Time-resolved imaging of bound and dissociating nuclear wave packets in strong-field ionized iodomethane

2019 ◽  
Vol 21 (26) ◽  
pp. 14090-14102 ◽  
Author(s):  
Y. Malakar ◽  
W. L. Pearson ◽  
M. Zohrabi ◽  
B. Kaderiya ◽  
Kanaka Raju P. ◽  
...  

We report the results of a time-resolved coincident ion momentum imaging experiment probing nuclear wave packet dynamics in the strong-field ionization and dissociation of iodomethane (CH3I).

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
D. Trabert ◽  
S. Brennecke ◽  
K. Fehre ◽  
N. Anders ◽  
A. Geyer ◽  
...  

AbstractWhen a very strong light field is applied to a molecule an electron can be ejected by tunneling. In order to quantify the time-resolved dynamics of this ionization process, the concept of the Wigner time delay can be used. The properties of this process can depend on the tunneling direction relative to the molecular axis. Here, we show experimental and theoretical data on the Wigner time delay for tunnel ionization of H2 molecules and demonstrate its dependence on the emission direction of the electron with respect to the molecular axis. We find, that the observed changes in the Wigner time delay can be quantitatively explained by elongated/shortened travel paths of the emitted electrons, which occur due to spatial shifts of the electrons’ birth positions after tunneling. Our work provides therefore an intuitive perspective towards the Wigner time delay in strong-field ionization.


2020 ◽  
Vol 102 (4) ◽  
Author(s):  
Huynh Van Sa Lam ◽  
Suresh Yarlagadda ◽  
Anbu Venkatachalam ◽  
Tomthin Nganba Wangjam ◽  
Rajesh K. Kushawaha ◽  
...  

2020 ◽  
Author(s):  
Felix Allum ◽  
Nils Anders ◽  
Mark Brouard ◽  
Phil H. Bucksbaum ◽  
Michael Burt ◽  
...  

The photodissociation dynamics of strong-field ionized methyl iodide (\ce{CH3I}) were probed using intense extreme ultraviolet (XUV) radiation produced by the SPring-8 Angstrom Compact free electron LAser (SACLA). Strong-field ionization and...


2011 ◽  
Vol 106 (7) ◽  
Author(s):  
Jonas L. Hansen ◽  
Henrik Stapelfeldt ◽  
Darko Dimitrovski ◽  
Mahmoud Abu-samha ◽  
Christian P. J. Martiny ◽  
...  

2010 ◽  
Vol 82 (1) ◽  
Author(s):  
Dominik Geißler ◽  
Tamás Rozgonyi ◽  
Jesús González-Vázquez ◽  
Leticia González ◽  
Sarah Nichols ◽  
...  

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