Radiative properties of soot particles

THERMOPEDIA ◽  
2008 ◽  
Author(s):  
Leonid A. Dombrovsky
Author(s):  
Kevin Torres Monclard ◽  
Olivier Gicquel ◽  
Ronan Vicquelin

Abstract The effect of soot radiation modeling, pressure, and level of soot volume fraction are investigated in two ethylene-air turbulent flames: a jet flame at atmospheric pressure studied at Sandia, and a confined pressurized flame studied at DLR. Both cases have previously been computed with large-eddy simulations coupled with thermal radiation. The present study aims at determining and analyzing the thermal radiation field for different models from these numerical results. A Monte-Carlo solver based on the Emission Reciprocity Method is used to solve the radiative transfer equation with detailed gas and soot properties in both configurations. The participating gases properties are described by an accurate narrowband ck model. Emission, absorption, and scattering from soot particles are accounted for. Two formulations of the soot refractive index are considered: a constant value and a wavelength formulation dependency. This is combined with different models for soot radiative properties: gray, Rayleigh theory, Rayleigh-Debye-Gans theory for fractal aggregates. The effects of soot radiative scattering is often neglected since their contribution is expected to be small. This contribution is determined quantitatively in different scenarios, showing great sensitivity to the soot particles morphology. For the same soot volume fraction, scattering from larger aggregates is found to modify the radiative heat transfer noticeably. Such a finding outlines the need for detailed information on soot particles. Finally, the role of soot volume fraction and pressure on radiative interactions between both solid and gaseous phases is investigated.


2020 ◽  
Author(s):  
Ulrike Lohmann ◽  
Franz Friebel ◽  
Zamin A. Kanji ◽  
Fabian Mahrt ◽  
Amewu A. Mensah ◽  
...  

<p>Clouds play a critical role in the hydrological cycle and modulating the Earth’s climate via precipitation and radiative forcing. Aerosol particles acting as cloud condensation nuclei and ice nucleating particles aid in cloud formation, shaping their microphysical structure. Previously thought to be unimportant for cloud formation, soot particles that undergo oxidation by ozone and/or aging with aqueous sulfuric acid result in being both good centers for cloud droplets and ice crystals formation. However, the associated changes in cloud radiative properties and the consequences for Earth’s climate remain uncertain, because these processes have not been considered in global climate models. Here we present both past and future global climate simulations, which for the first time consider the effect of such aged soot particles as cloud condensation nuclei and ice nucleating particles. Our results constitute the first evidence that aging of soot particles produce a 0.2 to 0.25 Wm<sup>-2</sup> less negative shortwave indirect aerosol forcing compared to previous estimates. We also conducted equilibrium climate sensitivity simulations representing a future warmer climate in which the carbon dioxide concentration is doubled compared to pre-industrial levels. Accounting for these soot aging processes significantly exacerbates the global mean surface temperature increase by 0.4 to 0.5 K. Thus, reducing emissions of soot particles will be beneficial for many aspects including air pollution and future climate.</p><p> </p>


Author(s):  
Ahmed M Abdel-Ghanya ◽  
Ibrahim M Al-Helal

Plastic nets are extensively used for shading purposes in arid regions such as in the Arabian Peninsula. Quantifying the convection exchange with shading net and understanding the mechanisms (free, mixed and forced) of convection are essential for analyzing energy exchange with shading nets. Unlike solar and thermal radiation, the convective energy, convective heat transfer coefficient and the nature of convection have never been theoretically estimated or experimentally measured for plastic nets under arid conditions. In this study, the convected heat exchanges with different plastic nets were quantified based on an energy balance applied to the nets under outdoor natural conditions. Therefore, each net was tacked onto a wooden frame, fixed horizontally at 1.5-m height over the floor. The downward and upward solar and thermal radiation fluxes were measured below and above each net on sunny days; also the wind speed over the net, and the net and air temperatures were measured, simultaneously. Nets with different porosities, colors and texture structures were used for the study. The short and long wave’s radiative properties of the nets were pre-determined in previous studies to be used. Re and Gr numbers were determined and used to characterize the convection mechanism over each net. The results showed that forced and mixed convection are the dominant modes existing over the nets during most of the day and night times. The nature of convection over nets depends mainly on the wind speed, net-air temperature difference and texture shape of the net rather than its color and its porosity.


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