Two-dimensional MnFeCo layered double oxide as catalyst for enhanced selective catalytic reduction of NOx with NH3 at low temperature (25–150 °C)

2020 ◽  
Vol 592 ◽  
pp. 117432 ◽  
Author(s):  
Xia Zhou ◽  
Feng Yu ◽  
Ruobing Sun ◽  
Junqi Tian ◽  
Qiang Wang ◽  
...  
Nanomaterials ◽  
2018 ◽  
Vol 8 (8) ◽  
pp. 620 ◽  
Author(s):  
Dan Zhao ◽  
Chao Wang ◽  
Feng Yu ◽  
Yulin Shi ◽  
Peng Cao ◽  
...  

A two-dimensional MnAl-layered double oxide (LDO) was obtained by flash nanoprecipitation method (FNP) and used for the selective catalytic reduction of NOx with NH3. The MnAl-LDO (FNP) catalyst formed a particle size of 114.9 nm. Further characterization exhibited rich oxygen vacancies and strong redox property to promote the catalytic activity at low temperature. The MnAl-LDO (FNP) catalyst performed excellent NO conversion above 80% at the temperature range of 100–400 °C, and N2 selectivity above 90% below 200 °C, with a gas hourly space velocity (GHSV) of 60,000 h−1, and a NO concentration of 500 ppm. The maximum NO conversion is 100% at 200 °C; when the temperature in 150–250 °C, the NO conversion can also reach 95%. The remarkable low-temperature catalytic performance of the MnAl-LDO (FNP) catalyst presented potential applications for controlling NO emissions on the account of the presentation of oxygen vacancies.


2018 ◽  
Vol 33 (21) ◽  
pp. 3559-3569 ◽  
Author(s):  
Xiaoyan Huang ◽  
Aijuan Xie ◽  
Jiayi Wu ◽  
Linjing Xu ◽  
Shiping Luo ◽  
...  

Abstract


2017 ◽  
Vol 41 (19) ◽  
pp. 11299-11307 ◽  
Author(s):  
Rong Liu ◽  
Yifan Xu ◽  
Fei Ye ◽  
Feng Jia ◽  
Rui Xu

Mn–Ce based catalysts supported on Ti-bearing blast furnace slag (industrial solid waste) and the doping of transition metals were studied.


RSC Advances ◽  
2017 ◽  
Vol 7 (42) ◽  
pp. 26226-26242 ◽  
Author(s):  
Shengen Zhang ◽  
Bolin Zhang ◽  
Bo Liu ◽  
Shuailing Sun

The reactions over Mn-containing selective catalytic reduction (SCR) catalysts.


2021 ◽  
Vol 11 (19) ◽  
pp. 6553-6563
Author(s):  
Hao Fan ◽  
Jie Fan ◽  
Tian Chang ◽  
Xiuru Wang ◽  
Xin Wang ◽  
...  

Fe improved the reducibility of Mn sites and reduced the oxidizing properties of bridging oxygen.


2020 ◽  
Vol 10 (10) ◽  
pp. 3450-3457
Author(s):  
Kang Zheng ◽  
Zhiyuan Zhou ◽  
Yongzhao Wang ◽  
Zhiling Xin ◽  
Zhiliang Zhao ◽  
...  

We report a facile method for dispersing Mn species onto two-dimensional Co3O4 nanosheets at the nanoscale for the selective catalytic reduction (SCR) of NOx with NH3.


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