scholarly journals Phase-matched enhancements of high-harmonic soft X-rays by adaptive wave-front control with a genetic algorithm

2004 ◽  
Vol 78 (3-4) ◽  
pp. 275-280 ◽  
Author(s):  
D. Yoshitomi ◽  
J. Nees ◽  
N. Miyamoto ◽  
T. Sekikawa ◽  
T. Kanai ◽  
...  
Author(s):  
Romain Geneaux ◽  
Hugo J. B. Marroux ◽  
Alexander Guggenmos ◽  
Daniel M. Neumark ◽  
Stephen R. Leone

Attosecond science opened the door to observing nuclear and electronic dynamics in real time and has begun to expand beyond its traditional grounds. Among several spectroscopic techniques, X-ray transient absorption spectroscopy has become key in understanding matter on ultrafast time scales. In this review, we illustrate the capabilities of this unique tool through a number of iconic experiments. We outline how coherent broadband X-ray radiation, emitted in high-harmonic generation, can be used to follow dynamics in increasingly complex systems. Experiments performed in both molecules and solids are discussed at length, on time scales ranging from attoseconds to picoseconds, and in perturbative or strong-field excitation regimes. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.


Instruments ◽  
2019 ◽  
Vol 3 (3) ◽  
pp. 47 ◽  
Author(s):  
Vittoria Petrillo ◽  
Michele Opromolla ◽  
Alberto Bacci ◽  
Illya Drebot ◽  
Giacomo Ghiringhelli ◽  
...  

Fine time-resolved analysis of matter—i.e., spectroscopy and photon scattering—in the linear response regime requires fs-scale pulsed, high repetition rate, fully coherent X-ray sources. A seeded Free Electron Laser (FEL) driven by a Linac based on Super Conducting cavities, generating 10 8 – 10 10 coherent photons at 2–5 keV with 0.2–1 MHz of repetition rate, can address this need. Three different seeding schemes, reaching the X-ray range, are described hereafter. The first two are multi-stage cascades upshifting the radiation frequency by a factor of 10–30 starting from a seed represented by a coherent flash of extreme ultraviolet light. This radiation can be provided either by the High Harmonic Generation of an optical laser or by an FEL Oscillator operating at 12–14 nm. The third scheme is a regenerative amplifier working with X-ray mirrors. The whole chain of the X-ray generation is here described by means of start-to-end simulations.


Author(s):  
Allan S. Johnson ◽  
Timur Avni ◽  
Esben W. Larsen ◽  
Dane R. Austin ◽  
Jon P. Marangos

High harmonic generation (HHG) of an intense laser pulse is a highly nonlinear optical phenomenon that provides the only proven source of tabletop attosecond pulses, and it is the key technology in attosecond science. Recent developments in high-intensity infrared lasers have extended HHG beyond its traditional domain of the XUV spectral range (10–150 eV) into the soft X-ray regime (150 eV to 3 keV), allowing the compactness, stability and sub-femtosecond duration of HHG to be combined with the atomic site specificity and electronic/structural sensitivity of X-ray spectroscopy. HHG in the soft X-ray spectral region has significant differences from HHG in the XUV, which necessitate new approaches to generating and characterizing attosecond pulses. Here, we examine the challenges and opportunities of soft X-ray HHG, and we use simulations to examine the optimal generating conditions for the development of high-flux, attosecond-duration pulses in the soft X-ray spectral range. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.


2006 ◽  
Vol 26 (3-4) ◽  
pp. 335-342
Author(s):  
Constance Valentin ◽  
Olga Boyko ◽  
Evaggelos Papalazarou ◽  
Gilles Rey ◽  
Brigitte Mercier ◽  
...  

2020 ◽  
Vol 59 (5) ◽  
pp. 1363
Author(s):  
Thomas Wodzinski ◽  
Swen Künzel ◽  
Jayanath C. P. Koliyadu ◽  
Mukhtar Hussain ◽  
Barbara Keitel ◽  
...  

Author(s):  
M.-C. Chen ◽  
P. Arpin ◽  
T. Popmintchev ◽  
M. R. Gerrity ◽  
M. Seaberg ◽  
...  
Keyword(s):  

2000 ◽  
Vol 85 (24) ◽  
pp. 5218-5221 ◽  
Author(s):  
Ofir E. Alon ◽  
Vitali Averbukh ◽  
Nimrod Moiseyev

2018 ◽  
Vol 51 (17) ◽  
pp. 174004 ◽  
Author(s):  
V Cardin ◽  
B E Schimdt ◽  
N Thiré ◽  
S Beaulieu ◽  
V Wanie ◽  
...  

Author(s):  
J. P. Marangos

In this theme issue, leading researchers discuss recent work on the measurement of ultrafast electronic and structural dynamics in matter using a new generation of short duration X-ray photon sources. These photon sources, based upon high harmonic generation from lasers and X-ray free-electron lasers, look set to have a high impact on ultrafast science. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.


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