Fischer–Tropsch synthesis over the Fe–Mn/Al2O3 catalyst: modeling and optimization of light olefins using the RSM method

2020 ◽  
Vol 44 (42) ◽  
pp. 18457-18468
Author(s):  
Maryam Arsalanfar
Keyword(s):  
Chemical Properties ◽  
Catalytic Performance ◽  
Tropsch Synthesis ◽  
Light Olefins ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Modeling And Optimization ◽  
Physico Chemical ◽  
Al2o3 Catalyst

The effect of various preparation parameters on the catalytic performance and physico-chemical properties of a supported Fe–Mn catalyst was investigated using the RSM method.

scholarly journals Fischer-Tropsch synthesis over Co/γ-Al2O3 catalyst loaded on ceramic monolith-structured substrate

2020 ◽  
Vol 9 (3) ◽  
pp. 88-93
Author(s):  
Uy Do Pham Noa ◽  
Huan Nguyen Manh ◽  
Loc Hoang Van ◽  
Chien Luc Minh ◽  
Giang Nguyen Thi Chau ◽  
...  
Keyword(s):  
Tubular Reactor ◽  
Chemical Properties ◽  
Tropsch Synthesis ◽  
Impregnation Method ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Physico Chemical ◽  
Bet Specific Surface Area ◽  
Slurry Method ◽  
Al2o3 Catalyst

Cobalt-based catalyst supported on γ-Al2O3­ was prepared by impregnation method and loaded on ceramic monolith-structured substrate by wash-coating slurry method. Physico-chemical properties of the catalysts were characterized by X-ray diffraction (XRD), Brunauer–Emmett–Teller (BET) specific surface area and H2 temperatured-programmed reduction (H2-TPR). Activity of the catalysts for Fischer-Tropsch synthesis was investigated in a tubular reactor in a temperature range of 200-275 oC at 20 bar and GHSV = 3000 h-1. Co/γ-Al2O3 catalyst loaded on ceramic monolith-structured substrate enhanced efficacy of Fischer-Tropsch synthesis by increasing and stabilizing CO conversion and C5+ selectivity, compared to Co/γ-Al2O3 powder catalyst.

Effect of Ba on the catalytic performance of Co-Ru/Al2O3 catalyst for Fischer-Tropsch synthesis

Fuel ◽  
2021 ◽  
Vol 292 ◽  
pp. 120398
Author(s):  
Shupeng Guo ◽  
Zhongyi Ma ◽  
Jungang Wang ◽  
Bo Hou ◽  
Litao Jia ◽  
...  
Keyword(s):  
Catalytic Performance ◽  
Tropsch Synthesis ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Al2o3 Catalyst

scholarly journals Assessment of composition and calcination parameters in Fischer-Tropsch synthesis over Fe–Mn–Ce/γ-Al2O3 nanocatalyst

2021 ◽  
Vol 76 ◽  
pp. 11
Author(s):  
Reza Roknabadi ◽  
Ali Akbar Mirzaei ◽  
Hossein Atashi
Keyword(s):  
Fixed Bed ◽  
Chemical Properties ◽  
Tropsch Synthesis ◽  
Metal Species ◽  
Light Olefins ◽  
Incipient Wetness Impregnation ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Study Results ◽  
And Performance

The effects of nanocatalyst composition and calcination parameters on the performance of the Fe–Mn–Ce ternary nanocatalysts supported on alumina granules in a laboratory fixed bed microreactor have been evaluated. Nanocatalysts were synthesized by incipient wetness impregnation under vacuum method (simultaneous impregnation of metal species). The samples used for hydrogenation of carbon monoxide via Fischer-Tropsch synthesis. The optimum nanocatalyst composition for production of light olefins (C=2 – C=4) from synthesis gas is 75 wt%Fe–20 wt%Mn–5 wt%Ce. The calcination parameters (temperature, time and atmosphere) were investigated and their effects on the structure and performance of the nanocatalysts were determined. The maximum ratio of olefins/(methane + paraffin) and the best activity and selectivity belonged to the nanocatalyst which was calcined in static air at 500 °C for 7 h. The nanocatalyst precursors and calcined samples (fresh and used) were characterized by XRD, N2 physisorption, FE‒SEM, EDAX, MAP, TG, DSC, and H2–TPR. The present study results confirm that the structural, morphological and physic-chemical properties of the nanocatalyst have been impressed with metal species and calcination parameters.

A study on physico-chemical properties and activity of Co-based catalysts supported on SBA-15 in the Fischer-Tropsch synthesis

2013 ◽  
Vol 10 (3/4) ◽  
pp. 313 ◽  
Author(s):  
Luu Cam Loc ◽  
Lac Kien Trieu ◽  
Ho Si Thoang ◽  
Huynh Thi My Trang ◽  
Nguyen Manh Huan ◽  
...  
Keyword(s):  
Chemical Properties ◽  
Tropsch Synthesis ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Physico Chemical

A comprehensive insight into the role of barium in catalytic performance of Co/Al2O3 catalyst for Fischer-Tropsch synthesis

Fuel ◽  
2019 ◽  
Vol 256 ◽  
pp. 115911 ◽  
Author(s):  
Shupeng Guo ◽  
Qiang Wang ◽  
Min Wang ◽  
Zhongyi Ma ◽  
Jungang Wang ◽  
...  
Keyword(s):  
Catalytic Performance ◽  
Tropsch Synthesis ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Al2o3 Catalyst ◽  
Insight Into

scholarly journals Formulation and catalytic performance of MOF-derived Fe@C/Al composites for high temperature Fischer–Tropsch synthesis

2018 ◽  
Vol 8 (1) ◽  
pp. 210-220 ◽  
Author(s):  
Lide Oar-Arteta ◽  
María José Valero-Romero ◽  
Tim Wezendonk ◽  
Freek Kapteijn ◽  
Jorge Gascon
Keyword(s):  
High Temperature ◽  
Mechanical Stability ◽  
Catalytic Performance ◽  
Tropsch Synthesis ◽  
Light Olefins ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis

The synthesis of MOF/AlOOH derived composites enhances the selectivity towards light olefins in HTFTS and the mechanical stability of the catalysts.

Isomorphic titanium-substituted mesoporous SBA-16 as support for cobalt Fischer–Tropsch synthesis catalysts: Balance between dispersion and reduction

2021 ◽  
Author(s):  
Liang Wei ◽  
Jian Chen ◽  
Shuai Lyu ◽  
Chengchao Liu ◽  
Yanxi Zhao ◽  
...  
Keyword(s):  
Catalytic Performance ◽  
Tropsch Synthesis ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Support Interaction ◽  
Delicate Balance ◽  
Metal Support Interaction ◽  
Metal Support ◽  
Synthesis Catalysts

The delicate balance between dispersion and reduction of the Co-based Fischer–Tropsch synthesis catalyst is the golden key to enhancing catalytic performance, which highly depends on an optimized metal–support interaction. In...

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