Seasonal variations of the transport of black carbon and carbon monoxide from the Asian continent to the western Pacific in the boundary layer

2011 ◽  
Vol 116 (D21) ◽  
Author(s):  
R. L. Verma ◽  
Y. Kondo ◽  
N. Oshima ◽  
H. Matsui ◽  
K. Kita ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Carbon Monoxide ◽  
Black Carbon ◽  
Seasonal Variations ◽  
Western Pacific ◽  
Asian Continent ◽  
The Western Pacific

scholarly journals Surface fluxes of bromoform and dibromomethane over the tropical western Pacific inferred from airborne in situ measurements

2017 ◽  
Author(s):  
Liang Feng ◽  
Paul I. Palmer ◽  
Robyn Butler ◽  
Stephen J. Andrews ◽  
Elliot L. Atlas ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Atmospheric Chemistry ◽  
Marine Boundary Layer ◽  
Current Knowledge ◽  
A Priori ◽  
Surface Fluxes ◽  
Western Pacific ◽  
Study Region ◽  
The Western Pacific ◽  
Aircraft Data

Abstract. We infer surface fluxes of bromoform (CHBr3) and dibromoform (CH2Br2) from aircraft observations over the western Pacific using a tagged version of the GEOS-Chem global 3-D atmospheric chemistry model and a Maximum A Posteriori inverse model. The distribution of a priori ocean emissions of these gases are reasonably consistent with observed atmospheric mole fractions of CHBr3 (r = 0.62) and CH2Br2 (r = 0.38). These a priori emissions result in a positive model bias in CHBr3 peaking in the marine boundary layer, but capture observed values of CH2Br2 with no significant bias by virtue of its longer atmospheric lifetime. Using GEOS-Chem, we find that observed variations in atmospheric CHBr3 are determined equally by sources over the western Pacific and those outside the study region, but observed variations in CH2Br2 are determined mainly by sources outside the western Pacific. Numerical closed-loop experiments show that the spatial and temporal distribution of boundary layer aircraft data have the potential to substantially improve current knowledge of these fluxes, with improvements related to data density. Using the aircraft data, we estimate aggregated regional fluxes of 3.6 ± 0.3 × 108 g/month and 0.7 ± 0.1 × 108 g/month for CHBr3 and CH2Br2 over 130°–155° E and 0°–12° N, respectively, which represent reductions of 20–40 % and substantial spatial deviations from the a priori inventory. We find no evidence to support a robust linear relationship between CHBr3 and CH2Br2 oceanic emissions, as used by previous studies.

scholarly journals Surface fluxes of bromoform and dibromomethane over the tropical western Pacific inferred from airborne in situ measurements

2018 ◽  
Vol 18 (20) ◽  
pp. 14787-14798
Author(s):  
Liang Feng ◽  
Paul I. Palmer ◽  
Robyn Butler ◽  
Stephen J. Andrews ◽  
Elliot L. Atlas ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Atmospheric Chemistry ◽  
Current Knowledge ◽  
A Priori ◽  
Surface Fluxes ◽  
Western Pacific ◽  
A Posteriori ◽  
Study Region ◽  
The Western Pacific ◽  
Aircraft Data

Abstract. We infer surface fluxes of bromoform (CHBr3) and dibromoform (CH2Br2) from aircraft observations over the western Pacific using a tagged version of the GEOS-Chem global 3-D atmospheric chemistry model and a maximum a posteriori inverse model. Using GEOS-Chem (GC) as an intermediary, we find that the distribution of a priori ocean emissions of these gases are reasonably consistent with observed atmospheric mole fractions of CHBr3 (r=0.62) and CH2Br2 (r=0.38). These a priori emissions result in a positive model bias in CHBr3 peaking in the marine boundary layer, but reproduce observed values of CH2Br2 with no significant bias by virtue of its longer atmospheric lifetime. Using GEOS-Chem, we find that observed variations in atmospheric CHBr3 are determined equally by sources over the western Pacific and those outside the study region, but observed variations in CH2Br2 are determined mainly by sources outside the western Pacific. Numerical closed-loop experiments show that the spatial and temporal distribution of boundary layer aircraft data have the potential to substantially improve current knowledge of these fluxes, with improvements related to data density. Using the aircraft data, we estimate aggregated regional fluxes of 3.6±0.3×108 and 0.7±0.1×108 g month−1 for CHBr3 and CH2Br2 over 130–155∘E and 0–12∘ N, respectively, which represent reductions of 20 %–40 % of the prior inventories by Ordóñez et al. (2012) and substantial spatial deviations from different a priori inventories. We find no evidence to support a robust linear relationship between CHBr3 and CH2Br2 oceanic emissions, as used by previous studies. We find that over regions with dense observation coverage, our choice of a priori inventory does not significantly impact our reported a posteriori flux estimates.

scholarly journals Observed Evolution of Northward-Propagating Intraseasonal Variation over the Western Pacific: A Case Study in Boreal Early Summer

2013 ◽  
Vol 141 (2) ◽  
pp. 690-706 ◽  
Author(s):  
Masaki Katsumata ◽  
Hiroyuki Yamada ◽  
Hisayuki Kubota ◽  
Qoosaku Moteki ◽  
Ryuichi Shirooka
Keyword(s):  
Boundary Layer ◽  
Large Scale ◽  
Lower Troposphere ◽  
Western Pacific ◽  
Boreal Summer ◽  
Intraseasonal Variation ◽  
Middle Troposphere ◽  
Inactive Period ◽  
The Western Pacific

Abstract This report describes the in situ observed evolution of the atmospheric profile during an event of the boreal summer intraseasonal variation (BSISV) in the tropical western Pacific Ocean. The convectively active region of the BSISV proceeded northward over the sounding and radar network. Over the array, the situation changed from a convectively inactive period to an active period. Inspection of the sounding data revealed the gradual moistening of the lower troposphere during the convectively inactive period. The sounding-derived heat and moisture budget analyses indicated that both the convective- and large-scale processes caused moistening of the lower and middle troposphere where the radar echo tops were observed most frequently. This study is the first to identify such a “preconditioning” process for the BSISV in the western Pacific using detailed in situ observational data. During the preconditioning, an increase in CAPE was observed, as in previous studies of the MJO. An increase of moisture in the boundary layer was responsible for the increase of CAPE. The large-scale horizontal convergence in the boundary layer may be a key factor to moisten the boundary layer through the convective-scale processes, as well as through the large-scale processes to moisten the lower and middle troposphere.

scholarly journals Carbon monoxide in the upper troposphere over the western Pacific between 1993 and 1996

1998 ◽  
Vol 103 (D15) ◽  
pp. 19093-19110 ◽  
Author(s):  
Hidekazu Matsueda ◽  
Hisayuki Y. Inoue ◽  
Yosuke Sawa ◽  
Yukitomo Tsutsumi ◽  
Masao Ishii
Keyword(s):  
Carbon Monoxide ◽  
Western Pacific ◽  
Upper Troposphere ◽  
The Western Pacific

scholarly journals The lofting of Western Pacific regional aerosol by island thermodynamics as observed around Borneo

2012 ◽  
Vol 12 (13) ◽  
pp. 5963-5983 ◽  
Author(s):  
N. H. Robinson ◽  
J. D. Allan ◽  
J. A. Trembath ◽  
P. D. Rosenberg ◽  
G. Allen ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Sea Breeze ◽  
Number Concentration ◽  
Western Pacific ◽  
Surface Mixed Layer ◽  
Free Troposphere ◽  
Mean Flow ◽  
Aerosol Composition ◽  
Air Mass ◽  
The Western Pacific

Abstract. Vertical profiles of aerosol chemical composition, number concentration and size were measured throughout the lower troposphere of Borneo, a large tropical island in the western Pacific Ocean. Aerosol composition, size and number concentration measurements (using an Aerodyne Aerosol Mass Spectrometer, Passive Cavity Aerosol Spectrometer Probe and Condensation Particle Counter, respectively) were made both upwind and downwind of Borneo, as well as over the island itself, on board the UK BAe-146 research aircraft as part of the OP3 project. Two meteorological regimes were identified – one dominated by isolated terrestrial convection (ITC) which peaked in the afternoon, and the other characterised by more regionally active mesoscale convective systems (MCS). Upwind profiles show aerosol to be confined to a shallow marine boundary layer below 930 ± 10 hPa (~760 m above sea level, a.s.l.). As this air mass advects over the island with the mean free troposphere synoptic flow during the ITC-dominated regime, it is convectively lofted above the terrestrial surface mixed layer to heights of between 945 ± 22 (~630 m a.s.l.) and 740 ± 44 hPa (~2740 m a.s.l.), consistent with a coupling between the synoptic steering level flow and island sea breeze circulations. Terrestrial aerosol was observed to be lofted into this higher layer through both moist convective uplift and transport through turbulent diurnal sea-breeze cells. At the peak of convective activity in the mid-afternoons, organic aerosol loadings in the lofted layer were observed to be substantially higher than in the morning (by a mean factor of three). This organic matter is dominated by secondary aerosol from processing of biogenic gas phase precursors. Aerosol number concentration profiles suggest formation of new particles aloft in the atmosphere. By the time the air mass reaches the west coast of the island, terrestrial aerosol is enhanced in the lofted layer. Such uplift of aerosol in Borneo is expected to increase aerosol lifetimes in the lower free troposphere downwind, as they are above the boundary layer and therefore less likely to be lost by wet or dry deposition. It is also likely to change the role they play in the semi-direct and direct aerosol effects. The long chain of islands extending from Malaysia to Australia may all similarly be expected to present an orographic barrier to low level mean flow. This would lead to significant transport of aerosol into the tropical free troposphere across the Western Pacific region.

scholarly journals Airmass Origin in the Arctic. Part I: Seasonality

2015 ◽  
Vol 28 (12) ◽  
pp. 4997-5014 ◽  
Author(s):  
Clara Orbe ◽  
Paul A. Newman ◽  
Darryn W. Waugh ◽  
Mark Holzer ◽  
Luke D. Oman ◽  
...  
Keyword(s):  
Boundary Layer ◽  
North America ◽  
Seasonal Variations ◽  
Large Scale ◽  
Climate Model ◽  
The Arctic ◽  
Boreal Winter ◽  
Earth Observing System ◽  
The Western Pacific ◽  
System Chemistry

Abstract The first climatology of airmass origin in the Arctic is presented in terms of rigorously defined airmass fractions that partition air according to where it last contacted the planetary boundary layer (PBL). Results from a present-day climate integration of the Goddard Earth Observing System Chemistry–Climate Model (GEOSCCM) reveal that the majority of air in the Arctic below 700 mb last contacted the PBL poleward of 60°N. By comparison, 62% (±0.8%) of the air above 700 mb originates over Northern Hemisphere midlatitudes (i.e., “midlatitude air”). Seasonal variations in the airmass fractions above 700 mb reveal that during boreal winter air from midlatitudes originates primarily over the oceans, with 26% (±1.9%) last contacting the PBL over the eastern Pacific, 21% (±0.87%) over the Atlantic, and 16% (±1.2%) over the western Pacific. During summer, by comparison, midlatitude air originates primarily over land, overwhelmingly so over Asia [41% (±1.0%)] and, to a lesser extent, over North America [24% (±1.5%)]. Seasonal variations in the airmass fractions are interpreted in terms of changes in the large-scale ventilation of the midlatitude boundary layer and the midlatitude tropospheric jet.

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