scholarly journals Moiré excitons in defective van der Waals heterostructures

2021 ◽  
Vol 118 (32) ◽  
pp. e2105468118
Author(s):  
Hongli Guo ◽  
Xu Zhang ◽  
Gang Lu

Excitons can be trapped by moiré potentials in van der Waals (vdW) heterostructures, forming ordered arrays of quantum dots. Excitons can also be trapped by defect potentials as single photon emitters. While the moiré and defect potentials in vdW heterostructures have been studied separately, their interplay remains largely unexplored. Here, we perform first-principles calculations to elucidate the interplay of the two potentials in determining the optoelectronic properties of twisted MoS2/WS2 heterobilayers. The binding energy, charge density, localization, and hybridization of the moiré excitons can be modulated by the competition and cooperation of the two potentials. Their interplay can also be tuned by vertical electric fields, which can either de-trap the excitons or strongly localize them. One can further tailor the interplay of the two potentials via defect engineering to create one-dimensional exciton lattices with tunable orientations. Our work establishes defect engineering as a promising strategy to realize on-demand optoelectronic responses.

2015 ◽  
Author(s):  
Snežana Lazić ◽  
Ekaterina Chernysheva ◽  
Žarko Gačević ◽  
Noemi García-Lepetit ◽  
Herko P. van der Meulen ◽  
...  

Author(s):  
Pankaj K. Jha ◽  
Ghazaleh K. Shirmanesh ◽  
Anna Mitskovets ◽  
Arun Nagpal ◽  
Hamidreza Akbari ◽  
...  

2021 ◽  
Vol 7 (43) ◽  
Author(s):  
Jae-Pil So ◽  
Ha-Reem Kim ◽  
Hyeonjun Baek ◽  
Kwang-Yong Jeong ◽  
Hoo-Cheol Lee ◽  
...  

2021 ◽  
Vol 7 (1) ◽  
Author(s):  
Lei Zhang ◽  
Cheng Tang ◽  
Stefano Sanvito ◽  
Aijun Du

AbstractIntrinsic one-dimensional (1D) ferroelectric materials are rarely reported but are highly sought to break the size limit of nanostructured conventional ferroelectrics. Herein, we report a class of inborn 1D ferroelectric nanowires, namely 1D NbOX3 (X = Cl, Br, and I), that can be directly obtained from experimentally realized van der Waals crystals. In addition to the sizable spontaneous polarization, 1D NbOX3 exhibits low ferroelectric switching barriers, small coercive electric fields, and high critical temperature, governed by the hybridization of the Nb empty d orbitals and the O p orbitals (d0 rule). Moreover, the double-channel structure of 1D NbOX3 also enables the emergence of 1D antiferroelectric metastable states. Our findings not only propose a class of 1D ferroelectric materials toward the development of miniaturized and high-density electronic devices, but also pave an avenue of obtaining intrinsic 1D ferroelectrics from van der Waals crystals.


2019 ◽  
Vol 17 (2) ◽  
pp. 020011 ◽  
Author(s):  
Jiandong Qiao Jiandong Qiao ◽  
Fuhong Mei Fuhong Mei ◽  
Yu Ye Yu Ye

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Kamyar Parto ◽  
Shaimaa I. Azzam ◽  
Kaustav Banerjee ◽  
Galan Moody

AbstractIn recent years, quantum-dot-like single-photon emitters in atomically thin van der Waals materials have become a promising platform for future on-chip scalable quantum light sources with unique advantages over existing technologies, notably the potential for site-specific engineering. However, the required cryogenic temperatures for the functionality of these sources has been an inhibitor of their full potential. Existing methods to create emitters in 2D materials face fundamental challenges in extending the working temperature while maintaining the emitter’s fabrication yield and purity. In this work, we demonstrate a method of creating site-controlled single-photon emitters in atomically thin WSe2 with high yield utilizing independent and simultaneous strain engineering via nanoscale stressors and defect engineering via electron-beam irradiation. Many of the emitters exhibit biexciton cascaded emission, single-photon purities above 95%, and working temperatures up to 150 K. This methodology, coupled with possible plasmonic or optical micro-cavity integration, furthers the realization of scalable, room-temperature, and high-quality 2D single- and entangled-photon sources.


Author(s):  
Teruo Someya ◽  
Jinzo Kobayashi

Recent progress in the electron-mirror microscopy (EMM), e.g., an improvement of its resolving power together with an increase of the magnification makes it useful for investigating the ferroelectric domain physics. English has recently observed the domain texture in the surface layer of BaTiO3. The present authors ) have developed a theory by which one can evaluate small one-dimensional electric fields and/or topographic step heights in the crystal surfaces from their EMM pictures. This theory was applied to a quantitative study of the surface pattern of BaTiO3).


2021 ◽  
Vol 125 (6) ◽  
pp. 1325-1335 ◽  
Author(s):  
Cesar Jara ◽  
Tomáš Rauch ◽  
Silvana Botti ◽  
Miguel A. L. Marques ◽  
Ariel Norambuena ◽  
...  

2021 ◽  
Author(s):  
Lixiang Han ◽  
Mengmeng Yang ◽  
Peiting Wen ◽  
Wei Gao ◽  
nengjie huo ◽  
...  

One dimensional (1D)-two dimensional (2D) van der Waals (vdWs) mixed-dimensional heterostructures with advantages of atomically sharp interface, high quality and good compatibility have attracted tremendous attention in recent years. The...


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