scholarly journals Sensitivity of aerosol optical properties to the aerosol size distribution over central Europe and the Mediterranean Basin

2020 ◽  
Keyword(s):  
Optical Properties ◽  
Size Distribution ◽  
Central Europe ◽  
Mediterranean Basin ◽  
Aerosol Size Distribution ◽  
Aerosol Optical Properties ◽  
The Mediterranean ◽  
The Mediterranean Basin

scholarly journals Sensitivity of aerosol optical properties to the aerosol size distribution over central Europe and the Mediterranean Basin using the WRF-Chem v.3.9.1.1 coupled model

2020 ◽  
Vol 13 (12) ◽  
pp. 5897-5915
Author(s):  
Laura Palacios-Peña ◽  
Jerome D. Fast ◽  
Enrique Pravia-Sarabia ◽  
Pedro Jiménez-Guerrero
Keyword(s):  
Optical Properties ◽  
Standard Deviation ◽  
Size Distribution ◽  
Central Europe ◽  
Mediterranean Basin ◽  
Aerosol Size Distribution ◽  
Aerosol Optical Properties ◽  
Accumulation Mode ◽  
The Mediterranean ◽  
The Mediterranean Basin

Abstract. The size distribution of atmospheric aerosols plays a key role for understanding and quantifying the uncertainties related to aerosol–radiation and aerosol–cloud interactions. These interactions ultimately depend on the size distribution through optical properties (such as aerosol optical depth, AOD) or cloud microphysical properties. Hence, the main objective of this contribution is to disentangle the impact of the representation of aerosol size distribution on aerosol optical properties over central Europe, particularly over the Mediterranean Basin, during a summertime aerosol episode. To fulfill this objective, a sensitivity test has been conducted using the coupled chemistry–meteorology model WRF-Chem (Weather Research Forecast model coupled with Chemistry). The test modified the parameters defining a lognormal size distribution (geometric diameter and standard deviation) by 10 %, 20 %, and 50 %. Results reveal that the reduction in the standard deviation of the accumulation mode leads to the largest impacts on AOD due to a transfer of particles from the accumulation mode to the coarse mode. A reduction in the geometric diameter of the accumulation mode also has an influence on AOD representation since particles in this mode are assumed to be smaller. In addition, an increase in the geometric diameter of the coarse mode produces a redistribution through the total size distribution by relocating particles from the finer modes to the coarse.

scholarly journals Sensitivity of aerosol optical properties to the aerosol size distribution over central Europe and the Mediterranean Basin

2020 ◽  
Author(s):  
Laura Palacios-Peña ◽  
Jerome D. Fast ◽  
Enrique Pravia-Sarabia ◽  
Pedro Jiménez-Guerrero
Keyword(s):  
Optical Properties ◽  
Size Distribution ◽  
Central Europe ◽  
Mediterranean Basin ◽  
Aerosol Size Distribution ◽  
Aerosol Optical Properties ◽  
Accumulation Mode ◽  
Coarse Mode ◽  
The Mediterranean ◽  
The Mediterranean Basin

Abstract. Aerosol size distribution is, among others, a key property of atmospheric aerosols when trying to establish the uncertainties related to aerosol-radiation (ARI) and aerosol-clouds (ACI) interactions. These interactions ultimately depend on the size distribution through optical properties as aerosol optical depth (AOD) or cloud microphysical properties. Hence, the main objective of this work is to study the impact of the representation of aerosol size distribution on aerosol optical properties over Central Europe, and particularly over the Mediterranean Basin during a summertime aerosol episode. To fulfill this objective, a sensitivity test has been carried out using the WRF-Chem on-line model. The test consisted on modifying the parameters which define a log-normal size distribution (the geometric diameter, from now on DG, and the standard deviation, SG) by 10, 20 and 50 %. Results reveal that the reduction in the SG of the accumulation mode leads to the largest impacts in the AOD representation due to a transfer of particles from the accumulation mode to the coarse mode. A reduction in the DG of the accumulation mode has also an influence on AOD representation since particles in this mode are assumed to be smaller. In addition, an increase in the DG of the coarse mode produces a redistribution through the total size distribution by relocating particles from the finer modes to the coarse.

scholarly journals Spatio-Temporal Identification of Areas Suitable for West Nile Disease in the Mediterranean Basin and Central Europe

PLoS ONE ◽  
2015 ◽  
Vol 10 (12) ◽  
pp. e0146024 ◽  
Author(s):  
Annamaria Conte ◽  
Luca Candeloro ◽  
Carla Ippoliti ◽  
Federica Monaco ◽  
Fabrizio De Massis ◽  
...  
Keyword(s):  
Central Europe ◽  
Mediterranean Basin ◽  
West Nile ◽  
The Mediterranean ◽  
Spatio Temporal ◽  
The Mediterranean Basin

scholarly journals Dust emission size distribution impact on aerosol budget and radiative forcing over the Mediterranean region: a regional climate model approach

2012 ◽  
Vol 12 (21) ◽  
pp. 10545-10567 ◽  
Author(s):  
P. Nabat ◽  
F. Solmon ◽  
M. Mallet ◽  
J. F. Kok ◽  
S. Somot
Keyword(s):  
Size Distribution ◽  
Radiative Forcing ◽  
Mediterranean Basin ◽  
Climate Model ◽  
Regional Climate ◽  
Dust Emission ◽  
Dust Deposition ◽  
The Mediterranean ◽  
Dust Distribution ◽  
The Mediterranean Basin

Abstract. The present study investigates the dust emission and load over the Mediterranean basin using the coupled chemistry–aerosol–regional climate model RegCM-4. The first step of this work focuses on dust particle emission size distribution modeling. We compare a parameterization in which the emission is based on the individual kinetic energy of the aggregates striking the surface to a recent parameterization based on an analogy with the fragmentation of brittle materials. The main difference between the two dust schemes concerns the mass proportion of fine aerosol that is reduced in the case of the new dust parameterization, with consequences for optical properties. At the episodic scale, comparisons between RegCM-4 simulations, satellite and ground-based data show a clear improvement using the new dust distribution in terms of aerosol optical depth (AOD) values and geographic gradients. These results are confirmed at the seasonal scale for the investigated year 2008. This change of dust distribution has sensitive impacts on the simulated regional dust budget, notably dry dust deposition and the regional direct aerosol radiative forcing over the Mediterranean basin. In particular, we find that the new size distribution produces a higher dust deposition flux, and smaller top of atmosphere (TOA) dust radiative cooling. A multi-annual simulation is finally carried out using the new dust distribution over the period 2000–2009. The average SW radiative forcing over the Mediterranean Sea reaches −13.6 W m−2 at the surface, and −5.5 W m−2 at TOA. The LW radiative forcing is positive over the basin: 1.7 W m−2 on average over the Mediterranean Sea at the surface, and 0.6 W m−2 at TOA.

scholarly journals Aerosol direct radiative forcing during Sahara dust intrusions in the Central Mediterranean

2010 ◽  
Vol 10 (8) ◽  
pp. 20673-20727
Author(s):  
M. R. Perrone ◽  
A. Bergamo ◽  
V. Bellantone
Keyword(s):  
Optical Properties ◽  
Radiative Transfer ◽  
Spectral Range ◽  
Mediterranean Basin ◽  
Transfer Model ◽  
Clear Sky ◽  
Fine Mode ◽  
The Mediterranean ◽  
The Mediterranean Basin ◽  
Sahara Dust

Abstract. The clear-sky, instantaneous Direct Radiative Effect (DRE) by all and anthropogenic particles is calculated during Sahara dust intrusions in the Mediterranean basin, to evaluate the role of anthropogenic particle's radiative effects and to obtain a better estimate of the DRE by desert dust. The clear-sky aerosol DRE is calculated by a two stream radiative transfer model in the solar (0.3–4 μm) and infrared (4–200 μm) spectral range, at the top of the atmosphere (ToA) and at the Earth's surface (sfc). Aerosol optical properties by AERONET sun-sky photometer measurements and aerosol vertical profiles by EARLINET lidar measurements, both performed at Lecce (40.33° N, 18.10° E) during Sahara dust intrusions occurred from 2003 to 2006 year, are used to perform radiative transfer simulations. Instantaneous values at 0.44 μm of the real (n) and imaginary (k) refractive index and of the of aerosol optical depth (AOD) vary within the 1.33–1.55, 0.0037–0.014, and 0.2–0.7 range, respectively during the analyzed dust outbreaks. Fine mode particles contribute from 34% to 85% to the AOD by all particles. The complex atmospheric chemistry of the Mediterranean basin that is also influenced by regional and long-range transported emissions from continental Europe and the dependence of dust optical properties on soil properties of source regions and transport pathways, are responsible for the high variability of n, k, and AOD values and of the fine mode particle contribution. Instantaneous all-wave (solar+infrared) DREs that are negative as a consequence of the cooling effect by aerosol particles, span the – (32–10) Wm−2 and the – (44–20) Wm−2 range at the ToA and surface, respectively. The instantaneous all-wave DRE by anthropogenic particles that is negative, varies within – (13–7) Wm−2 and – (18–11) Wm−2 at the ToA and surface, respectively. It represents from 41% up to 89% and from 32% up to 67% of the all-wave DRE by all particles at the ToA and surface, respectively during the analysed dust outbreaks. A linear relationship to calculate the DRE by natural particles in the solar and infrared spectral range is provided.

scholarly journals Aerosol direct radiative forcing during Sahara dust intrusions in the central Mediterranean

2009 ◽  
Vol 9 (5) ◽  
pp. 22539-22579 ◽  
Author(s):  
M. R. Perrone ◽  
A. Bergamo ◽  
V. Bellantone
Keyword(s):  
Optical Properties ◽  
Radiative Transfer ◽  
Spectral Range ◽  
Mediterranean Basin ◽  
Transfer Model ◽  
Clear Sky ◽  
Fine Mode ◽  
The Mediterranean ◽  
The Mediterranean Basin ◽  
Sahara Dust

Abstract. The clear-sky, instantaneous Direct Radiative Effect (DRE) by all and anthropogenic particles is calculated during Sahara dust intrusions in the Mediterranean basin, to evaluate the role of anthropogenic particle's radiative effects and to get a better estimate of the DRE by desert dust. The clear-sky aerosol DRE is calculated by a two stream radiative transfer model in the solar (0.3–4 μm) and infrared (4–200 μm) spectral range, at the top of the atmosphere (ToA) and at the Earth's surface (sfc). Aerosol optical properties by AERONET sun-sky photometer measurements and aerosol vertical profiles by EARLINET lidar measurements, both performed at Lecce (40.33° N, 18.10° E) during Sahara dust intrusions occurred from 2003 to 2006 year, are used to initialize radiative transfer simulations. Instantaneous values at 0.44 μm of the real (n) and imaginary (k) refractive index and of the of aerosol optical depth (AOD) vary within the 1.33–1.55, 0.0037–0.014, and 0.2–0.7 range, respectively during the analyzed dust outbreaks. Fine mode particles contribute from 34% to 85% to the AOD by all particles. The complex atmospheric chemistry of the Mediterranean basin that is also influenced by regional and long-range transported emissions from continental Europe and the dependence of dust optical properties on soil properties of source regions and transport pathways are responsible for the high variability of n, k, and AOD values and of the fine mode particle contribution. Instantaneous net (solar+infrared) DREs that are negative as a consequence of the cooling effect by aerosol particles, span the – (32–10) W m−2 and the – (44–20) W m−2 range at the ToA and surface, respectively. The instantaneous net DRE by anthropogenic particles that is negative, varies within −(13–8) W m−2 and −(17–11) W m−2 at the ToA and surface, respectively. It represents from 41 up to 89% and from 36 up to 67% of the net DRE by all particles at the ToA and surface, respectively. A linear relationship to calculate the DRE by natural particles in the solar and infrared spectral range is provided.

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