A General MOF-intermediated synthesis of hollow CoFe-based trimetallic phosphides composed of ultrathin nanosheets for boosting water oxidation electrocatalysis

Nanoscale ◽  
2021 ◽  
Author(s):  
Cheng Wang ◽  
Hongyuan Shang ◽  
Yuan Wang ◽  
Jie Li ◽  
Siyu Guo ◽  
...  
Keyword(s):  
Reaction Kinetics ◽  
Oxygen Evolution ◽  
Electrode Material ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Grand Challenge ◽  
Ultrathin Nanosheets

Engineering an electrode material for boosting reaction kinetics is highly expected for the oxygen evolution reaction (OER) in the anodic half reaction, which is still a grand challenge for energy...

“Pit-dot” ultrathin nanosheets of hydrated copper pyrophosphate as efficient pre-catalysts for robust water oxidation

2021 ◽  
Author(s):  
Junfeng Xie ◽  
Xueying Yang ◽  
Yameng Wang ◽  
Luyao Kang ◽  
Jiechen Li ◽  
...  
Keyword(s):  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Ultrathin Nanosheets

Herein, hydrated copper pyrophosphate ultrathin nanosheets with unique “pit-dot” nanostructure were fabricated as efficient pre-catalysts for oxygen evolution reaction, and systematic post-catalytic characterizations confirmed the important role of the boosted...

Controllable growth of graphdiyne layered nanosheets for high-performance water oxidation

2021 ◽  
Author(s):  
Shuya Zhao ◽  
Yurui Xue ◽  
Zhongqiang Wang ◽  
Zhiqiang Zheng ◽  
Xiaoyu Luan ◽  
...  
Keyword(s):  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
High Performance ◽  
Low Cost ◽  
Highly Active ◽  
Controllable Growth

Developing highly active, stable and low-cost electrocatalysts capable of an efficient oxygen evolution reaction (OER) is urgent and challenging.

Bifunctional citrate-Ni0.9Co0.1(OH)x layer coated fluorine-doped hematite for simultaneous hole extraction and injection towards efficient photoelectrochemical water oxidation

Nanoscale ◽  
2021 ◽  
Author(s):  
Peng Wang ◽  
Feng Li ◽  
Xuefeng Long ◽  
Tong Wang ◽  
Huan Chai ◽  
...  
Keyword(s):  
Surface Modification ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Surface Oxygen ◽  
Co Catalyst ◽  
Photoelectrochemical Water Oxidation

Surface modification by loading a water oxidation co-catalyst (WOC) is generally considered to be an efficient means to optimize the sluggish surface oxygen evolution reaction (OER) of hematite photoanode for...

Oriental and robust anchoring of Fe via anodic interfacial coordination assembly on ultrathin Co hydroxides for efficient water oxidation

Nanoscale ◽  
2021 ◽  
Author(s):  
Ya-Nan Zhou ◽  
Ruo-Yao Fan ◽  
Yu-Ning Cao ◽  
Hui-Ying Wang ◽  
Bin Dong ◽  
...  
Keyword(s):  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Active Sites

The oriental distribution and strong conjunction of Fe active sites in multiple metals hydroxides are very crucial to modulate the activity and stability for efficient oxygen evolution reaction (OER). Whereas,...

scholarly journals Spin-sate reconfiguration induced by alternating magnetic field for efficient oxygen evolution reaction

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Gang Zhou ◽  
Peifang Wang ◽  
Hao Li ◽  
Bin Hu ◽  
Yan Sun ◽  
...  
Keyword(s):  
Reaction Kinetics ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Active Sites ◽  
Reaction Pathway ◽  
Low Cost ◽  
Orbital Interaction ◽  
New Paradigm ◽  
Metal Organic ◽  
Energy Conversion Devices

AbstractOxygen evolution reaction (OER) plays a determining role in electrochemical energy conversion devices, but challenges remain due to the lack of effective low-cost electrocatalysts and insufficient understanding about sluggish reaction kinetics. Distinguish from complex nano-structuring, this work focuses on the spin-related charge transfer and orbital interaction between catalysts and intermediates to accelerate catalytic reaction kinetics. Herein, we propose a simple magnetic-stimulation approach to rearrange spin electron occupation in noble-metal-free metal-organic frameworks (MOFs) with a feature of thermal-differentiated superlattice, in which the localized magnetic heating in periodic spatial distribution makes the spin flip occur at particular active sites, demonstrating a spin-dependent reaction pathway. As a result, the spin-rearranged Co0.8Mn0.2 MOF displays mass activities of 3514.7 A gmetal−1 with an overpotential of ~0.27 V, which is 21.1 times that of pristine MOF. Our findings provide a new paradigm for designing spin electrocatalysis and steering reaction kinetics.

One-step synthesis of multi-walled carbon nanotubes/ultra-thin Ni(OH)2 nanoplate composite as efficient catalysts for water oxidation

2014 ◽  
Vol 2 (30) ◽  
pp. 11799-11806 ◽  
Author(s):  
Xuemei Zhou ◽  
Zhaoming Xia ◽  
Zhiyun Zhang ◽  
Yuanyuan Ma ◽  
Yongquan Qu
Keyword(s):  
Carbon Nanotubes ◽  
Hydrothermal Synthesis ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Highly Efficient ◽  
Multi Walled Carbon Nanotubes ◽  
One Step ◽  
Walled Carbon Nanotubes

One-step hydrothermal synthesis of ultra-thin β-Ni(OH)2 nanoplates (1.5–3.0 nm thickness) and their composite with multi-walled carbon nanotubes in the absence of surfactants function as highly efficient and stable electrocatalysts for oxygen evolution reaction.

scholarly journals Single-atom cobalt-hydroxyl modification of polymeric carbon nitride for highly enhanced photocatalytic water oxidation: ball milling increased single atom loading

2022 ◽  
Author(s):  
Fei Yu ◽  
Tingting Huo ◽  
Quanhua Deng ◽  
Guoan Wang ◽  
Yuguo Xia ◽  
...  
Keyword(s):  
Ball Milling ◽  
Water Splitting ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Carbon Nitride ◽  
Single Atom ◽  
Overall Water Splitting ◽  
Polymeric Carbon

Expediting the oxygen evolution reaction (OER) is the key to achieving efficient photocatalytic overall water splitting. Herein, single-atom Co−OH modified polymeric carbon nitride (Co-PCN) was synthesized with single-atom loading increased...

Ultrathin amorphous cobalt–vanadium hydr(oxy)oxide catalysts for the oxygen evolution reaction

2018 ◽  
Vol 11 (7) ◽  
pp. 1736-1741 ◽  
Author(s):  
Juzhe Liu ◽  
Yongfei Ji ◽  
Jianwei Nai ◽  
Xiaogang Niu ◽  
Yi Luo ◽  
...  
Keyword(s):  
Catalytic Activity ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Oxide Catalysts ◽  
Simple Strategy

A simple strategy to synthesize ultrathin, amorphous and alloyed structural cobalt–vanadium hydr(oxy)oxide catalysts with enhanced water oxidation catalytic activity.

Lattice Oxygen Redox Chemistry in Solid-State Electrocatalysts for Water Oxidation

2021 ◽  
Author(s):  
Ning Zhang ◽  
Yang Chai
Keyword(s):  
Solid State ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Water Electrolysis ◽  
Redox Chemistry ◽  
Lattice Oxygen ◽  
Vital Importance ◽  
Production Of Hydrogen ◽  
Overall Efficiency

Fundamental understandings towards oxygen evolution reaction (OER) are of vital importance as it dominates the overall efficiency of water electrolysis – a compelling technique for sustainable production of hydrogen feedstock....

Promoting the urea oxidation and water oxidation through interface construction on CeO2 @CoFe2O4 heterostructure

2021 ◽  
Author(s):  
Zhixin Dai ◽  
Xiaoqiang Du ◽  
Yanhong Wang ◽  
Xinghua Han ◽  
Xiaoshuang Zhang
Keyword(s):  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
Oxidation Reaction ◽  
Spinel Ferrites

Spinel ferrites are considered as practical and promising oxygen evolution reaction (OER) and urea oxidation reaction (UOR) electrocatalysts because of their advantages in adsorption and activation of electrocatalytic substances. CeO2...

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