scholarly journals Perspective - the need and prospects for negative emission technologies - direct air capture through the lens of current sorption process development

2021 ◽  
Vol 38 (12) ◽  
pp. 2375-2380
Author(s):  
Matthew J. Realff ◽  
Youn Ji Min ◽  
Christopher W. Jones ◽  
Ryan P. Lively
2020 ◽  
Author(s):  
Radu Custelcean ◽  
Kathleen A. Garrabrant ◽  
Pierrick Agullo ◽  
Neil J. Williams

Negative emission technologies, including direct air capture (DAC) of carbon dioxide, are now considered essential for mitigating climate change, but existing DAC processes tend to have excessively high energy requirements, mostly associated with sorbent regeneration. Here we demonstrate a new approach to DAC that combines atmospheric CO<sub>2</sub> absorption by an aqueous oligopeptide (i.e., glycylglycine) with bicarbonate crystallization by a simple guanidine compound (i.e., glyoxal-bis-iminoguanidine). In this phase-changing system, the peptide and the guanidine compounds work in synergy, and the cyclic CO<sub>2</sub> capacity can be maximized by matching the p<i>K</i><sub>a</sub> values of the two components. The resulting DAC process has a significantly lower regeneration energy compared to state-of-the-art solvent-based DAC technologies.


2020 ◽  
Author(s):  
Radu Custelcean ◽  
Kathleen A. Garrabrant ◽  
Pierrick Agullo ◽  
Neil J. Williams

Negative emission technologies, including direct air capture (DAC) of carbon dioxide, are now considered essential for mitigating climate change, but existing DAC processes tend to have excessively high energy requirements, mostly associated with sorbent regeneration. Here we demonstrate a new approach to DAC that combines atmospheric CO<sub>2</sub> absorption by an aqueous oligopeptide (i.e., glycylglycine) with bicarbonate crystallization by a simple guanidine compound (i.e., glyoxal-bis-iminoguanidine). In this phase-changing system, the peptide and the guanidine compounds work in synergy, and the cyclic CO<sub>2</sub> capacity can be maximized by matching the p<i>K</i><sub>a</sub> values of the two components. The resulting DAC process has a significantly lower regeneration energy compared to state-of-the-art solvent-based DAC technologies.


2018 ◽  
Vol 6 (10) ◽  
pp. 1380-1384 ◽  
Author(s):  
Jan Wohland ◽  
Dirk Witthaut ◽  
Carl-Friedrich Schleussner

2021 ◽  
Vol 46 ◽  
pp. 101487
Author(s):  
Marco Marchese ◽  
Giulio Buffo ◽  
Massimo Santarelli ◽  
Andrea Lanzini

2019 ◽  
Vol 10 (1) ◽  
Author(s):  
Giulia Realmonte ◽  
Laurent Drouet ◽  
Ajay Gambhir ◽  
James Glynn ◽  
Adam Hawkes ◽  
...  

Joule ◽  
2021 ◽  
Author(s):  
Francesco Sabatino ◽  
Alexa Grimm ◽  
Fausto Gallucci ◽  
Martin van Sint Annaland ◽  
Gert Jan Kramer ◽  
...  

2021 ◽  
Vol 167 (3-4) ◽  
Author(s):  
Ariane Wenger ◽  
Michael Stauffacher ◽  
Irina Dallo

AbstractLimiting global warming to 1.5 °C requires negative emission technologies (NETs), which remove carbon dioxide from the atmosphere and permanently store it to offset unavoidable emissions. Successful large-scale deployment of NETs depends not only on technical, biophysical, ecological, and economic factors, but also on public perception and acceptance. However, previous studies on this topic have been scarce. In 2019, Switzerland adopted a net zero greenhouse gas emissions by 2050 target, which will require the use of NETs. To examine the current Swiss public perception and acceptance of five different NETs, we conducted an online survey with Swiss citizens (N = 693). By using a between-subjects design, we investigated differences in public opinion, perception, and acceptance across three of the most used frames in the scientific literature — technological fix, moral hazard, and climate emergency. Results showed that the public perception and acceptance of NETs does not differ between the frames. The technological fix frame best reflected participants’ opinion, whereas participants perceived the moral hazard frame the least credible and the climate emergency frame the most unclear. Moreover, our findings confirm the public’s unfamiliarity with NETs. We found no strong opposition, as participants indicated a moderate acceptance and a neutral evaluation of all five NETs, with afforestation standing out as the most accepted and positively evaluated NET. We conclude that, in the future, the public debate on NETs should be intensified, and the public perception should be monitored regularly to inform the development of NETs.


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