Long-term trend of wintertime precipitation chemistry at a remote islet site influenced by anthropogenic emissions from continental East Asia

2021 ◽  
pp. 118626
Author(s):  
Linh Thi Thuy Do ◽  
Stephen M. Griffith ◽  
Wei-Ti Tseng ◽  
Neng-Huei Lin
2010 ◽  
Vol 10 (16) ◽  
pp. 7739-7751 ◽  
Author(s):  
M. Gloor ◽  
J. L. Sarmiento ◽  
N. Gruber

Abstract. The ratio of CO2 accumulating in the atmosphere to the CO2 flux into the atmosphere due to human activity, the airborne fraction AF, is central to predict changes in earth's surface temperature due to greenhouse gas induced warming. This ratio has remained remarkably constant in the past five decades, but recent studies have reported an apparent increasing trend and interpreted it as an indication for a decrease in the efficiency of the combined sinks by the ocean and terrestrial biosphere. We investigate here whether this interpretation is correct by analyzing the processes that control long-term trends and decadal-scale variations in the AF. To this end, we use simplified linear models for describing the time evolution of an atmospheric CO2 perturbation. We find firstly that the spin-up time of the system for the AF to converge to a constant value is on the order of 200–300 years and differs depending on whether exponentially increasing fossil fuel emissions only or the sum of fossil fuel and land use emissions are used. We find secondly that the primary control on the decadal time-scale variations of the AF is variations in the relative growth rate of the total anthropogenic CO2 emissions. Changes in sink efficiencies tend to leave a smaller imprint. Therefore, before interpreting trends in the AF as an indication of weakening carbon sink efficiency, it is necessary to account for trends and variations in AF stemming from anthropogenic emissions and other extrinsic forcing events, such as volcanic eruptions. Using atmospheric CO2 data and emission estimates for the period 1959 through 2006, and our simple predictive models for the AF, we find that likely omissions in the reported emissions from land use change and extrinsic forcing events are sufficient to explain the observed long-term trend in AF. Therefore, claims for a decreasing long-term trend in the carbon sink efficiency over the last few decades are currently not supported by atmospheric CO2 data and anthropogenic emissions estimates.


2018 ◽  
Vol 25 (2) ◽  
pp. 198-220 ◽  
Author(s):  
David C. Kang

What has been the impact of Donald J. Trump’s presidency on the place of the United States in East Asia? Trump already has shown a proclivity for upending the mainstream American consensus about grand strategy to East Asia, with the real possibility of a trade war with China or a shooting war with North Korea on the horizon. However, this article will place President Trump’s first year in office into a larger context of long-term decline of U.S. leadership and influence in East Asia, arguing that this trend has been underway for quite some time, and that Trump has not altered fundamentally this trajectory. Some of Trump’s actions may accelerate a decline in U.S. leadership, but by no means was Trump the first nor will he be the last U.S. president to deal with a swiftly changing East Asia. The region has been changing rapidly for decades, and there are no indications that this will stop anytime soon. However, continuing and gradual U.S. withdrawal from leadership does not mean less American-East Asia interaction. East Asia will remain the most important trading and investment region for the U.S. for the foreseeable future.


2015 ◽  
Vol 120 (17) ◽  
pp. 8658-8670 ◽  
Author(s):  
Shanjun Cheng ◽  
Xiaodan Guan ◽  
Jianping Huang ◽  
Fei Ji ◽  
Ruixia Guo

2020 ◽  
Author(s):  
Man Yue ◽  
Minghuai Wang

<p>Abstract: Planetary boundary layer (PBL) plays an important role in climate and air quality simulations. Large uncertainties remain in understanding the long-term trend of PBL height (PBLH). In this study, radiosonde data and ERA-Interim reanalysis data are applied to reveal the critical climate factors and mechanisms dominating the long-term trend of PBLH over East Asia. Our results show that, observed long-term shift in PBLH trend is found to be consistent with changes in sensible heat flux (SHFLX), net downward surface shortwave flux (SWFLX) and low cloud cover (LCC). Increases in soil moisture and LCC in recent years can modulate the energy partition through the SHFLX and modifying the surface radiation budget, and further lead to the long-term shift trend of PBLH. Long-term trend of PBLH over East Asia is further examined in climate models (including NCAR CESM2) and data from the Coupled Model Inter-comparison Project Phase 6 (CMIP6) experiments. The global climate models are not able to reproduce the long-term trend of PBLH over East Asia. CESM2 is shown to not catch the long-term variability of sensible heat flux and surface shortwave flux. Further analysis is performed to examine how the trend of mean PBLH and extreme low PBLH may be different.</p>


2011 ◽  
Vol 11 (16) ◽  
pp. 8745-8758 ◽  
Author(s):  
S. Chatani ◽  
K. Sudo

Abstract. Air quality simulations in which the global chemical transport model CHASER and the regional chemical transport model WRF/chem are coupled have been developed to consider the dynamic transport of chemical species across the boundaries of the domain of the regional chemical transport model. The simulation captures the overall seasonal variations of surface ozone, but overestimates its concentration over Japanese populated areas by approximately 20 ppb from summer to early winter. It is deduced that ozone formation around Northeast China and Japan in summer is overestimated in the simulation. On the other hand, the simulation well reproduces the interannual variability and the long-term trend of observed surface ozone over Japan. Sensitivity experiments have been performed to investigate the influence of the variation in inflow to East Asia on the interannual variability and the long-term trend of surface ozone over Japan during 1996–2005. The inflow defined in this paper includes the recirculation of species with sources within the East Asian region as well as the transport of species with sources out of the East Asian region. Results of sensitivity experiments suggest that inflow to East Asia accounts for approximately 30 % of the increasing trend of surface ozone, whereas it has much less influence on the interannual variability of observed surface ozone compared to meteorological processes within East Asia.


2010 ◽  
Vol 10 (12) ◽  
pp. 30823-30856
Author(s):  
S. Chatani ◽  
K. Sudo

Abstract. Air quality simulation in which global and regional chemical transport models are coupled has been developed to investigate the influence of the variation in inflow to East Asia on the interannual variability and the long-term trend of surface ozone over Japan during 1996–2005. The simulation overestimates the concentration of surface ozone from summer to early winter. It is deduced that ozone formation around Northeast China is overestimated in the simulation. On the other hand, the simulation reproduces the interannual variability and the long-term trend of observed surface ozone over Japan well. Results of sensitivity experiments suggest that inflow to East Asia accounts for approximately 30% of the increasing trend of surface ozone, whereas it has much less influence on the interannual variability of observed surface ozone compared to meteorological processes within East Asia.


2019 ◽  
Vol 54 (1-2) ◽  
pp. 1131-1144 ◽  
Author(s):  
Jaeyeon Lee ◽  
Seok-Woo Son ◽  
Hyeong-Oh Cho ◽  
Junsu Kim ◽  
Dong-Hyun Cha ◽  
...  

2018 ◽  
Vol 9 (2) ◽  
pp. 157-169
Author(s):  
Sang-Wook Kim ◽  
Kanghyun Song ◽  
Young-Eun Yoo ◽  
Seok-Woo Son ◽  
Su-Jong Jeong

2008 ◽  
Vol 42 (13) ◽  
pp. 3156-3165 ◽  
Author(s):  
X WANG ◽  
J HUANG ◽  
M JI ◽  
K HIGUCHI

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