Determination of interface structure of YBCO/LCMO by a spherical aberration- corrected HRTEM

Author(s):  
Z. L. Zhang ◽  
U. Kaiser ◽  
S. Soltan ◽  
H. -U. Habermeier
2020 ◽  
Vol 6 (37) ◽  
pp. eabb8431
Author(s):  
Sergei Lopatin ◽  
Areej Aljarb ◽  
Vladimir Roddatis ◽  
Tobias Meyer ◽  
Yi Wan ◽  
...  

High-resolution scanning transmission electron microscopy (HR-STEM) with spherical aberration correction enables researchers to peer into two-dimensional (2D) materials and correlate the material properties with those of single atoms. The maximum intensity of corrected electron beam is confined in the area having sub-angstrom size. Meanwhile, the residual threefold astigmatism of the electron probe implies a triangular shape distribution of the intensity, whereas its tails overlap and thus interact with several atomic species simultaneously. The result is the resonant modulation of contrast that interferes the determination of phase transition of 2D materials. Here, we theoretically reveal and experimentally determine the origin of resonant modulation of contrast and its unintended impact on violating the power-law dependence of contrast on coordination modes between transition metal and chalcogenide atoms. The finding illuminates the correlation between atomic contrast, spatially inequivalent chalcogenide orientation, and residual threefold astigmatism on determining the atomic structure of emerging 2D materials.


2014 ◽  
Vol 20 (5) ◽  
pp. 1447-1452 ◽  
Author(s):  
Binghui Ge ◽  
Yumei Wang ◽  
Yunjie Chang ◽  
Yuan Yao

AbstractHigh precision determination of atomic position is necessary for quantitative electron microscopy so that small width of peaks, which represent atoms in structural images, adequate resolution, and sufficiently strong image contrast are needed. The width of peak is usually determined by the point spread (PS) of instruments, but the PS of objects should also be taken into consideration in aberration-corrected transmission electron microscopy when point resolution of a microscope reaches the sub-angstrom scale, and thus the PS of the instrument is comparable with that of the object. In this article, PS is investigated by studying peak width with variation of atomic number, sample thickness, and spherical aberration coefficients in both negative Cs (NCSI) and positive Cs imaging (PCSI) modes by means of dynamical image simulation. Through comparing the peak width with various atomic number, thickness, and values of spherical aberration, NCSI mode is found to be superior to PCSI considering the smaller width.


2009 ◽  
Vol 110 (1) ◽  
pp. 36-42 ◽  
Author(s):  
Koji Kuramochi ◽  
Takashi Yamazaki ◽  
Yasutoshi Kotaka ◽  
Masahiro Ohtsuka ◽  
Iwao Hashimoto ◽  
...  

2013 ◽  
Vol 69 (3) ◽  
pp. 289-296 ◽  
Author(s):  
Masahiro Ohtsuka ◽  
Takashi Yamazaki ◽  
Yasutoshi Kotaka ◽  
Hironori Fujisawa ◽  
Masaru Shimizu ◽  
...  

2010 ◽  
Vol 91 (3) ◽  
pp. 36001 ◽  
Author(s):  
M. J. Casanove ◽  
N. Combe ◽  
F. Houdellier ◽  
M. J. Hÿtch

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