scholarly journals Large-Scale Computational Screening of Novel Compounds for Carbon Capture

2014 ◽  
Vol 70 (a1) ◽  
pp. C1538-C1538
Author(s):  
Matthew Dunstan ◽  
Wen Liu ◽  
Shyue Ping Ong ◽  
Anubhav Jain ◽  
Kristin Persson ◽  
...  
Keyword(s):  
Carbon Capture ◽  
Power Plants ◽  
Large Scale ◽  
Waste Heat ◽  
Experimental Studies ◽  
Carbon Capture And Storage ◽  
Kinetic Properties ◽  
Computational Screening ◽  
Energy Penalty ◽  
And Storage

Carbon capture and storage (CCS) applications offer a plausible solution to the urgent need for a carbon neutral energy source from stationary sources, including power plants and industrial processes. The most mature technology for post-combustion capture currently uses a liquid sorbent, amine scrubbing. However, with the existing technology, a large amount of heat is required for the regeneration of the liquid sorbent, which introduces a substantial energy penalty. Operation at higher temperatures could reduce this energy penalty by allowing the integration of waste heat back into the power cycle. New solid absorbents for use at intermediate to high temperatures, such as CaO, have shown promise in pilot plant studies, but are still far from ideal due to their poor capacity retention upon successive cycling. This presentation will describe our studies aimed at rationally selecting and designing materials for carbon capture and storage applications. We use ab initio calculations of oxide materials from the Materials Project database1 in an effort to screen for novel materials with optimal thermodynamic and kinetic properties for CO2 looping applications. From the determination of a material's optimised structure and ground state energy we have then constructed a screening routine for materials within the database based on simulating their carbonation equilibria and phase stability under differing atmospheric concentrations of CO2. A number of promising materials were identified from the screening, and we are currently investigating their properties experimentally, by using a combination of methods (including thermogravimetric analysis, in situ x-ray diffraction and microscopy). In this way we are able to assess the validity of the screening methodology, and use the insights afforded by experimental studies to iteratively improve the entire process.

scholarly journals A Review on CO2 Capture Technologies with Focus on CO2-Enhanced Methane Recovery from Hydrates

Energies ◽  
2021 ◽  
Vol 14 (2) ◽  
pp. 387
Author(s):  
Salvatore F. Cannone ◽  
Andrea Lanzini ◽  
Massimo Santarelli
Keyword(s):  
Natural Gas ◽  
Carbon Capture ◽  
Power Plants ◽  
Large Scale ◽  
Carbon Capture And Storage ◽  
Co2 Removal ◽  
Methane Recovery ◽  
The World ◽  
Co2 Transportation ◽  
And Storage

Natural gas is considered a helpful transition fuel in order to reduce the greenhouse gas emissions of other conventional power plants burning coal or liquid fossil fuels. Natural Gas Hydrates (NGHs) constitute the largest reservoir of natural gas in the world. Methane contained within the crystalline structure can be replaced by carbon dioxide to enhance gas recovery from hydrates. This technical review presents a techno-economic analysis of the full pathway, which begins with the capture of CO2 from power and process industries and ends with its transportation to a geological sequestration site consisting of clathrate hydrates. Since extracted methane is still rich in CO2, on-site separation is required. Focus is thus placed on membrane-based gas separation technologies widely used for gas purification and CO2 removal from raw natural gas and exhaust gas. Nevertheless, the other carbon capture processes (i.e., oxy-fuel combustion, pre-combustion and post-combustion) are briefly discussed and their carbon capture costs are compared with membrane separation technology. Since a large-scale Carbon Capture and Storage (CCS) facility requires CO2 transportation and storage infrastructure, a technical, cost and safety assessment of CO2 transportation over long distances is carried out. Finally, this paper provides an overview of the storage solutions developed around the world, principally studying the geological NGH formation for CO2 sinks.

scholarly journals Total cost of carbon capture and storage implemented at a regional scale: northeastern and midwestern United States

2020 ◽  
Vol 10 (5) ◽  
pp. 20190065 ◽  
Author(s):  
William J. Schmelz ◽  
Gal Hochman ◽  
Kenneth G. Miller
Keyword(s):  
United States ◽  
Carbon Capture ◽  
Power Plants ◽  
Large Scale ◽  
Regional Scale ◽  
Carbon Capture And Storage ◽  
Midwestern United States ◽  
Additional Costs ◽  
The Cost ◽  
And Storage

We model the costs of carbon capture and storage (CCS) in subsurface geological formations for emissions from 138 northeastern and midwestern electricity-generating power plants. The analysis suggests coal-sourced CO 2 emissions can be stored in this region at a cost of $52–$60 ton −1 , whereas the cost to store emission from natural-gas-fired plants ranges from approximately $80 to $90. Storing emissions offshore increases the lowest total costs of CCS to over $60 per ton of CO 2 for coal. Because there apparently is sufficient onshore storage in the northeastern and midwestern United States, offshore storage is not necessary or economical unless there are additional costs or suitability issues associated with the onshore reservoirs. For example, if formation pressures are prohibitive in a large-scale deployment of onshore CCS, or if there is opposition to onshore storage, offshore storage space could probably store emissions at an additional cost of less than $10 ton −1 . Finally, it is likely that more than 8 Gt of total CO 2 emissions from this region can be stored for less $60 ton −1 , slightly more than the $50 ton −1 Section 45Q tax credits incentivizing CCS.

scholarly journals Scrutinising the Gap between the Expected and Actual Deployment of Carbon Capture and Storage—A Bibliometric Analysis

Energies ◽  
2018 ◽  
Vol 11 (9) ◽  
pp. 2319 ◽  
Author(s):  
Peter Viebahn ◽  
Emile Chappin
Keyword(s):  
Carbon Capture ◽  
Power Plants ◽  
Public Perception ◽  
Large Scale ◽  
National Level ◽  
Carbon Capture And Storage ◽  
Holistic Approach ◽  
Energy System ◽  
Research Front ◽  
And Storage

For many years, carbon capture and storage (CCS) has been discussed as a technology that may make a significant contribution to achieving major reductions in greenhouse gas emissions. At present, however, only two large-scale power plants capture a total of 2.4 Mt CO2/a. Several reasons are identified for this mismatch between expectations and realised deployment. Applying bibliographic coupling, the research front of CCS, understood to be published peer-reviewed papers, is explored to scrutinise whether the current research is sufficient to meet these problems. The analysis reveals that research is dominated by technical research (69%). Only 31% of papers address non-technical issues, particularly exploring public perception, policy, and regulation, providing a broader view on CCS implementation on the regional or national level, or using assessment frameworks. This shows that the research is advancing and attempting to meet the outlined problems, which are mainly non-technology related. In addition to strengthening this research, the proportion of papers that adopt a holistic approach may be increased in a bid to meet the challenges involved in transforming a complex energy system. It may also be useful to include a broad variety of stakeholders in research so as to provide a more resilient development of CCS deployment strategies.

scholarly journals Life Cycle Assessment of Direct Air Carbon Capture and Storage with Low-Carbon Energy Sources

2021 ◽  
Author(s):  
Tom Terlouw ◽  
Karin Treyer ◽  
christian bauer ◽  
Marco Mazzotti
Keyword(s):  
Life Cycle Assessment ◽  
Life Cycle ◽  
Carbon Capture ◽  
Large Scale ◽  
Carbon Capture And Storage ◽  
Low Carbon ◽  
Solid Sorbent ◽  
Low Carbon Energy ◽  
And Storage ◽  
Limited Scope

Prospective energy scenarios usually rely on Carbon Dioxide Removal (CDR) technologies to achieve the climate goals of the Paris Agreement. CDR technologies aim at removing CO2 from the atmosphere in a permanent way. However, the implementation of CDR technologies typically comes along with unintended environmental side-effects such as land transformation or water consumption. These need to be quantified before large-scale implementation of any CDR option by means of Life Cycle Assessment (LCA). Direct Air Carbon Capture and Storage (DACCS) is considered to be among the CDR technologies closest to large-scale implementation, since first pilot and demonstration units have been installed and interactions with the environment are less complex than for biomass related CDR options. However, only very few LCA studies - with limited scope - have been conducted so far to determine the overall life-cycle environmental performance of DACCS. We provide a comprehensive LCA of different low temperature DACCS configurations - pertaining to solid sorbent-based technology - including a global and prospective analysis.

Sequential Combustion in Ansaldo Energia Gas Turbines: The Technology Enabler for CO2-Free, Highly Efficient Power Production Based on Hydrogen

2020 ◽  
Author(s):  
Andrea Ciani ◽  
John P. Wood ◽  
Anders Wickström ◽  
Geir J. Rørtveit ◽  
Rosetta Steeneveldt ◽  
...  
Keyword(s):  
Power Generation ◽  
Free Energy ◽  
Gas Turbines ◽  
Carbon Capture ◽  
Power Plants ◽  
Carbon Capture And Storage ◽  
Combined Cycle ◽  
Fuel Flexibility ◽  
Combustion Technology ◽  
And Storage

Abstract Today gas turbines and combined cycle power plants play an important role in power generation and in the light of increasing energy demand, their role is expected to grow alongside renewables. In addition, the volatility of renewables in generating and dispatching power entails a new focus on electricity security. This reinforces the importance of gas turbines in guaranteeing grid reliability by compensating for the intermittency of renewables. In order to achieve the Paris Agreement’s goals, power generation must be decarbonized. This is where hydrogen produced from renewables or with CCS (Carbon Capture and Storage) comes into play, allowing totally CO2-free combustion. Hydrogen features the unique capability to store energy for medium to long storage cycles and hence could be used to alleviate seasonal variations of renewable power generation. The importance of hydrogen for future power generation is expected to increase due to several factors: the push for CO2-free energy production is calling for various options, all resulting in the necessity of a broader fuel flexibility, in particular accommodating hydrogen as a future fuel feeding gas turbines and combined cycle power plants. Hydrogen from methane reforming is pursued, with particular interest within energy scenarios linked with carbon capture and storage, while the increased share of renewables requires the storage of energy for which hydrogen is the best candidate. Compared to natural gas the main challenge of hydrogen combustion is its increased reactivity resulting in a decrease of engine performance for conventional premix combustion systems. The sequential combustion technology used within Ansaldo Energia’s GT36 and GT26 gas turbines provides for extra freedom in optimizing the operation concept. This sequential combustion technology enables low emission combustion at high temperatures with particularly high fuel flexibility thanks to the complementarity between its first stage, stabilized by flame propagation and its second (sequential) stage, stabilized by auto-ignition. With this concept, gas turbines are envisaged to be able to provide reliable, dispatchable, CO2-free electric power. In this paper, an overview of hydrogen production (grey, blue, and green hydrogen), transport and storage are presented targeting a CO2-free energy system based on gas turbines. A detailed description of the test infrastructure, handling of highly reactive fuels is given with specific aspects of the large amounts of hydrogen used for the full engine pressure tests. Based on the results discussed at last year’s Turbo Expo (Bothien et al. GT2019-90798), further high pressure test results are reported, demonstrating how sequential combustion with novel operational concepts is able to achieve the lowest emissions, highest fuel and operational flexibility, for very high combustor exit temperatures (H-class) with unprecedented hydrogen contents.

scholarly journals Carbon Capture and Storage: A Review of Mineral Storage of CO2 in Greece

2018 ◽  
Vol 10 (12) ◽  
pp. 4400 ◽  
Author(s):  
Kyriaki Kelektsoglou
Keyword(s):  
Co2 Sequestration ◽  
Carbon Capture ◽  
Power Plants ◽  
Carbon Capture And Storage ◽  
Mineral Carbonation ◽  
Current State ◽  
Novel Method ◽  
Carbon Dioxide Co2 ◽  
Carbonate Materials ◽  
And Storage

As the demand for the reduction of global emissions of carbon dioxide (CO2) increases, the need for anthropogenic CO2 emission reductions becomes urgent. One promising technology to this end, is carbon capture and storage (CCS). This paper aims to provide the current state-of-the-art of CO2 capure, transport, and storage and focuses on mineral carbonation, a novel method for safe and permanent CO2 sequestration which is based on the reaction of CO2 with calcium or magnesium oxides or hydroxides to form stable carbonate materials. Current commercial scale projects of CCS around Europe are outlined, demonstrating that only three of them are in operation, and twenty-one of them are in pilot phase, including the only one case of mineral carbonation in Europe the case of CarbFix in Iceland. This paper considers the necessity of CO2 sequestration in Greece as emissions of about 64.6 million tons of CO2 annually, originate from the lignite fired power plants. A real case study concerning the mineral storage of CO2 in Greece has been conducted, demonstrating the applicability of several geological forms around Greece for mineral carbonation. The study indicates that Mount Pindos ophiolite and Vourinos ophiolite complex could be a promising means of CO2 sequestration with mineral carbonation. Further studies are needed in order to confirm this aspect.

Sign in / Sign up

Export Citation Format

Share Document