scholarly journals Using MODIS and AERONET to Determine GCM Aerosol Size

2006 ◽  
Vol 63 (4) ◽  
pp. 1338-1347 ◽  
Author(s):  
Glen Lesins ◽  
Ulrike Lohmann

Abstract Aerosol size is still a poorly constrained quantity in general circulation models (GCMs). By using the modal radii of the coarse and fine mode retrieved from 103 stations in the Aerosol Robotic Network (AERONET) and the fine mode aerosol optical depth fraction derived from both the Moderate Resolute Imaging Spectroradiometer (MODIS) Terra and AERONET, a globally and monthly averaged aerosol size distribution dataset was computed assuming internally mixed aerosols. Different methods were employed in creating the size distribution datasets that were input to the ECHAM4 climate model giving a globally averaged aerosol optical depth (AOD) at 500 nm that ranged from 0.11 to 0.20 depending on the method. This translates into a globally averaged direct aerosol top-of-atmosphere forcing range from −1.6 to −3.9 W m−2. Reducing the uncertainty in the aerosol sizes is important when using AOD to validate models since mass burden errors can then be assumed to be the main AOD error source. This paper explores a procedure that can help achieve this goal.

2018 ◽  
Vol 10 (11) ◽  
pp. 1838 ◽  
Author(s):  
Yang Zhang ◽  
Zhengqiang Li ◽  
Zhihong Liu ◽  
Juan Zhang ◽  
Lili Qie ◽  
...  

The fine-mode aerosol optical depth (AODf) is an important parameter for the environment and climate change study, which mainly represents the anthropogenic aerosols component. The Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar (PARASOL) instrument can detect polarized signal from multi-angle observation and the polarized signal mainly comes from the radiation contribution of the fine-mode aerosols, which provides an opportunity to obtain AODf directly. However, the currently operational algorithm of Laboratoire d’Optique Atmosphérique (LOA) has a poor AODf retrieval accuracy over East China on high aerosol loading days. This study focused on solving this issue and proposed a grouped residual error sorting (GRES) method to determine the optimal aerosol model in AODf retrieval using the traditional look-up table (LUT) approach and then the AODf retrieval accuracy over East China was improved. The comparisons between the GRES retrieved and the Aerosol Robotic Network (AERONET) ground-based AODf at Beijing, Xianghe, Taihu and Hong_Kong_PolyU sites produced high correlation coefficients (r) of 0.900, 0.933, 0.957 and 0.968, respectively. The comparisons of the GRES retrieved AODf and PARASOL AODf product with those of the AERONET observations produced a mean absolute error (MAE) of 0.054 versus 0.104 on high aerosol loading days (AERONET mean AODf at 865 nm = 0.283). An application using the GRES method for total AOD (AODt) retrieval also showed a good expandability for multi-angle aerosol retrieval of this method.


2014 ◽  
Vol 14 (21) ◽  
pp. 11633-11656 ◽  
Author(s):  
T. F. Eck ◽  
B. N. Holben ◽  
J. S. Reid ◽  
A. Arola ◽  
R. A. Ferrare ◽  
...  

Abstract. During the July 2011 Deriving Information on Surface conditions from Column and Vertically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) field experiment in Maryland, significant enhancements in Aerosol Robotic Network (AERONET) sun–sky radiometer measured aerosol optical depth (AOD) were observed in the immediate vicinity of non-precipitating cumulus clouds on some days. Both measured Ångström exponents and aerosol size distribution retrievals made before, during and after cumulus development often suggest little change in fine mode particle size; therefore, implying possible new particle formation in addition to cloud processing and humidification of existing particles. In addition to sun–sky radiometer measurements of large enhancements of fine mode AOD, lidar measurements made from both ground-based and aircraft-based instruments during the experiment also measured large increases in aerosol signal at altitudes associated with the presence of fair weather cumulus clouds. These data show modifications of the aerosol vertical profile as a result of the aerosol enhancements at and below cloud altitudes. The airborne lidar data were utilized to estimate the spatial extent of these aerosol enhancements, finding increased AOD, backscatter and extinction out to 2.5 km distance from the cloud edge. Furthermore, in situ measurements made from aircraft vertical profiles over an AERONET site during the experiment also showed large increases in aerosol scattering and aerosol volume after cloud formation as compared to before. The 15-year AERONET database of AOD measurements at the Goddard Space Flight Center (GSFC), Maryland site, was investigated in order to obtain a climatological perspective of this phenomenon of AOD enhancement. Analysis of the diurnal cycle of AOD in summer showed significant increases in AOD from morning to late afternoon, corresponding to the diurnal cycle of cumulus development.


2020 ◽  
Author(s):  
Dmitry M. Kabanov ◽  
Christoph Ritter ◽  
Sergey M. Sakerin

Abstract. In this work hourly averaged sun photometer data from the sites Barentsburg and Ny-Ålesund, both located in Spitsbergen in the European Arctic, are compared. Our data set comprises the years 2011 to 2017. We found for more turbid periods (aerosol optical depth τ0.5 > 0.1) that typically Barentsburg is more polluted than Ny-Ålesund, especially in the short wave spectrum. However, the diurnal variation of AOD is highly correlated. Next, τ was divided into a fine and coarse mode. It was found that generally the fine mode aerosol optical depth dominates and also shows a larger interannual as inner annual variation. Tau fine τf is in fact larger in spring during the Arctic Haze period. Overall the aerosol optical depth seems to decrease, although this is not statistically significant.


2020 ◽  
Vol 57 (3) ◽  
pp. 030101
Author(s):  
高迦南 Gao Jianan ◽  
李丽萍 Li Liping ◽  
崔廷伟 Cui Tingwei ◽  
陈晨 Chen Chen

2010 ◽  
Vol 10 (4) ◽  
pp. 1689-1699 ◽  
Author(s):  
R. M. Mitchell ◽  
S. K. Campbell ◽  
Y. Qin

Abstract. Collocated sun photometer and nephelometer measurements at Tinga Tingana in the Australian Outback over the decade 1997–2007 show a significant increase in aerosol loading following the onset of severe drought conditions in 2002. This increase is confined to the season of dust activity, particularly September to March. In contrast, background aerosol levels during May, June and July remained stable. The enhanced aerosol loadings during the latter 5 years of the study period can be understood as a combination of dune destabilisation through loss of ephemeral vegetation and surface crust, and the changing supply of fluvial sediments to ephemeral lakes and floodplains within the Lake Eyre Basin. Major dust outbreaks are generally highly localised, although significant dust activity was observed at Tinga Tingana on 50% of days when a major event occurred elsewhere in the Lake Eyre Basin, suggesting frequent basin-wide dust mobilisation. Combined analysis of aerosol optical depth and scattering coefficient shows weak correlation between the surface and column aerosol (R2=0.24). The aerosol scale height is broadly distributed with a mode typically between 2–3 km, with clearly defined seasonal variation. Climatological analysis reveals bimodal structure in the annual cycle of aerosol optical depth, with a summer peak related to maximal dust activity, and a spring peak related to lofted fine-mode aerosol. There is evidence for an increase in near-surface aerosol during the period 2003–2007 relative to 1997–2002, consistent with an increase in dust activity. This accords with an independent finding of increasing aerosol loading over the Australian region as a whole, suggesting that rising dust activity over the Lake Eyre Basin may be a significant contributor to changes in the aerosol budget of the continent.


2009 ◽  
Vol 2 (2) ◽  
pp. 213-229 ◽  
Author(s):  
N. Huneeus ◽  
O. Boucher ◽  
F. Chevallier

Abstract. We have developed a simplified aerosol model together with its tangent linear and adjoint versions for the ultimate aim of optimizing global aerosol and aerosol precursor emission using variational data assimilation. The model was derived from the general circulation model LMDz; it groups together the 24 aerosol species simulated in LMDz into 4 species, namely gaseous precursors, fine mode aerosols, coarse mode desert dust and coarse mode sea salt. The emissions have been kept as in the original model. Modifications, however, were introduced in the computation of aerosol optical depth and in the processes of sedimentation, dry and wet deposition and sulphur chemistry to ensure consistency with the new set of species and their composition. The simplified model successfully manages to reproduce the main features of the aerosol distribution in LMDz. The largest differences in aerosol load are observed for fine mode aerosols and gaseous precursors. Differences between the original and simplified models are mainly associated to the new deposition and sedimentation velocities consistent with the definition of species in the simplified model and the simplification of the sulphur chemistry. Furthermore, simulated aerosol optical depth remains within the variability of monthly AERONET observations for all aerosol types and all sites throughout most of the year. Largest differences are observed over sites with strong desert dust influence. In terms of the daily aerosol variability, the model is less able to reproduce the observed variability from the AERONET data with larger discrepancies in stations affected by industrial aerosols. The simplified model however, closely follows the daily simulation from LMDz. Sensitivity analyses with the tangent linear version show that the simplified sulphur chemistry is the dominant process responsible for the strong non-linearity of the model.


2013 ◽  
Vol 13 (20) ◽  
pp. 10425-10444 ◽  
Author(s):  
P. E. Saide ◽  
G. R. Carmichael ◽  
Z. Liu ◽  
C. S. Schwartz ◽  
H. C. Lin ◽  
...  

Abstract. An aerosol optical depth (AOD) three-dimensional variational data assimilation technique is developed for the Gridpoint Statistical Interpolation (GSI) system for which WRF-Chem forecasts are performed with a detailed sectional model, the Model for Simulating Aerosol Interactions and Chemistry (MOSAIC). Within GSI, forward AOD and adjoint sensitivities are performed using Mie computations from the WRF-Chem optical properties module, providing consistency with the forecast. GSI tools such as recursive filters and weak constraints are used to provide correlation within aerosol size bins and upper and lower bounds for the optimization. The system is used to perform assimilation experiments with fine vertical structure and no data thinning or re-gridding on a 12 km horizontal grid over the region of California, USA, where improvements on analyses and forecasts is demonstrated. A first set of simulations was performed, comparing the assimilation impacts of using the operational MODIS (Moderate Resolution Imaging Spectroradiometer) dark target retrievals to those using observationally constrained ones, i.e., calibrated with AERONET (Aerosol RObotic NETwork) data. It was found that using the observationally constrained retrievals produced the best results when evaluated against ground based monitors, with the error in PM2.5 predictions reduced at over 90% of the stations and AOD errors reduced at 100% of the monitors, along with larger overall error reductions when grouping all sites. A second set of experiments reveals that the use of fine mode fraction AOD and ocean multi-wavelength retrievals can improve the representation of the aerosol size distribution, while assimilating only 550 nm AOD retrievals produces no or at times degraded impact. While assimilation of multi-wavelength AOD shows positive impacts on all analyses performed, future work is needed to generate observationally constrained multi-wavelength retrievals, which when assimilated will generate size distributions more consistent with AERONET data and will provide better aerosol estimates.


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