Gas ionization by focused laser beams

1984 ◽  
Vol 62 (10) ◽  
pp. 1010-1013 ◽  
Author(s):  
A. L. de Brito

It is shown that the effect of line broadening by focusing may contribute considerably to the observed laser-induced ionization of gases even when the ionization energy of the gas molecules is well above the mean photon energy of the laser radiation.


1985 ◽  
Vol 63 (7) ◽  
pp. 1013-1013
Author(s):  
F. L. Curzon

It is pointed out that the frequency spectrum of a laser beam is not broadened when the beam is focused by a normal lens. This assertion contradicts the conclusion reached by the authors of the articles cited in the title above.





1968 ◽  
Vol 21 (1) ◽  
pp. 13 ◽  
Author(s):  
RW Parsons ◽  
VI Metchnik ◽  
RJ Dyne

The shape of a collision-broadened spectral line depends on the assumptions made about the collision processes involved. If the collision cross section varies inversely as the relative speed of the colliding molecules, the half-width to the half-power points and to the points of steepest slope should be 1/27T1' and 1/(2";3)7T1' respectively, where l' is the mean interval between line-broadening collisions. It is shown that, in a gas of "hard-sphere" molecules, the shape of the line is modified and the above half-widths are reduced by' 6�4 and 9�7% respectively. While it is not suggested that gas molecules behave entirely as hard spheres, it is suggested that some deviations from the Van Vleck-Weisskopf-Lorentz shape may occur, and that it may be possible to detect these deviations experimentally



1984 ◽  
Vol 62 (7) ◽  
pp. 661-668 ◽  
Author(s):  
Adelsindo Liberato de Brito ◽  
Arthur Jabs

We point out that the spectral width of a quasimonochromatic light beam broadens when the beam is focused. A quantitative formula for this broadening is derived from classical wave theory. The effect is shown to explain some experiments on laser beams done by Panarella which he explained using the ad hoc hypothesis that the frequency of the photons changes along with the intensity of the light beam. The line broadening by focusing might also contribute to gas ionization by incident light when the ionization potential is well above the mean photon energy. Remarks are made on some direct applications of the Heisenberg relations in comparison with our treatment.



The development with time of the excitation of a transition between two atomic or molecular energy levels under the influence of monochromatic laser radiation is examined under conditions of strictly inhomogeneous line broadening due to such causes as doppler shift arising from translational velocity. The ratio of the number of molecules, N 2 , in an excited state to the total number, N , is calculated for various ratios of the intensity parameter β ═ E 0 μ / ħ to the half line-width ∆ , where E 0 is the amplitude of the electric field in the incident radiation and is the dipole moment matrix element for the transition. Excitation functions obtained in a previous paper (I) for various values of the ratio γ/β , where γ is the half line-width in the absence of inhomo­geneous broadening, are used to obtain the variation of N 2 / N with time under conditions of mixed broadening for various values of the ratio γ/∆ and γ/β , when the exciting radiation is in exact resonance with the central frequency of the transition.



2008 ◽  
Vol 16 (26) ◽  
pp. 22090 ◽  
Author(s):  
Carlos J. Zapata-Rodríguez ◽  
Miguel A. Porras


1997 ◽  
Vol 30 (4) ◽  
pp. 427-430 ◽  
Author(s):  
F. Sánchez-Bajo ◽  
F. L. Cumbrera

A modified application of the variance method, using the pseudo-Voigt function as a good approximation to the X-ray diffraction profiles, is proposed in order to obtain microstructural quantities such as the mean crystallite size and root-mean-square (r.m.s.) strain. Whereas the variance method in its original form is applicable only to well separated reflections, this technique can be employed in the cases where there is line-profile overlap. Determination of the mean crystallite size and r.m.s. strain for several crystallographic directions in a nanocrystalline cubic sample of 9-YSZ (yttria-stabilized zirconia) has been performed by means of this procedure.



1977 ◽  
Vol 16 (4) ◽  
pp. 1104 ◽  
Author(s):  
Lee W. Casperson ◽  
C. Yeh ◽  
Wing F. Yeung


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