scholarly journals Sources and oxidative potential of water-soluble humic-like substances (HULIS<sub>WS</sub>) in fine particulate matter (PM<sub>2.5</sub>) in Beijing

2017 ◽  
Author(s):  
Yiqiu Ma ◽  
Yubo Cheng ◽  
Xinghua Qiu ◽  
Gang Cao ◽  
Yanhua Fang ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Biomass Burning ◽  
Fine Particulate Matter ◽  
Waste Incineration ◽  
Water Soluble ◽  
Redox Activity ◽  
Aerosol Formation ◽  
Heating Season ◽  
Secondary Aerosol ◽  
Fine Particulate

Abstract. Water-soluble humic-like substances (HULISWS) are a major redox-active component of ambient fine particulate matter (PM2.5); however, information on their sources and associated redox activity is limited. In this study, total HULISWS, various HULISWS species, and HULISWS-associated dithiothreitol (DTT) activity were quantified in PM2.5 samples collected during a 1-year period in Beijing. Strong correlation was observed between HULISWS and DTT activity; both exhibited higher levels during the heating season than during the non-heating season. Positive matrix factorization analysis of both HULISWS and DTT activity was performed. Four combustion-related sources, namely coal combustion, biomass burning, waste incineration, and vehicle exhaust, and one secondary factor were resolved. In particular, waste incineration was identified as a source of HULISWS for the first time. Biomass burning and secondary aerosol formation were the major contributors (> 59 %) to both HULISWS and associated DTT activity throughout the year. During the non-heating season, secondary aerosol formation was the most important source, whereas during the heating season, the predominant contributor was biomass burning. The four combustion-related sources accounted for > 70 % of HULISWS and DTT activity, implying that future reduction in PM2.5 emissions from combustion activities can substantially reduce the HULISWS burden and their potential health impact in Beijing.

scholarly journals Sources and oxidative potential of water-soluble humic-like substances (HULIS<sub>WS</sub>) in fine particulate matter (PM<sub>2.5</sub>) in Beijing

2018 ◽  
Vol 18 (8) ◽  
pp. 5607-5617 ◽  
Author(s):  
Yiqiu Ma ◽  
Yubo Cheng ◽  
Xinghua Qiu ◽  
Gang Cao ◽  
Yanhua Fang ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Biomass Burning ◽  
Fine Particulate Matter ◽  
Waste Incineration ◽  
Water Soluble ◽  
Redox Activity ◽  
Aerosol Formation ◽  
Heating Season ◽  
Secondary Aerosol ◽  
Fine Particulate

Abstract. Water-soluble humic-like substances (HULISWS) are a major redox-active component of ambient fine particulate matter (PM2.5); however, information on their sources and associated redox activity is limited. In this study, HULISWS mass concentration, various HULISWS species, and dithiothreitol (DTT) activity of HULISWS were quantified in PM2.5 samples collected during a 1-year period in Beijing. Strong correlation was observed between HULISWS and DTT activity; both exhibited higher levels during the heating season than during the nonheating season. Positive matrix factorization analysis of both HULISWS and DTT activity was performed. Four combustion-related sources, namely coal combustion, biomass burning, waste incineration, and vehicle exhausts, and one secondary factor were resolved. In particular, waste incineration was identified as a source of HULISWS for the first time. Biomass burning and secondary aerosol formation were the major contributors (> 59 %) to both HULISWS and associated DTT activity throughout the year. During the nonheating season, secondary aerosol formation was the most important source, whereas during the heating season, the predominant contributor was biomass burning. The four combustion-related sources accounted for > 70 % of HULISWS and DTT activity, implying that future reduction in PM2.5 emissions from combustion activities can substantially reduce the HULISWS burden and their potential health impact in Beijing.

Insights into the Origin of Water Soluble Organic Carbon in Atmospheric Fine Particulate Matter

2009 ◽  
Vol 43 (11) ◽  
pp. 1099-1107 ◽  
Author(s):  
David C. Snyder ◽  
Andrew P. Rutter ◽  
Ryan Collins ◽  
Chris Worley ◽  
James J. Schauer
Keyword(s):  
Particulate Matter ◽  
Organic Carbon ◽  
Fine Particulate Matter ◽  
Water Soluble ◽  
Fine Particulate ◽  
Water Soluble Organic Carbon ◽  
Soluble Organic Carbon

scholarly journals Spatial and temporal variability of sources of ambient fine particulate matter (PM<sub>2.5</sub>) in California

2014 ◽  
Vol 14 (22) ◽  
pp. 12085-12097 ◽  
Author(s):  
S. Hasheminassab ◽  
N. Daher ◽  
A. Saffari ◽  
D. Wang ◽  
B. D. Ostro ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Biomass Burning ◽  
Total Mass ◽  
Fine Particulate Matter ◽  
The State ◽  
Vehicular Emissions ◽  
San Jose ◽  
Annual Average ◽  
Fine Particulate ◽  
Sampling Locations

Abstract. To identify major sources of ambient fine particulate matter (PM2.5, dp < 2.5 μm) and quantify their contributions in the state of California, a positive matrix factorization (PMF) receptor model was applied on Speciation Trends Network (STN) data, collected between 2002 and 2007 at eight distinct sampling locations, including El Cajon, Rubidoux, Los Angeles, Simi Valley, Bakersfield, Fresno, San Jose, and Sacramento. Between five to nine sources of fine PM were identified at each sampling site, several of which were common among multiple locations. Secondary aerosols, including secondary ammonium nitrate and ammonium sulfate, were the most abundant contributor to ambient PM2.5 mass at all sampling sites, except for San Jose, with an annual average cumulative contribution of 26 to 63%, across the state. On an annual average basis, vehicular emissions (including both diesel and gasoline vehicles) were the largest primary source of fine PM at all sampling sites in southern California (17–18% of total mass), whereas in Fresno and San Jose, biomass burning was the most dominant primary contributor to ambient PM2.5 (27 and 35% of total mass, respectively), in general agreement with the results of previous source apportionment studies in California. In Bakersfield and Sacramento, vehicular emissions and biomass burning displayed relatively equal annual contributions to ambient PM2.5 mass (12 and 25%, respectively). Other commonly identified sources at all sites included aged and fresh sea salt and soil, which contributed to 0.5–13%, 2–27%, and 1–19% of the total mass, respectively, across all sites and seasons. In addition, a few minor sources were identified exclusively at some of the sites (e.g., chlorine sources, sulfate-bearing road dust, and different types of industrial emissions). These sources overall accounted for a small fraction of the total PM mass across the sampling locations (1 to 15%, on an annual average basis).

scholarly journals Fine Particulate Matter Pollution Characteristics and Source Apportionment of Changchun Atmosphere

2021 ◽  
Author(s):  
Jie Tang ◽  
Zhuo Yang ◽  
Yue Tui ◽  
Ju Wang
Keyword(s):  
Particulate Matter ◽  
Mass Concentration ◽  
Elemental Carbon ◽  
Motor Vehicle ◽  
Fine Particulate Matter ◽  
Water Soluble ◽  
Chemical Components ◽  
Sample Collection ◽  
Pollution Characteristics ◽  
Fine Particulate

Abstract In order to study the pollution characteristics and main sources of fine particulate matter in the atmosphere of the city of Changchun, PM2.5 samples were collected during the four seasons in 2014, and representative months for each season are January, April, July, and October. Sample collection was carried out on 10 auto-monitoring stations in Changchun, and PM2.5 mass concentration, and its chemical components (including inorganic elements, organic carbon, elemental carbon, and water-soluble ions) were measured. The results show that the annual average mass concentration of PM2.5 in Changchun in 2014 was about 66.77 µg/m3. Organic matter was the highest component in PM2.5, followed by secondary inorganic ions (SNA), mineral dust (MIN), elemental carbon (EC), and trace elements (TE). Positive Matrix Factorization (PMF) results gave seven factors, namely, industrial, biomass- and coal-burning, industrial and soil dust, motor-vehicle, soil and secondary-ion, light-industrial, and hybrid-automotive and -industrial sources in PM2.5, with contributing values of 18.9%, 24.2%, 5.7%, 23.0%, 11.5%, 13.0%, and 3.6%, respectively.

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