scholarly journals Time-Resolved Photoelectron Spectroscopy of Conical Intersections with Attosecond Pulse Trains

Author(s):  
Deependra Jadoun ◽  
Markus Kowalewski
2021 ◽  
Vol 12 (1) ◽  
Author(s):  
S. Heinrich ◽  
T. Saule ◽  
M. Högner ◽  
Y. Cui ◽  
V. S. Yakovlev ◽  
...  

AbstractTime-resolved photoelectron spectroscopy with attosecond precision provides new insights into the photoelectric effect and gives information about the timing of photoemission from different electronic states within the electronic band structure of solids. Electron transport, scattering phenomena and electron-electron correlation effects can be observed on attosecond time scales by timing photoemission from valence band states against that from core states. However, accessing intraband effects was so far particularly challenging due to the simultaneous requirements on energy, momentum and time resolution. Here we report on an experiment utilizing intracavity generated attosecond pulse trains to meet these demands at high flux and high photon energies to measure intraband delays between sp- and d-band states in the valence band photoemission from tungsten and investigate final-state effects in resonant photoemission.


2019 ◽  
Vol 21 (26) ◽  
pp. 13902-13905 ◽  
Author(s):  
Shunsuke Adachi ◽  
Tom Schatteburg ◽  
Alexander Humeniuk ◽  
Roland Mitrić ◽  
Toshinori Suzuki

Time-resolved photoelectron spectroscopy using vacuum-UV probe pulses enables observing ultrafast dynamics during and after passing through conical intersections.


2011 ◽  
Vol 115 (16) ◽  
pp. 3755-3765 ◽  
Author(s):  
Roland Mitrić ◽  
Jens Petersen ◽  
Matthias Wohlgemuth ◽  
Ute Werner ◽  
Vlasta Bonačić-Koutecký ◽  
...  

2001 ◽  
Vol 114 (6) ◽  
pp. 2519-2522 ◽  
Author(s):  
S. Lochbrunner ◽  
T. Schultz ◽  
M. Schmitt ◽  
J. P. Shaffer ◽  
M. Z. Zgierski ◽  
...  

2015 ◽  
Vol 17 (47) ◽  
pp. 31978-31987 ◽  
Author(s):  
Franziska Buchner ◽  
Berit Heggen ◽  
Hans-Hermann Ritze ◽  
Walter Thiel ◽  
Andrea Lübcke

Time-resolved photoelectron spectroscopy is performed on aqueous guanosine solution to study its excited-state relaxation dynamics.


2012 ◽  
Vol 37 (12) ◽  
pp. 2211 ◽  
Author(s):  
Shaohao Chen ◽  
Kenneth J. Schafer ◽  
Mette B. Gaarde

Sign in / Sign up

Export Citation Format

Share Document