scholarly journals The description of the excitation energy sharing in nuclear fission within the Langevin approach

2021 ◽  
Vol 256 ◽  
pp. 00007
Author(s):  
F.A. Ivanyuk ◽  
S. Chiba
Keyword(s):  
Excitation Energy ◽  
Mass Number ◽  
Nuclear Fission ◽  
Deformation Energy ◽  
Langevin Equations ◽  
Excitation Energies ◽  
Tooth Structure ◽  
Fission Fragments ◽  
Langevin Approach ◽  
Energy Sharing

We apply the four-dimensional Langevin approach to the description of fission of 235U by neutrons and calculate the dependence of the excitation energy of fission fragments on their mass number. For this we run the Langevin equations until the compound nucleus splits into two separated fragments. This is possible since the we used in this work two-center shell model shape parametrization that describes well both compact and separated shapes. The excitation energies of each fragment are calculated assuming that the temperatures of both fragments are the same. The deformation energy of the fragment immediately after scission is added to its excitation energy. The saw-tooth structure of the dependence neutron multiplicity on the fragment’s mass number in reaction 235U + n at En = 5 Mev is qualitatively reproduced.

scholarly journals The 4-dimensional Langevin approach to low energy nuclear fission

2018 ◽  
Vol 169 ◽  
pp. 00005
Author(s):  
F.A. Ivanyuk ◽  
C. Ishizuka ◽  
M.D. Usang ◽  
S. Chiba
Keyword(s):  
Excitation Energy ◽  
Mass Number ◽  
Nuclear Fission ◽  
Deformation Energy ◽  
Low Energy ◽  
Tooth Structure ◽  
Fission Fragments ◽  
Langevin Approach ◽  
Intrinsic Excitation ◽  
Mother Nucleus

We applied the four-dimensional Langevin approach to the description of fission of 235U by neutrons and calculated the dependence of the excitation energy of fission fragments on their mass number. For this we have fitted the compact just-before-scission configuration obtained by the Langevin calculations by the two separated fragments and calculated the intrinsic excitation and the deformation energy of each fragment accurately taking into account the shell and pairing effects and their dependence on the temperature and mass of the fragments. For the sharing of energy between the fission fragments we have used the simplest and most reliable assumption - the temperature of each fragment immediately after the neck rupture is the same as the temperature of mother nucleus just before scission. The calculated excitation energy of fission fragments clearly demonstrates the saw-tooth structure in the dependence on fragment mass number.

scholarly journals Impact of nuclear inertia momenta on fission observables

2018 ◽  
Vol 193 ◽  
pp. 01004
Author(s):  
P. Tamagno ◽  
O. Litaize
Keyword(s):  
Rigid Body ◽  
Excitation Energy ◽  
Nuclear Fission ◽  
Particle Model ◽  
Rotational Inertia ◽  
Neutron Fission ◽  
Fission Fragments ◽  
Rigid Body Model ◽  
Two Parameters ◽  
The Impact

Fission is probably the nuclear process the less accurately described with current models because it involves dynamics of nuclear matter with strongly coupled manybody interactions. It is thus diffcult to find models that are strongly rooted in good physics, accurate enough to reproduce target observables and that can describe many of the nuclear fission observables in a consistent way. One of the most comprehensive current modeling of the fission process relies on the fission sampling and Monte-Carlo de-excitation of the fission fragments. This model is implemented for instance in the FIFRELIN code. In this model fission fragments and their state are first sampled from pre-neutron fission yields, angular momentum distribution and excitation energy repartition law then the decay of both initial fragments is simulated. This modeling provides many observables: prompt neutron and gamma fission spectra, multiplicities and also fine decompositions: number of neutrons emitted as a function of the fragment mass, spectra per fragments, etc. This model relies on nuclear structure databases and on several basic nuclear models describing for instance gamma strength functions or level densities. Additionally some free parameters are still to be determined, namely two parameters describing the excitation energy repartition law, the spin cutoff of the heavy and light fragments and a rescaling parameter for the rotational inertia momentum of the fragments with respect of the rigid-body model. In the present work we investigate the impact of this latter parameter. For this we mainly substitute the corrected rigid-body value by a quantity obtained from a microscopic description of the fission fragment. The independent-particle model recently implemented in the CONRAD code is used to provide nucleonic wave functions that are required to compute inertia momenta with an Inglis-Belyaev cranking model. The impact of this substitution is analyzed on different fission observables provided by the FIFRELIN code.

Study of viscosity on the fission dynamics of the excited nuclei 228U produced in 19F + 209Bi reactions

2015 ◽  
Vol 24 (07) ◽  
pp. 1550052 ◽  
Author(s):  
H. Eslamizadeh
Keyword(s):  
Experimental Data ◽  
Symmetry Axis ◽  
Measured Data ◽  
Total Spin ◽  
Langevin Equations ◽  
Two Dimensional ◽  
Excitation Energies ◽  
Fission Fragments ◽  
Excited Nuclei ◽  
Good Agreement

A two-dimensional (2D) dynamical model based on Langevin equations was applied to study the fission dynamics of the compound nuclei 228 U produced in 19 F + 209 Bi reactions at intermediate excitation energies. The distance between the centers of masses of the future fission fragments was used as the first dimension and the projection of the total spin of the compound nucleus onto the symmetry axis, K, was considered as the second dimension in Langevin dynamical calculations. The magnitude of post-saddle friction strength was inferred by fitting measured data on the average pre-scission neutron multiplicity for 228 U . It was shown that the results of calculations are in good agreement with the experimental data by using values of the post-saddle friction equal to 6–8 × 1021 s -1.

scholarly journals Role of the excitation energy of the compound nucleus in binary decay processes

2018 ◽  
Vol 169 ◽  
pp. 00015
Author(s):  
H. Paşca ◽  
A.V. Andreev ◽  
G.G. Adamian ◽  
N.V. Antonenko
Keyword(s):  
Excitation Energy ◽  
Charge Distribution ◽  
Compound Nucleus ◽  
High Excitation ◽  
Point Model ◽  
Excitation Energies ◽  
Scission Point ◽  
Fission Fragments

Employing the improved scission-point model, the isotopic and excitation energy trends of the charge distribution of fission fragments are studied in fission of even-even Th isotopes at low and high excitation energies.

scholarly journals Fission in a microscopic framework: From basic science to support for applications

2021 ◽  
Vol 256 ◽  
pp. 00016
Author(s):  
Ionel Stetcu ◽  
Aurel Bulgac ◽  
Shi Jin ◽  
Kenneth J. Roche ◽  
Nicolas Schunck
Keyword(s):  
Excitation Energy ◽  
Local Density ◽  
Microscopic Theory ◽  
Nuclear Fission ◽  
Many Body ◽  
Time Dynamics ◽  
Recent Developments ◽  
Pairing Field ◽  
Energy Sharing ◽  
Rule Out

Recent developments, both in theoretical modeling and computational power, have allowed us to make progress on a goal not fully achieved yet in nuclear theory: a microscopic theory of nuclear fission. Even if the complete microscopic description remains a computationally demanding task, the information that can be provided by current calculations can be extremely useful to guide and constrain more phenomenological approaches, which are simpler to implement. First, a microscopic model that describes the real-time dynamics of the fissioning system can justify or rule out some of the approximations. Second, the microscopic approach can be used to obtain trends, e.g., with increasing excitation energy of the fissioning system, or even to compute observables that cannot be otherwise calculated in phenomenological approaches or that can be hindered by the limitations of the method. We briefly present in this contribution the time-dependent superfluid local density approximation (TDSLDA) approach to nuclear fission, approach that has become a very successful theoretical model in many areas of many-body research. The TDSLDA incorporates the effects of the continuum, the dynamics of the pairing field, and the numerical solution is implemented with controlled approximations and negligible numerical errors. The main part of the current contribution will be dedicated to discussing the method, and recent results concerning the fission dynamics. In addition, we present results on the excitation energy sharing between the fragments, which are in agreement with a qualitative conclusions extracted from a limited number of experimental measurements of properties of prompt neutrons.

Modification of HAM/3 excitation energies for ΠΠ* transitions of linear molecules

1980 ◽  
Vol 58 (16) ◽  
pp. 1687-1690 ◽  
Author(s):  
Delano P. Chong
Keyword(s):  
Excitation Energy ◽  
Explicit Expression ◽  
Excited States ◽  
Configuration Interaction ◽  
Excitation Energies ◽  
Carbon Suboxide ◽  
Numerical Examples ◽  
Energy Correction ◽  
Linear Molecules ◽  
Configuration Interaction Calculations

The excitation energies calculated by the HAM/3 procedure for ΠΠ* transitions in linear molecules can be internally inconsistent by as much as ± 0.6 eV. In the recent study by Åsbrink etal., the problem was avoided by adopting Recknagel's expressions and requiring the proper average ΠΠ* excitation energy. In this paper, we trace the small inconsistency back to its origin in HAM/3 theory and derive the analytical expression for the energy correction as well as Recknagel's formulas. Numerical examples studied include all seven linear molecules investigated by Åsbrink etal. The explicit expression for the correction enables us to perform meaningful configuration-interaction calculations on the excited states, as illustrated by the carbon suboxide molecule.

The excitation energy of fragments in nuclear fission

Atomic Energy ◽  
1960 ◽  
Vol 6 (3) ◽  
pp. 184-189
Author(s):  
B. T. Geilikman
Keyword(s):  
Excitation Energy ◽  
Nuclear Fission

scholarly journals Predicting the UV–vis spectra of oxazine dyes

2011 ◽  
Vol 7 ◽  
pp. 432-441 ◽  
Author(s):  
Scott Fleming ◽  
Andrew Mills ◽  
Tell Tuttle
Keyword(s):  
Excitation Energy ◽  
Density Functional ◽  
Polarizable Continuum Model ◽  
Implicit Solvent ◽  
Continuum Approach ◽  
Excitation Energies ◽  
Functional Theory ◽  
Partial Charges ◽  
Td Dft ◽  
Polarizable Continuum

In the current work we have investigated the ability of time-dependent density functional theory (TD-DFT) to predict the absorption spectra of a series of oxazine dyes and the effect of solvent on the accuracy of these predictions. Based on the results of this study, it is clear that for the series of oxazine dyes an accurate prediction of the excitation energy requires the inclusion of solvent. Implicit solvent included via a polarizable continuum approach was found to be sufficient in reproducing the excitation energies accurately in the majority of cases. Moreover, we found that the SMD solvent model, which is dependent on the full electron density of the solute without partitioning into partial charges, gave more reliable results for our systems relative to the conductor-like polarizable continuum model (CPCM), as implemented in Gaussian 09. In all cases the inclusion of solvent reduces the error in the predicted excitation energy to <0.3 eV and in the majority of cases to <0.1 eV.

scholarly journals A New Benchmark Set for Excitation Energy of Charge Transfer States: Systematic Investigation of Coupled-Cluster Type Methods

2020 ◽  
Author(s):  
Balázs Kozma ◽  
Attila Tajti ◽  
Baptiste Demoulin ◽  
Róbert Izsák ◽  
Marcel Nooijen ◽  
...  
Keyword(s):  
Charge Transfer ◽  
Excitation Energy ◽  
Systematic Investigation ◽  
Coupled Cluster ◽  
Excitation Energies ◽  
Chemical Methods ◽  
Valence States ◽  
Quantum Chemical Methods ◽  
Material Physics ◽  
Cluster Methods

There are numerous publications on benchmarking quantum chemistry methods for excited states. These studies rarely include Charge Transfer (CT) states although many interesting phenomena in e.g. biochemistry and material physics involve transfer of electron between fragments of the system. Therefore, it is timely to test the accuracy of quantum chemical methods for CT states, as well. In this study we first suggest a set benchmark systems consisting of dimers having low-energy CT states. On this set, the excitation energy has been calculated with coupled cluster methods including triple excitations (CC3, CCSDT-3, CCSD(T)(a)* ), as well as with methods including full or approximate doubles (CCSD, STEOM-CCSD, CC2, ADC(2), EOM-CCSD(2)). The results show that the popular CC2 and ADC(2) methods are much more inaccurate for CT states than for valence states. On the other hand, CCSD seems to have similar systematic overestimation of the excitation energies for both valence and CT states. Concerning triples methods, the new CCSD(T)(a)* method including non-iterative triple excitations preforms very well for all type of states, delivering essentially CCSDT quality results.<br>

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