A Sediment Magnetic Record in the North Pacific Across the Mid-Pleistocene Transition and its Implication on Asian Dust Evolution

Eolian dust deposited in the North Pacific is an important archive of the evolutionary history of Asian interior source regions and climate system. Here, we present a ∼1 Myr sediment magnetic record from the central North Pacific to characterize eolian dust properties since the middle Pleistocene. For the studied sediments, magnetic components are mainly identified as biogenic magnetite and detrital magnetic minerals (dust and volcanic origins) based on coercivity analysis, microscopic observations, and sedimentological information. The detrital magnetic component is characterized by high coercivity (>100 mT) and shows a long-term increase in concentration since ∼1 Ma. In particular, the concentration shows a considerable increase at ∼0.8–0.7 Ma compared to the inorganic silicate fraction, indicative of magnetic mineral enrichment in detrital sediment fraction. At the same time, the coercivity distribution of the detrital component also decreases, which can be attributed to an increase in the ferrimagnetic mineral contribution. As the detrital sediments are primarily wind-blown particles, such ferrimagnetic enrichment implies a change in dust source materials after ∼0.8 Ma, which could be explained by the reorganization of atmospheric circulation and/or regional aridification in source regions across the mid-Pleistocene transition. The dust property change in source areas is likely to be synchronized across the North Pacific based on the similarity of the long-term trend of magnetic signals.

The 3.6-Ma aridity and westerlies history over midlatitude Asia linked with global climatic cooling

Midlatitude Asia (MLA), strongly influenced by westerlies-controlled climate, is a key source of global atmospheric dust, and plays a significant role in Earth’s climate system . However, it remains unclear how the westerlies, MLA aridity, and dust flux from this region evolved over time. Here, we report a unique high-resolution eolian dust record covering the past 3.6 Ma, retrieved from the thickest loess borehole sequence (671 m) recovered to date, at the southern margin of the Taklimakan desert in the MLA interior. The results show that eolian dust accumulation, which is closely related to aridity and the westerlies, indicates existence of a dry climate, desert area, and stable land surface, promoting continuous loess deposition since at least ∼3.6 Ma. This region experienced long-term stepwise drying at ∼2.7, 1.1, and 0.5 Ma, coeval with a dominant periodicity shift from 41-ka cyclicity to 100-ka cyclicity between 1.1 Ma and 0.5 Ma. These features match well with global ice volume variability both in the time and frequency domains (including the Mid-Pleistocene Transition), highlighting global cooling-forced aridity and westerlies climate changes on these timescales. Numerical modeling demonstrates that global cooling can dry MLA and intensify the westerlies, which facilitates dust emission and transport, providing an interpretive framework. Increased dust may have promoted positive feedbacks (e.g., decreasing atmospheric CO2 concentrations and modulating radiation budgets), contributing to further cooling. Unraveling the long-term evolution of MLA aridity and westerlies climate is an indispensable component of the unfolding mystery of global climate change.

Cenozoic Nd isotopic variation of Asian dust in the northern Tibetan Plateau and the North Pacific Ocean

<p>Cenozoic changes in climate, erosion, and atmospheric circulation in Asian interior continents can be reconstructed from records of eolian dust deposition from sediments of the North Pacific Ocean (NPO). Through a careful investigation of Nd isotope as eolian dust source tracer, the well-known core GPC3 in the central NPO has provided so far the most complete Asian dust records since ~40 Ma. Nd isotope in the GPC3 eolian dust thus documented an integrated history of Nd isotopic change of very fine eolian dust contributed from various geological terranes in Asian dust source areas. Unraveling this ~40 Myr-long Nd isotopic change in the NPO provides a first order constraint on the provenance change of the Asian dust source areas as a whole. However, this work cannot be done without an explicit Nd isotopic history for each geological terrane within the broad Asian dust source areas, since the Asian dust source area can be at least divided isotopically into two regions with distinct Nd isotopic values, e.g., the northern Tibetan Plateau (NTP) and the Central Asian Orogen (CAO). In this work, we present new data of river sediment Nd isotopic data around the entire Qaidam and Xining Basins to yield a more comprehensive Nd isotopic regimes at the NTP with compiling previously reported data. We have established an integrated Cenozoic Nd isotopic records of finer dust in the NTP based on previous records and our new Nd isotopic records in the Xining Basin from 52 to 17 Ma and Linxia basin from 23 to 5 Ma using both bulk sediments and clay fractions (<2 μm). After comparison of the reconstructed Nd isotopic variation in fine dust at the NTP with that in the NPO, we have further assessed the relative contributions of NTP and CAO to the Asian dust preserved in the NPO during the last 40 Myr, which indicates a dominant late Oligocene-Neogene uplift and growth of the mountains at the NTP and the CAO regions.</p>

Mechanism for enhanced eolian dust flux recorded in North Pacific Ocean sediments since 4.0 Ma: Aridity or humidity at dust source areas in the Asian interior?

Eolian material within pelagic North Pacific Ocean (NPO) sediments contains considerable information about paleoclimate evolution in Asian dust source areas. Eolian signals preserved in NPO sediments have been used as indices for enhanced Asian interior aridity. We here report a detailed eolian dust record, with chemical index of alteration (CIA) and Rb/Sr variations, for NPO sediments from Ocean Drilling Program Hole 885A over the past 4.0 m.y. CIA and Rb/Sr co-vary with the dust signal carried by combined eolian hematite and goethite concentrations. Changes in CIA around the intensification of Northern Hemisphere glaciation (iNHG) event at ca. 2.75 Ma indicate that dust production in source areas was associated mostly with physical and chemical weathering before and after the iNHG event, respectively. We here attribute the eolian flux increase into the NPO across the iNHG event mainly to increased availability of wind-erodible sediment in dust source areas derived from snow and glacial meltwater runoff, which resulted from glacial expansion and enhanced snowfall in the mountains surrounding the Tarim region in response to global cooling. Our results provide a deeper understanding of Asian interior environmental changes in response to global paleoclimate changes, where dust source areas became intermittently moister rather than more arid in response to global cooling.

Sources and origins of eolian dust to the Philippine Sea determined by major minerals and elemental geochemistry

We investigated the microscopic mineral characteristics of modern eolian dust particulates and the trace-element compositions of the siliciclastic fractions of these samples, collected from the Philippine Sea in 2014 and 2015, and conducted an air mass backwards trajectory analysis of dust particulates in the spring and winter of 2015, to better constrain the provenances and transport dynamics of dust delivered to this region. The microscopic minerals show obvious signatures of dust deposition and physical abrasion, indicating long-distance wind transport from the Asian deserts. The trace-element compositions (Zr–Th–Sc) display a binary mixture of eolian materials derived from the eastern Asian deserts and the central Asian deserts, which is similar to the result of the Sr–Nd isotopic compositions of modern sediment trap sediments collected on the Benham Rise in 2015. We demonstrate that modern dust sediments in the Philippine Sea primarily originate from the Ordos Desert (generally > 80%), while the contributions of the Taklimakan Desert and the Badain Jaran Desert are small. Eolian dust particulates raised from source regions are predominantly transported to the Philippine Sea by the East Asian winter monsoon, but not by the westerlies. In addition, our results indicate that increased precipitation in the source regions can result in relatively low dust fluxes in the Philippine Sea, and there is a period of 6–7 days for eolian dust originating from source areas to be delivered to the Philippine Sea.