Inverse modeling of the 2021 spring super dust storms in East Asia

This spring, super dust storms reappeared in East Asia after being absent for a (two) decade(s). The event caused enormous losses both in Mongolia and in China. Accurate simulation of such super sandstorms is valuable for the quantification of health damages, aviation risks, and profound impacts on the Earth system, but also to reveal the driving climate and the process of desertification. However, accurate simulation of dust life cycles is challenging mainly due to imperfect knowledge of emissions. In this study, the emissions that lead to the 2021 spring dust storms are estimated through assimilation of MODIS AOD and ground-based PM10 concentration data. To be able to use the AOD observations to represent the dust load, an Angstrom-based data screening is designed to select only observations that are dominated by dust. In addition, a non-dust AOD bias correction has been designed to remove the part of the AOD that could be attributed to other aerosols than dust. With this, the dust concentrations during the 2021 spring super storms could be reproduced and validated with concentration observations. The emission inversion results reveal that wind blown dust emissions originated from both China and Mongolia during spring 2021. Specifically, 18.3M and 27.2M ton of particles were released in Chinese desert and Mongolia desert respectively during these severe dust events. By source apportionment it has been estimated that 58 % of the dust deposited in the densely populated Fenwei Plain (FWP) in the northern China originate from transnational transport from Mongolia desert. For the North China Plain (NCP), local Chinese desert play a less significant roles in the dust affection; the long-distance transport from Mongolia contributes for about 69 % to the dust deposition in NCP, even if it locates more than 1000 km away from the nearest Mongolian desert.

Atmospheric Iron and Aluminium Deposition and Sea-Surface Dissolved Iron and Aluminium Concentrations in the South China Sea off Malaysia Borneo (Sarawak Waters)

South China Sea (SCS) is an oligotrophic sea which usually receives low nutrients supply. However, massive atmospheric dust input was occurred during the haze event in Southeast Asia for almost every year. The input of dissolved iron (DFe) and dissolved aluminium (DAl) from dust and nearby land into SCS off Sarawak Borneo region during the worst haze event in 2015 of the Southeast Asia were investigated. The estimation dust deposition during this study was 0.162 mg/m2/yr. The atmospheric fluxes of total Fe and total Al at the offshore Sarawak waters were 0.611 µmol/m2/yr and 2.03 µmol/m2/yr, respectively, where the readily available dissolved Fe and Al from the dust were 0.11 µmol/m2/yr (DFe) and 0.31 µmol/m2/yr (DAl). Fe has higher solubility (17.78%) than Al (15.21%). The lateral fluxes (e.g. from the nearby land) were 37.08 nmol/m2/yr (DFe) and 125 nmol/m2/yr (DAl), with strong Fe organic ligand class L1 (log K:22.43 – 24.33). High concentrations of DFe and DAl at the surface water of the offshore region, coincided with high concentration of macronutrients due to the prevailing south-westerly winds originated from the west Kalimantan. Low residence times, ~0.92 (DFe) and ~1.31 (DAl) years, corresponded well with DAlexcess in surface seawater due to biological utilization of DFe. Future works emphasize on natural organic Fe(III) ligands and phytoplankton study are needed for better understanding on biogeochemistry of Fe and Al at SCS off Malaysia Borneo.

Liquid-mediated particle capture by nonwoven filter media for automotive engine intake air filtration

This article reports on development, characterization, and performance of liquid-treated nonwoven air filter media for automotive engine intake application. A polypropylene fiber-based needle-punched nonwoven fabric was prepared for treatment with four viscous liquids (glycerol, SAE 20W/50 engine oil, PEG 400, and deionized water) by liquid spraying technique. The filtration performance was evaluated in terms of initial and final gravimetric filtration efficiencies, fractional filtration efficiency, evolution of pressure drop, and dust holding capacity. The liquid-treated filter media registered higher gravimetric as well as fractional filtration efficiency and higher dust holding capacity as compared to the untreated ones. The initial and final gravimetric filtration efficiencies were found to be directly related to liquid add-on via a power law relationship. The liquid-treated filter media also exhibited higher fractional filtration efficiency than their untreated counterparts for all sizes of tested particles. Interestingly, the increase of fractional efficiency was more for smaller particles as compared to larger ones. This was explained quantitatively through single fiber efficiency due to adhesion. The viscosity of liquid was found to be a very crucial parameter as the dust deposition morphology was contingent to the flow of liquid onto the filter media. The stickiest liquid yielded highest filtration efficiencies, displayed slowest rise of pressure drop, and exhibited highest dust holding capacity.

Subsurface iron accumulation and rapid aluminum removal in the Mediterranean following African dust deposition

Mineral dust deposition is an important supply mechanism for trace elements in the low-latitude ocean. Our understanding of the controls of such inputs has been mostly built on laboratory and surface ocean studies. The lack of direct observations and the tendency to focus on near-surface waters prevent a comprehensive evaluation of the role of dust in oceanic biogeochemical cycles. In the frame of the PEACETIME project (ProcEss studies at the Air-sEa Interface after dust deposition in the MEditerranean sea), the responses of the aluminum (Al) and iron (Fe) cycles to two dust wet deposition events over the central and western Mediterranean Sea were investigated at a timescale of hours to days using a comprehensive dataset gathering dissolved and suspended particulate concentrations, along with sinking fluxes. Dissolved Al (dAl) removal was dominant over dAl released from dust. The Fe / Al ratio of suspended and sinking particles revealed that biogenic particles, and in particular diatoms, were key in accumulating and exporting Al relative to Fe. By combining these observations with published Al / Si ratios of diatoms, we show that adsorption onto biogenic particles, rather than active uptake, represents the main sink for dAl in Mediterranean waters. In contrast, systematic dissolved Fe (dFe) accumulation occurred in subsurface waters (∼ 100–1000 m), while dFe input from dust was only transient in the surface mixed layer. The rapid transfer of dust to depth, the Fe-binding ligand pool in excess to dFe in subsurface (while nearly saturated in surface), and low scavenging rates in this particle-poor depth horizon are all important drivers of this subsurface dFe enrichment. At the annual scale, this previously overlooked mechanism may represent an additional pathway of dFe supply for the surface ocean through diapycnal diffusion and vertical mixing. However, low subsurface dFe concentrations observed at the basin scale (

The Southern Ocean diatom Pseudo-nitzschia subcurvata flourished better under simulated glacial than interglacial ocean conditions: Combined effects of CO2 and iron

The ‘Iron Hypothesis’ suggests a fertilization of the Southern Ocean by increased dust deposition in glacial times. This promoted high primary productivity and contributed to lower atmospheric pCO2. In this study, the diatom Pseudo-nitzschia subcurvata, known to form prominent blooms in the Southern Ocean, was grown under simulated glacial and interglacial climatic conditions to understand how iron (Fe) availability (no Fe or Fe addition) in conjunction with different pCO2 levels (190 and 290 μatm) influences growth, particulate organic carbon (POC) production and photophysiology. Under both glacial and interglacial conditions, the diatom grew with similar rates. In comparison, glacial conditions (190 μatm pCO2 and Fe input) favored POC production by P. subcurvata while under interglacial conditions (290 μatm pCO2 and Fe deficiency) POC production was reduced, indicating a negative effect caused by higher pCO2 and low Fe availability. Under interglacial conditions, the diatom had, however, thicker silica shells. Overall, our results show that the combination of higher Fe availability with low pCO2, present during the glacial ocean, was beneficial for the diatom P. subcurvata, thus contributing more to primary production during glacial compared to interglacial times. Under the interglacial ocean conditions, on the other hand, the diatom could have contributed to higher carbon export due to its higher degree of silicification.