Progress Toward Understanding Catastrophic Failure of Electric Vehicle Li-Ion Batteries: Multi-Physics Modeling

Author(s):  
Mehdi Gilaki ◽  
Alex Francis ◽  
Daniel Bautista ◽  
Ilya Avdeev

The goal of this work is to enhance understanding of critical design aspects that would prevent automotive lithium-ion battery packs from catastrophic failures. Modeling lithium-ion batteries is a complex multiscale multi-physics problem. The most dangerous energy producing component of a lithium ion cylindrical cell, jellyroll, is a layered spiral structure, which consists of thin layers of electrodes and separator only microns thick. In this study, we investigate the feasibility of using commercial explicit finite element code LS-DYNA to understand the structural integrity of lithium-ion batteries subjected to crushing condition through computer simulation. The jellyroll was treated as homogeneous material with an effective stress-strain curve obtained through characterization experiments of representative jellyroll samples and individual electrode layers. Physical and numerical impact tests have been conducted on cylindrical cells using developed drop test system. Results of material homogenization, experimental drop testing, and initial structural simulations are discussed. The investigation of structural cell deformations coupled with thermal heat generation and distribution after the crash brings us one step closer to accurate modeling of the entire battery pack that consists of hundreds of cells.

2019 ◽  
Vol 7 (20) ◽  
pp. 12593-12603 ◽  
Author(s):  
Münir M. Besli ◽  
Alpesh Khushalchand Shukla ◽  
Chenxi Wei ◽  
Michael Metzger ◽  
Judith Alvarado ◽  
...  

The structural integrity of layered Ni-rich oxide cathode materials is one of the most essential factors that critically affect the performance and reliability of lithium-ion batteries.


2019 ◽  
Vol 11 (21) ◽  
pp. 6050 ◽  
Author(s):  
Pablo Korth Pereira Ferraz ◽  
Julia Kowal

Modern battery energy systems are key enablers of the conversion of our energy and mobility sector towards renewability. Most of the time, their batteries are connected to power electronics that induce high frequency current ripple on the batteries that could lead to reinforced battery ageing. This study investigates the influence of high frequency current ripple on the ageing of commercially available, cylindrical 18,650 lithium-ion batteries in comparison to identical batteries that are aged with a conventional battery test system. The respective ageing tests that have been carried out to obtain numerous parameters such as the capacity loss, the gradient of voltage curves and impedance spectra are explained and evaluated to pinpoint how current ripple possibly affects battery ageing. Finally, the results suggest that there is little to no further influence of current ripple that is severe enough to stand out against ageing effects due to the underlying accelerated cyclic ageing.


Author(s):  
Weijuan Wang ◽  
Hui Xu ◽  
Genxi Yu ◽  
Daming Chen ◽  
Shangqi Sun ◽  
...  

Rationally engineering flexible anodes with electrochemical and mechanical robustness while maintaining the structural integrity is highly desirable for the realization of high-performance flexible lithium-ion batteries (LIBs). Herein, an integrated flexible...


2019 ◽  
Vol 7 (43) ◽  
pp. 25155-25164 ◽  
Author(s):  
Jianding Li ◽  
Huajun Zhao ◽  
Meimei Wang ◽  
Yongyang Zhu ◽  
Bo Li ◽  
...  

A ZnO encapsulated in a 3D NCNF composite exhibits excellent electrochemical performances both in a half cell and full cell. The improved performances are mainly explained based on the two aspects of structural integrity and kinetics enhancement.


2019 ◽  
Vol 55 (4) ◽  
pp. 545-548 ◽  
Author(s):  
Hirotaka Inomata ◽  
Yasufumi Takahashi ◽  
Daiko Takamatsu ◽  
Akichika Kumatani ◽  
Hiroki Ida ◽  
...  

Cathode surface coating with metal-oxide thin layers has been intensively studied to improve the cycle durability of lithium-ion batteries.


Author(s):  
Ilya V. Avdeev ◽  
Mehdi Gilaki

High-voltage lithium-ion batteries are increasingly used in electric and hybrid-electric vehicles. Due to a risk of being in an accident, these energy storage systems should be analyzed thoroughly so that the risk of failure or serious damage during accidents is minimized. In this research a three-dimensional finite element simulation of a cylindrical battery cell is performed to study the behavior of the cell under various loading conditions. Li-Ion batteries consist of very thin layers of anodes, cathodes and separators that are packed into a cylindrical-spiral shape. This non-homogeneity nature of the battery cells makes the finite element explicit model very complicated. In this study, a homogenized 3-D model of the cell has been developed that is more suitable for explicit high-strain-rate transient analyses. Another model using layered solid or thick shell elements was generated. For the latter, partially two-phased homogenized material properties were used. Three different configurations are considered to analyze the battery packs: an indentation test with a rigid tube, longitudinal crushing between rigid plates, and transverse crushing. Results from these numerical simulations were consistent for models with thick shell elements and homogenized models.


2016 ◽  
Vol 4 (32) ◽  
pp. 12487-12496 ◽  
Author(s):  
Xueying Li ◽  
Yuanyuan Ma ◽  
Guozhong Cao ◽  
Yongquan Qu

Porous FeOx@C yolk/shell nanowires with optimized void space delivered a stable cyclability over 400 cycles, high capacities and a good rate capability. The optimized void space contributes to preserve structural integrity and maintain good electrical contact between FeOx and C.


Author(s):  
Ashkan Nazari ◽  
Roja Esmaeeli ◽  
Seyed Reza Hashemi ◽  
Haniph Aliniagerdroudbari ◽  
Siamak Farhad

In this study, the low-temperature energy efficiency of lithium-ion batteries (LIBs) with different chemistries and nominal capacities at various charge and discharge rates is studied through multi-physics modeling and computer simulation. The model is based on the irreversible heat generation in the battery, leading to the charge/discharge efficiency in LIBs with graphite/LiFePO4, graphite/LiMn2O4, and graphite/LiCoO2 electrode materials in which the effects of the battery nominal capacity at various charge and discharge rates are studied. Using characterized sources of the heat generation in the LIB leads to providing a battery efficiency plot at different operation condition for each LIBs. The results of this study assist the battery engineers to have much more accurate prediction over the efficiency of the LIBs at low temperatures.


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