scholarly journals Monitoring studies to assess the condition of drinking water supply sources in potentially radon-hazardous areas by specific gross alpha activity

Author(s):  
Lidiya Karl ◽  
Tatiana Lashchenova ◽  
Albert Marenny
2019 ◽  
Vol 12 (2(св)) ◽  
pp. 121-128
Author(s):  
A. A. Pivovarov ◽  
E. A. Pivovarova ◽  
V. E. Kurganov

The aim of the work is to develop control levels of specific total alpha-activity of water samples for a number of sources of centralized drinking water supply in the Republic of Khakassia on the basis of the results of long-term laboratory studies. Materials and methods. The analysis is carried out on the basis of the results of laboratory studies of water sources of centralized drinking water supply of the population of the Republic of Khakassia, performed by accredited testing laboratories of institutions of the state sanitary and epidemiological service of the Republic for the period from 2001 to 2018, using alpha-beta radiometric, alpha-spectrometric methods with radiochemical preparation of counting samples, gamma-spectrometric method. The control levels of specific total alpha-activity of water samples from the sources of centralized drinking water supply in the Republic of Khakassia were established by the statistical maximum – the sum of the average value with a doubled standard deviation, with the volume of research more than 30, and the maximum value with the volume of research less than 30. Results. About half of the studied water samples from the sources of the centralized drinking water supply of the Republic of Khakassia, annually, are noted with exceeding the control level of specific total alpha-activity (0,2 Bq/kg). The values obtained in the studied samples vary up to 5,57 Bq/kg. During the observation period, samples of water exceeding the reference level of specific total alpha-activity (0.2 Bq/kg) were identified in settlements of the Altai, Askizsky, Beysky, Bogradsky, Ordzhonikidzevsky, Tashtypsky, Ust–Abakansky, Shira districts and the city of Sorsk, smt. Prigorsk (Chernogorsk). In previous studies, it was found that high levels of specific total alpha-activity in the country are mainly due to natural radionuclides uranium-238 (238U), uranium-234 (234U). In a number of settlements of the Republic, the sum of the ratio of specific activities of natural radionuclides to the corresponding levels of intervention exceeds 1,0. Average annual individual effective doses of internal exposure to natural radionuclides of drinking water, at or above 0,1 mSv/year (values in the range of 0,1-0,2 mSv/year), which does not require urgent radiation protection measures. At the same time, monitoring of indicators of radiation safety of water sources of water supply should be carried out in accordance with the established requirements. In this connection, in order to improve control, for the rapid assessment of the radiation situation and making timely decisions to ensure radiation safety of the population, the calculation of control levels of specific total alpha-activity was carried out. As a result of calculations, specific values of control levels for each of water source were obtained. The calculated values range from 0,2 to 2,6 Bq/kg. Conclusion. The control levels are “site standards” and are calculated for each of the source of water supply. Their excess will be considered as a signal of “negative change” of the radiation situation”, which may be associated with an increase of the specific activities of 234U, 238U, or the appearance of highly radiotoxic radionuclides: 226Ra, 210Po, 228Ra.


2020 ◽  
Author(s):  
Katalin Csondor ◽  
Petra Baják ◽  
Bálint Izsák ◽  
Márta Vargha ◽  
Heinz Surbeck ◽  
...  

<p>In Hungary the drinking water supply is mainly based on groundwater from aquifers characterized by different lithology. Riverbank filtered systems represent 40 % of drinking water supply. According to the EURATOM drinking water directive, there are recent regulations in Hungary regarding the natural radioactivity of drinking waters. Based on this, if gross alpha or gross beta radiation exceeds the limit, nuclide-specific measurements are required to be performed by the relevant waterworks. Since the mobility of uranium and radium is strongly influenced by the geochemical conditions, knowledge on the geochemical parameters of water is required. Therefore hydrogeology has a crucial role in revealing the origin of elevated activity concentrations. This research presents a case study in Hungary where the drinking water supply is provided by bank filtered and karst wells. The main aim of this study is to determine which radionuclides may cause the elevated radioactivity and explain their occurrence using hydrogeological approach, considering also the temporal variation of groundwater/surface water ratio. In most of the wells of the research area the gross alpha values are above the screening level, 0.1 Bq L<sup>-1</sup>. The study revealed the correlation between the river water level fluctuation and the uranium content of the wells. Among the investigated radionuclides, the uranium activity concentrations responded the most to the water level changes of the river and showed systematically higher values during low water conditions. In addition the karst wells showed low activity concentrations. This suggests, that uranium is transported by the groundwater component, and possibly sourced from the fluviatile sediments. The results of this study highlighted the transient nature of river bank filtered systems, which should be taken into account in the monitoring and water supply strategy. Nevertheless, the study emphasizes the importance of considering the dynamics of groundwater and associated geochemical environment in addition to geological factors, when investigating the radioactivity of groundwater or other potential contaminants.</p><p>This study was supported by the ÚNKP-19-3 New National Excellence Program of the Ministry of Human Capacities. This study is part of a project that has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 810980.</p>


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