scholarly journals The impact of abrupt suspension of solar radiation management (termination effect) in experiment G2 of the Geoengineering Model Intercomparison Project (GeoMIP)

2013 ◽  
Vol 118 (17) ◽  
pp. 9743-9752 ◽  
Author(s):  
Andy Jones ◽  
Jim M. Haywood ◽  
Kari Alterskjaer ◽  
Olivier Boucher ◽  
Jason N. S. Cole ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Solar Radiation Management ◽  
Model Intercomparison ◽  
Intercomparison Project ◽  
Radiation Management ◽  
The Impact

scholarly journals Heterogeneous reaction of N<sub>2</sub>O<sub>5</sub> with airborne TiO<sub>2</sub> particles and its implication for stratospheric particle injection

2014 ◽  
Vol 14 (4) ◽  
pp. 4421-4456 ◽  
Author(s):  
M. J. Tang ◽  
P. J. Telford ◽  
F. D. Pope ◽  
L. Rkiouak ◽  
N. L. Abraham ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Climate Model ◽  
Heterogeneous Reaction ◽  
High Refractive Index ◽  
Heterogeneous Reactions ◽  
Solar Radiation Management ◽  
Particle Injection ◽  
Stratospheric Chemistry ◽  
Radiation Management ◽  
The Impact

Abstract. Injection of aerosol particles (or their precursors) into the stratosphere to scatter solar radiation back into space, has been suggested as a solar-radiation management scheme for the mitigation of global warming. TiO2 has recently been highlighted as a possible candidate particle because of its high refractive index, but its impact on stratospheric chemistry via heterogeneous reactions is as yet unknown. In this work the heterogeneous reaction of airborne sub-micrometre TiO2 particles with N2O5 has been investigated for the first time, at room temperature and different relative humidities (RH), using an atmospheric pressure aerosol flow tube. The uptake coefficient of N2O5 onto TiO2, γ(N2O5), was determined to be ∼ 1.0 × 10−3 at low RH, increasing to ∼ 3 × 10−3 at 60% RH. The uptake of N2O5 onto TiO2 is then included in the UKCA chemistry climate model to assess the impact of this reaction on stratospheric chemistry. While the impact of TiO2 on the scattering of solar radiation is chosen to be similar to the aerosol from the Mt. Pinatubo eruption, the impact of TiO2 injection on stratospheric N2O5 is much smaller.

scholarly journals Heterogeneous reaction of N<sub>2</sub>O<sub>5</sub> with airborne TiO<sub>2</sub> particles and its implication for stratospheric particle injection

2014 ◽  
Vol 14 (12) ◽  
pp. 6035-6048 ◽  
Author(s):  
M. J. Tang ◽  
P. J. Telford ◽  
F. D. Pope ◽  
L. Rkiouak ◽  
N. L. Abraham ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Climate Model ◽  
Heterogeneous Reaction ◽  
High Refractive Index ◽  
Heterogeneous Reactions ◽  
Solar Radiation Management ◽  
Particle Injection ◽  
Stratospheric Chemistry ◽  
Radiation Management ◽  
The Impact

Abstract. Injection of aerosol particles (or their precursors) into the stratosphere to scatter solar radiation back into space has been suggested as a solar-radiation management scheme for the mitigation of global warming. TiO2 has recently been highlighted as a possible candidate particle because of its high refractive index, but its impact on stratospheric chemistry via heterogeneous reactions is as yet unknown. In this work the heterogeneous reaction of airborne sub-micrometre TiO2 particles with N2O5 has been investigated for the first time, at room temperature and different relative humidities (RH), using an atmospheric pressure aerosol flow tube. The uptake coefficient of N2O5 onto TiO2, γ(N2O5), was determined to be ~1.0 × 10−3 at low RH, increasing to ~3 × 10−3 at 60% RH. The uptake of N2O5 onto TiO2 is then included in the UKCA chemistry–climate model to assess the impact of this reaction on stratospheric chemistry. While the impact of TiO2 on the scattering of solar radiation is chosen to be similar to the aerosol from the Mt Pinatubo eruption, the impact of TiO2 injection on stratospheric N2O5 is much smaller.

scholarly journals North Atlantic Oscillation response in GeoMIP experiments G6solar and G6sulfur: why detailed modelling is needed for understanding regional implications of solar radiation management

2020 ◽  
Author(s):  
Andy Jones ◽  
Jim M. Haywood ◽  
Anthony C. Jones ◽  
Simone Tilmes ◽  
Ben Kravitz ◽  
...  
Keyword(s):  
Solar Radiation ◽  
North Atlantic Oscillation ◽  
North Atlantic ◽  
Winter Season ◽  
Solar Radiation Management ◽  
Positive Anomaly ◽  
Continental Scale ◽  
Detailed Modelling ◽  
Radiation Management ◽  
The Impact

Abstract. The realisation of the difficulty of limiting global mean temperatures to within 1.5 °C or 2.0 °C above pre-industrial levels stipulated by the 21st Conference of Parties in Paris has led to increased interest in solar radiation management (SRM) techniques. Proposed SRM schemes aim to increase planetary albedo to reflect more sunlight back to space and induce a cooling that acts to partially offset global warming. Under the auspices of the Geoengineering Model Intercomparion Project, we have performed model experiments whereby global temperature under the high forcing SSP5–8.5 scenario is reduced to follow that of the medium forcing SSP2–4.5 scenario. Two different mechanisms to achieve this are employed, the first via a reduction in the solar constant (experiment G6solar) and the second via modelling injections of sulfur dioxide (experiment G6sulfur) which forms sulfate aerosol in the stratosphere. Results from two state-of-the-art coupled Earth system models both show an impact on the North Atlantic Oscillation (NAO) in G6sulfur but not in G6solar. Both models show a persistent positive anomaly in the NAO during the Northern Hemisphere winter season in G6sulfur, suggesting an increase in zonal flow and an increase in North Atlantic storm track activity impacting the Eurasian continent leading to regional warming. These findings are broadly consistent with previous findings on the impact of stratospheric volcanic aerosol on the NAO and emphasise that detailed modelling of geoengineering processes is required if accurate impacts of SRM impacts are to be simulated. Differences remain between the two models in predicting regional changes over the continental USA and Africa, suggesting that more models need to perform such simulations before attempting to draw any conclusions regarding potential continental-scale climate change under SRM.

scholarly journals A new Geoengineering Model Intercomparison Project (GeoMIP) experiment designed for climate and chemistry models

2014 ◽  
Vol 7 (4) ◽  
pp. 5447-5464 ◽  
Author(s):  
S. Tilmes ◽  
M. J. Mills ◽  
U. Niemeier ◽  
H. Schmidt ◽  
A. Robock ◽  
...  
Keyword(s):  
Model Comparison ◽  
Stratospheric Aerosol ◽  
Atmospheric Composition ◽  
Model Intercomparison ◽  
Data Set ◽  
Aerosol Forcing ◽  
Input Dataset ◽  
Intercomparison Project ◽  
Total Burden ◽  
The Impact

Abstract. A new Geoengineering Model Intercomparison Project (GeoMIP) experiment "G4 specified stratospheric aerosols" (short name: G4SSA) is proposed to investigate the impact of stratospheric aerosol geoengineering on atmospheric composition, climate, and the environment. In contrast to the earlier G4 GeoMIP experiment, which requires an emission of sulphur dioxide (SO2) into the model, a prescribed aerosol forcing file is provided to the community, to be consistently applied to future model experiments between 2020 and 2100. This stratospheric aerosol distribution, with a total burden of about 2 Tg S has been derived using the ECHAM5-HAM microphysical model, based on a continuous annual tropical emission of 8 Tg SO2 year−1. A ramp-up of geoengineering in 2020 and a ramp-down in 2070 over a period of two years are included in the distribution, while a background aerosol burden should be used for the last 3 decades of the experiment. The performance of this experiment using climate and chemistry models in a multi-model comparison framework will allow us to better understand the significance of the impact of geoengineering and the abrupt termination after 50 years on climate and composition of the atmosphere in a changing environment. The zonal and monthly mean stratospheric aerosol input dataset is available at https://www2.acd.ucar.edu/gcm/geomip-g4-specified-stratospheric-aerosol-data-set.

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