Energy Transfer Between Single Semiconductor Quantum Dots and Organic Dye Molecules

2018 ◽  
Vol 232 (9-11) ◽  
pp. 1513-1526 ◽  
Author(s):  
Dzmitry Melnikau ◽  
Thomas Hendel ◽  
Pavel A. Linkov ◽  
Pavel S. Samokhvalov ◽  
Igor R. Nabiev ◽  
...  

Abstract An understanding of the mechanisms of energy transfer and conversion on the nanoscale is one of the key requirements for an implementation of highly efficient photonic nanodevices based on hybrid organic/inorganic nanomaterials. In this work we conduct steady-state and time resolved optical studies of the emission properties of an ensembles and single semiconductor quantum dots and attached organic dye molecules. We revealed that the luminescence intensity of a hybrid structure does not follow the blinking behavior of quantum dots. We also demonstrated an efficient single photon generation from single hybrid nanostructures which involves an energy transfer from donor to acceptor as main excitation source.

2019 ◽  
Vol 9 (1) ◽  
Author(s):  
Il-Wook Cho ◽  
Mee-Yi Ryu

AbstractSurface passivation is an effective method to protect the surfaces and improve the luminescence properties of perovskite (PS) films. CdSe/ZnS core-shell quantum dots (QDs) have been employed for surface passivation of PS films because of their size-dependent tunable bandgaps. Herein, the energy transfer (ET) behavior of CH3NH3PbI2Br PS films covered with CdSe/ZnS QDs (QD/PS hybrid structures) is characterized by using photoluminescence (PL) and time-resolved PL spectroscopy. The PL decay time and the integrated PL intensity of the QD/PS hybrid structure increase compared with those of the bare PS films, owing to ET from the QDs to the PS and reduced charge traps. The ET efficiency increases from ~7% to 63% for the QD/PS hybrid structure when the core diameter of the QDs decreases from 6.5 to 2.7 nm, respectively. This can be explained by the charge transfer rate enhancement due to the control of energy level alignment of QDs. These results allow us to understand fundamental mechanisms such as ET from QDs to PS films as a function of the size of the QD.


2004 ◽  
Vol 6 ◽  
pp. 90-90 ◽  
Author(s):  
Thomas Aichele ◽  
Valéry Zwiller ◽  
Oliver Benson

ChemPhysChem ◽  
2011 ◽  
Vol 13 (1) ◽  
pp. 330-335 ◽  
Author(s):  
Marya Hardzei ◽  
Mikhail Artemyev ◽  
Michael Molinari ◽  
Michel Troyon ◽  
Alyona Sukhanova ◽  
...  

Nano Letters ◽  
2020 ◽  
Vol 20 (9) ◽  
pp. 6357-6363 ◽  
Author(s):  
Łukasz Dusanowski ◽  
Dominik Köck ◽  
Eunso Shin ◽  
Soon-Hong Kwon ◽  
Christian Schneider ◽  
...  

2021 ◽  
Author(s):  
Pietro Lombardi ◽  
Ramin Emadi ◽  
Rocco Duquennoy ◽  
Ghiilam Murtaza ◽  
Maja Colautti ◽  
...  

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