Toshihiko Hirooka ◽  
Kevin Hamilton ◽  
Anne K. Smith ◽  
Masatomo Fujiwara

Abstract. This paper reports on a project to compare the representation of the semiannual oscillation (SAO) in the equatorial stratosphere and lower mesosphere within six major global atmospheric reanalysis datasets and with recent satellite Sounding of the Atmosphere Using Broadband Emission Radiometry (SABER) and Microwave Limb Sounder (MLS) observations. All reanalyses have a good representation of the quasi-biennial oscillation (QBO) in the equatorial lower and middle stratosphere and each displays a clear SAO centered near the stratopause. However, the differences among reanalyses are much more substantial in the SAO region than in the QBO-dominated region. The degree of disagreement among the reanalyses is characterized by the standard deviation (SD) of the monthly mean zonal wind and temperature; this depends on latitude, longitude, height, and time. The zonal wind SD displays a prominent equatorial maximum that increases with height, while the temperature SD reaches a minimum near the Equator and is largest in the polar regions. Along the Equator, the zonal wind SD is smallest around the longitude of Singapore, where consistently high-quality near-equatorial radiosonde observations are available. Interestingly, the near-Singapore minimum in SD is evident to at least ∼3 hPa, i.e., considerably higher than the usual ∼10 hPa ceiling for in situ radiosonde observations. Our measurement of the agreement among the reanalyses shows systematic improvement over the period considered (1980–2016), up to near the stratopause. Characteristics of the SAO at 1 hPa, such as its detailed time variation and the displacement off the Equator of the zonal wind SAO amplitude maximum, differ significantly among the reanalyses. Disagreement among the reanalyses becomes still greater above 1 hPa. One of the reanalyses in our study also has a version produced without assimilating satellite observations, and a comparison of the SAO in these two versions demonstrates the very great importance of satellite-derived temperatures in the realistic analysis of the tropical upper stratospheric circulation.


2014 ◽  
Vol 14 (17) ◽  
pp. 24623-24666 ◽  
Author(s):  
C. Vigouroux ◽  
T. Blumenstock ◽  
M. Coffey ◽  
Q. Errera ◽  
O. García ◽  
...  

Abstract. Ground-based Fourier transform infrared (FTIR) measurements of solar absorption spectra can provide ozone total columns with a precision of 2%, but also independent partial column amounts in about four vertical layers, one in the troposphere and three in the stratosphere up to about 45 km, with a precision of 5–6%. We use eight of the Network for the Detection of Atmospheric Compososition Change (NDACC) stations having a long-term time series of FTIR ozone measurements to study the total and vertical ozone trends and variability, namely: Ny-Alesund (79° N), Thule (77° N), Kiruna (68° N), Harestua (60° N), Jungfraujoch (47° N), Izaña (28° N), Wollongong (34° S) and Lauder (45° S). The length of the FTIR time-series varies by station, but is typically from about 1995 to present. We applied to the monthly means of the ozone total and four partial columns a stepwise multiple regression model including the following proxies: solar cycle, Quasi-Biennial Oscillation (QBO), El Niño-Southern Oscillation (ENSO), Arctic and Antarctic Oscillation (AO/AAO), tropopause pressure (TP), equivalent latitude (EL), Eliassen-Palm flux (EPF), and volume of polar stratospheric clouds (VPSC). At the Arctic stations, the trends are found mostly negative in the troposphere and lower stratosphere, very mixed in the middle stratosphere, positive in the upper stratosphere due to a large increase in the 1995–2003 period, and non-significant when considering the total columns. The trends for mid-latitude and subtropical stations are all non-significant, except at Lauder in the troposphere and upper stratosphere, and at Wollongong for the total columns and the lower and middle stratospheric columns; at Jungfraujoch, the upper stratospheric trend is close to significance (+0.9 ± 1.0 % decade−1). Therefore, some signs of the onset of ozone mid-latitude recovery are observed only in the Southern Hemisphere, while a few more years seems to be needed to observe it at the northern mid-latitude station.


2007 ◽  
Vol 7 (3) ◽  
pp. 7933-7985 ◽  
Author(s):  
M. C. Pitts ◽  
L. W. Thomason ◽  
L. R. Poole ◽  
D. M. Winker

Abstract. The role of polar stratospheric clouds in polar ozone loss has been well documented. The CALIPSO satellite mission offers a new opportunity to characterize PSCs on spatial and temporal scales previously impossible. A PSC detection algorithm based on a single wavelength threshold approach has been developed for CALIPSO. The method appears to accurately detect PSCs of all opacities, including tenuous clouds, with a very low rate of false positives and few missed clouds. We applied the algorithm to CALIOP data acquired during the 2006 Antarctic winter season from 13 June through 31 October. The spatial and temporal distribution of CALIPSO PSC observations is illustrated with weekly maps of PSC occurrence. The evolution of the 2006 PSC season is depicted by time series of daily PSC frequency as a function of altitude. Comparisons with "virtual" solar occultation data indicate that CALIPSO provides a different view of the PSC season than attained with previous solar occultation satellites. Measurement-based time series of PSC areal coverage and vertically-integrated PSC volume are computed from the CALIOP data. The observed area covered with PSCs is significantly smaller than would be inferred from the commonly used temperature-based proxy TNAT but is similar in magnitude to that inferred from TSTS . The potential of CALIOP measurements for investigating PSC composition is illustrated using combinations of lidar backscatter and volume depolarization for two CALIPSO PSC scenes.


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