scholarly journals Healing the Ozone Layer

2019 ◽  
pp. 304-322
Author(s):  
Frederike Albrecht ◽  
Charles F. Parker
Keyword(s):  
Gold Standard ◽  
Environmental Governance ◽  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
Policy Changes ◽  
Stratospheric Ozone Layer ◽  
Environmental Regimes ◽  
Global Environmental ◽  
Ozone Depleting Substances

The Montreal Protocol—the regime designed to protect the stratospheric ozone layer—has widely been hailed as the gold standard of global environmental governance and is one of few examples of international institutional cooperative arrangements successfully solving complex transnational problems. Although the stratospheric ozone layer still bears the impacts of ozone depleting substances (ODSs), the problem of ozone depletion is well on its way to being solved due to the protocol. This chapter examines how the protocol was designed and implemented in a way that has allowed it to successfully overcome a number of thorny challenges that most international environmental regimes must face: how to attract sufficient participation, how to promote compliance and manage non-compliance, how to strengthen commitments over time, how to neutralize or co-opt potential ‘veto players’, how to make the costs of implementation affordable, how to leverage public opinion in support of the regime’s goals, and, ultimately, how to promote the behavioural and policy changes needed to solve the problems and achieve the goals the regime was designed to solve. The chapter concludes that while some of the reasons for the Montreal Protocol’s success, such as fairly affordable, available substitutes for ODSs, are not easy to replicate, there are many other elements of this story that can be utilized when thinking about how to design solutions to other transnational environmental problems.

scholarly journals Stratospheric ozone measurements at Arosa (Switzerland): history and scientific relevance

2018 ◽  
Vol 18 (9) ◽  
pp. 6567-6584 ◽  
Author(s):  
Johannes Staehelin ◽  
Pierre Viatte ◽  
Rene Stübi ◽  
Fiona Tummon ◽  
Thomas Peter
Keyword(s):  
Climate Change ◽  
Climate Models ◽  
Weather Forecasting ◽  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
Global Environmental Policy ◽  
Chemical Destruction ◽  
History Of ◽  
Ozone Depleting Substances

Abstract. Climatic Observatory (LKO) in Arosa (Switzerland), marking the beginning of the world's longest series of total (or column) ozone measurements. They were driven by the recognition that atmospheric ozone is important for human health, as well as by scientific curiosity about what was, at the time, an ill characterised atmospheric trace gas. From around the mid-1950s to the beginning of the 1970s studies of high atmosphere circulation patterns that could improve weather forecasting was justification for studying stratospheric ozone. In the mid-1970s, a paradigm shift occurred when it became clear that the damaging effects of anthropogenic ozone-depleting substances (ODSs), such as long-lived chlorofluorocarbons, needed to be documented. This justified continuing the ground-based measurements of stratospheric ozone. Levels of ODSs peaked around the mid-1990s as a result of a global environmental policy to protect the ozone layer, implemented through the 1987 Montreal Protocol and its subsequent amendments and adjustments. Consequently, chemical destruction of stratospheric ozone started to slow around the mid-1990s. To some extent, this raises the question as to whether continued ozone observation is indeed necessary. In the last decade there has been a tendency to reduce the costs associated with making ozone measurements globally including at Arosa. However, the large natural variability in ozone on diurnal, seasonal, and interannual scales complicates the capacity for demonstrating the success of the Montreal Protocol. Chemistry-climate models also predict a super-recovery of the ozone layer at mid-latitudes in the second half of this century, i.e. an increase of ozone concentrations beyond pre-1970 levels, as a consequence of ongoing climate change. These factors, and identifying potentially unexpected stratospheric responses to climate change, support the continued need to document stratospheric ozone changes. This is particularly valuable at the Arosa site, due to the unique length of the observational record. This paper presents the evolution of the ozone layer, the history of international ozone research, and discusses the justification for the measurements in the past, present and into future.

scholarly journals Evidence for a continuous decline in lower stratospheric ozone offsetting ozone layer recovery

2018 ◽  
Vol 18 (2) ◽  
pp. 1379-1394 ◽  
Author(s):  
William T. Ball ◽  
Justin Alsing ◽  
Daniel J. Mortlock ◽  
Johannes Staehelin ◽  
Joanna D. Haigh ◽  
...  
Keyword(s):  
Lower Stratosphere ◽  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
Downward Trend ◽  
Polar Regions ◽  
Total Column Ozone ◽  
Ozone Depleting Substances ◽  
Column Ozone ◽  
Total Column

Abstract. Ozone forms in the Earth's atmosphere from the photodissociation of molecular oxygen, primarily in the tropical stratosphere. It is then transported to the extratropics by the Brewer–Dobson circulation (BDC), forming a protective ozone layer around the globe. Human emissions of halogen-containing ozone-depleting substances (hODSs) led to a decline in stratospheric ozone until they were banned by the Montreal Protocol, and since 1998 ozone in the upper stratosphere is rising again, likely the recovery from halogen-induced losses. Total column measurements of ozone between the Earth's surface and the top of the atmosphere indicate that the ozone layer has stopped declining across the globe, but no clear increase has been observed at latitudes between 60° S and 60° N outside the polar regions (60–90°). Here we report evidence from multiple satellite measurements that ozone in the lower stratosphere between 60° S and 60° N has indeed continued to decline since 1998. We find that, even though upper stratospheric ozone is recovering, the continuing downward trend in the lower stratosphere prevails, resulting in a downward trend in stratospheric column ozone between 60° S and 60° N. We find that total column ozone between 60° S and 60° N appears not to have decreased only because of increases in tropospheric column ozone that compensate for the stratospheric decreases. The reasons for the continued reduction of lower stratospheric ozone are not clear; models do not reproduce these trends, and thus the causes now urgently need to be established.

scholarly journals Inconsistencies between chemistry climate model and observed lower stratospheric trends since 1998

2019 ◽  
Author(s):  
William T. Ball ◽  
Gabriel Chiodo ◽  
Marta Abalos ◽  
Justin Alsing
Keyword(s):  
Large Scale ◽  
Climate Models ◽  
Climate Model ◽  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
Total Column Ozone ◽  
Temperature Trends ◽  
Ozone Depleting Substances ◽  
The Tropics

Abstract. The stratospheric ozone layer shields surface life from harmful ultraviolet radiation. Following the Montreal Protocol ban of long-lived ozone depleting substances (ODSs), rapid depletion of total column ozone (TCO) ceased in the late 1990s and ozone above 32 km now enjoys a clear recovery. However, there is still no confirmation of TCO recovery, and evidence has emerged that ongoing quasi-global (60° S–60° N) lower stratospheric ozone decreases may be responsible, dominated by low latitudes (30° S–30° N). Chemistry climate models (CCMs) used to project future changes predict that lower stratospheric ozone will decrease in the tropics by 2100, but not at mid-latitudes (30°–60°). Here, we show that CCMs display an ozone decline similar to that observed in the tropics over 1998–2016, likely driven by a increase of tropical upwelling. On the other hand, mid-latitude lower stratospheric ozone is observed to decrease, while CCMs show an increase. Despite opposing lower stratospheric ozone changes, which should induce opposite temperature trends, CCM and observed temperature trends agree; we demonstrate that opposing model-observation stratospheric water vapour (SWV) trends, and their associated radiative effects, explain why temperature changes agree in spite of opposing ozone trends. We provide new evidence that the observed mid-latitude trends can be explained by enhanced mixing between the tropics and extratropics. We further show that the temperature trends are consistent with the observed mid-latitude ozone decrease. Together, our results suggest that large scale circulation changes expected in the future from increased greenhouse gases (GHGs) may now already be underway, but that most CCMs are not simulating well mid-latitude ozone layer changes. The reason CCMs do not exhibit the observed changes urgently needs to be understood to improve confidence in future projections of the ozone layer.

scholarly journals Stratospheric ozone measurements at Arosa (Switzerland): History and scientific relevance

2017 ◽  
Author(s):  
Johannes Staehelin ◽  
Pierre Viatte ◽  
Rene Stübi ◽  
Fiona Tummon ◽  
Thomas Peter
Keyword(s):  
Ozone Depletion ◽  
Climate Models ◽  
Stratospheric Ozone ◽  
Cost Savings ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
Global Environmental Policy ◽  
History Of ◽  
Ozone Depleting Substances ◽  
Column Ozone

Abstract. In 1926 the stratospheric ozone measurements of the Light Climatic Observatory (LKO) of Arosa (Switzerland) started, marking the start of the world's longest total (or column) ozone measurements. These measurements were driven by the recognition of the importance of atmospheric ozone for human health as well as by scientific curiosity in this by then not well characterized atmospheric trace gas. Since the mid-1970s ground-based measurements of stratospheric ozone have also been justified to society by the need to document the effects of anthropogenic Ozone Depleting Substances (ODSs), which cause stratospheric ozone depletion. Levels of ODSs peaked around the mid-1990s as a result of a global environmental policy to protect the ozone layer implemented by the 1987 Montreal Protocol and its subsequent amendments and adjustments. Consequently, chemical ozone depletion caused by ODSs stopped worsening around the mid-1990s. This renders justification for continued ozone measurements more difficult, and is likely to do so even more in future, when stratospheric ozone recovery is expected. Tendencies of increased cost savings in ozone measurements seem perceptible worldwide, also in Arosa. However, the large natural variability in ozone on diurnal, seasonal and interannual scales complicates to demonstrate the success of the Montreal Protocol. Moreover, chemistry-climate models predict a “super-recovery” of the ozone layer in the second half of this century, i.e. an increase of ozone concentrations beyond pre-1970 levels, as a consequence of ongoing climate change. This paper presents the evolution of the ozone layer and the history of international ozone research and discusses the justification of these measurements for past, present and future.

scholarly journals Continuous decline in lower stratospheric ozone offsets ozone layer recovery

2017 ◽  
Author(s):  
William T. Ball ◽  
Justin Alsing ◽  
Daniel J. Mortlock ◽  
Johannes Staehelin ◽  
Joanna D. Haigh ◽  
...  
Keyword(s):  
Respiratory Health ◽  
Stratospheric Ozone ◽  
Ultra Violet ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
Polar Regions ◽  
Total Column Ozone ◽  
Ozone Trends ◽  
Ozone Depleting Substances ◽  
Column Ozone

Abstract. Ozone forms in the Earth's atmosphere from the photodissociation of molecular oxygen, primarily in the tropical stratosphere. It is then transported to the extratropics by the Brewer-Dobson circulation (BDC), forming a protective ozone layer around the globe. Human emissions of halogen-containing ozone-depleting substances (hODSs) led to a decline in stratospheric ozone until they were banned by the Montreal Protocol (MP), and since 1998 ozone in the upper stratosphere shows a likely recovery. Total column ozone (TCO) measurements of ozone between the Earth's surface and the top of the atmosphere, indicate that the ozone layer has stopped declining across the globe, but no clear increase has been observed at latitudes outside the polar regions (60–90). Here we report evidence from multiple satellite measurements that ozone in the lower stratosphere between 60° S and 60° N has declined continuously since 1985. We find that, even though upper stratospheric ozone is recovering in response to the MP, the lower stratospheric changes more than compensate for this, resulting in the conclusion that, globally (60°&tinsp;S–60° N), stratospheric column ozone (StCO) continues to deplete. We find that globally, TCO appears to not have decreased because tropospheric column ozone (TrCO) increases, likely the result of human activity and harmful to respiratory health, are compensating for the stratospheric decreases. The reason for the continued reduction of lower stratospheric ozone is not clear, models do not reproduce these trends, and so the causes now urgently need to be established. Reductions in lower stratospheric ozone trends may partly lead to a small reduction in the warming of the climate, but a reduced ozone layer may also permit an increase in harmful ultra-violet (UV) radiation at the surface and would impact human and ecosystem health.

scholarly journals Tropospheric temperature response to stratospheric ozone recovery in the 21st century

2010 ◽  
Vol 10 (9) ◽  
pp. 22019-22046 ◽  
Author(s):  
Y. Hu ◽  
Y. Xia ◽  
Q. Fu
Keyword(s):  
21St Century ◽  
Climate Model ◽  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Montreal Protocol ◽  
The Arctic ◽  
Boreal Winter ◽  
Tropospheric Temperature ◽  
Surface Warming ◽  
Stratospheric Ozone Layer

Abstract. Observations show a stabilization or a weak increase of the stratospheric ozone layer since the late 1990s. Recent coupled chemistry-climate model simulations predicted that the stratospheric ozone layer will likely return to pre-1980 levels in the middle of the 21st century, as a results of the decline of ozone depleting substances under the 1987 Montreal Protocol. Since the ozone layer is an important component in determining stratospheric and tropospheric-surface energy balance, the recovery of the ozone layer may have significant impact on tropospheric-surface climate. Here, using multi-model ensemble results from both the Intergovernmental Panel on Climate Change Fourth Assessment Report (IPCC-AR4) models and coupled chemistry-climate models, we show that as ozone recovery is considered, the troposphere is warmed more than that without considering ozone recovery, suggesting an enhancement of tropospheric warming due to ozone recovery. It is found that the enhanced tropospheric warming is mostly significant in the upper troposphere, with a global mean magnitude of ~0.41 K for 2001–2050. We also find that relatively large enhanced warming occurs in the extratropics and polar regions in summer and autumn in both hemispheres while the enhanced warming is stronger in the Northern Hemisphere than in the Southern Hemisphere. Enhanced warming is also found at the surface. The strongest enhancement of surface warming is located in the Arctic in boreal winter. The global annual mean enhancement of surface warming is about 0.16 K for 2001–2050.

Stratospheric ozone layer observations over tsukuba, Japan by NIES ozone DIAL.

2007 ◽  
Author(s):  
Boyan Tatarov ◽  
Chan Bong Park ◽  
Hideaki Nakane ◽  
Nobuo Sugimoto ◽  
Ichiro Matsui ◽  
...  
Keyword(s):  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Stratospheric Ozone Layer

Chlorine Oxide in the Stratospheric Ozone Layer: Ground-Based Detection and Measurement

Science ◽  
1981 ◽  
Vol 211 (4487) ◽  
pp. 1158-1161 ◽  
Author(s):  
A. PARRISH ◽  
R. L. DE ZAFRA ◽  
P. M. SOLOMON ◽  
J. W. BARRETT ◽  
E. R. CARLSON
Keyword(s):  
Stratospheric Ozone ◽  
Ozone Layer ◽  
Chlorine Oxide ◽  
Stratospheric Ozone Layer

Atmospheric impacts of short-lived chlorinated species over the recent past: a chemistry-climate perspective

2021 ◽  
Author(s):  
Ewa Bednarz ◽  
Ryan Hossaini ◽  
Luke Abraham ◽  
Peter Braesicke ◽  
Martyn Chipperfield
Keyword(s):  
Atmospheric Chemistry ◽  
Climate Model ◽  
Stratospheric Ozone ◽  
Lower Boundary ◽  
Montreal Protocol ◽  
Recent Past ◽  
Substantial Impact ◽  
Ozone Depleting Substances ◽  
The Impact

<p>The emissions of most long-lived halogenated ozone-depleting substances (ODSs) are now decreasing, owing to controls on their production introduced by Montreal Protocol and its amendments. However, short-lived halogenated compounds can also have substantial impact on atmospheric chemistry, including stratospheric ozone, particularly if emitted near climatological uplift regions. It has recently become evident that emissions of some chlorinated very short-lived species (VSLSs), such as chloroform (CHCl<sub>3</sub>) and dichloromethane (CH<sub>2</sub>Cl<sub>2</sub>), could be larger than previously believed and increasing, particularly in Asia. While these may exert a significant influence on atmospheric chemistry and climate, their impacts remain poorly characterised. </p><p> </p><p>We address this issue using the UM-UKCA chemistry-climate model (CCM). While not only the first, to our knowledge, model study addressing this problem using a CCM, it is also the first such study employing a whole atmosphere model, thereby simulating the tropospheric Cl-VSLSs emissions and the resulting stratospheric impacts in a fully consistent manner. We use a newly developed Double-Extended Stratospheric-Tropospheric (DEST) chemistry scheme, which includes emissions of all major chlorinated and brominated VSLSs alongside an extended treatment of long-lived ODSs.</p><p> </p><p>We examine the impacts of rising Cl-VSLSs emissions on atmospheric chlorine tracers and ozone, including their long-term trends. We pay particular attention to the role of ‘nudging’, as opposed to the free-running model set up, for the simulated Cl-VSLSs impacts, thereby demostrating the role of atmospheric dynamics in modulating the atmospheric responses to Cl-VSLSs. In addition, we employ novel estimates of Cl-VSLS emissions over the recent past and compare the results with the simulations that prescribe Cl-VSLSs using simple lower boundary conditions. This allows us to demonstrate the impact such choice has on the dominant location and seasonality of the Cl-VSLSs transport into the stratosphere.</p>

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