Simultaneous determination of gross alpha/beta activities in water by liquid scintillation counting and its applications in the environmental monitoring

Based on the standards of ISO11704-2018 and ASTM D7283-17, a method for simultaneous determination of gross alpha and gross beta activity concentrations in water by liquid scintillation counting (LSC) was established, which can be applied to various types of water samples in routine monitoring, such as drinking water, groundwater, geothermal water, seawater, and radioactive wastewater. The sample’s pH value and concentrated volume must be controlled to avoid quenching as much as possible. The validation tests show that the deviations of gross alpha and gross beta activities can satisfy quality control requirements in a wide range of activity ratios. For the actual samples, the measurement results of the LSC method are in good agreement with those of the thick source method. Moreover, the LSC method performs better in detection limit and a simpler pretreatment process than the thick source method.

Corrections to Kusnetz method for measurements of radon progeny concentrations in air

In 1956, H.L. Kusnetz proposed a quick method for radon progeny concentration measurement in mine atmosphere using a single gross-alpha count of a membrane-filtered air. The method is still widely used today and is based on a number of impractical assumptions. An instantaneous sampling time (less than ten seconds), is one of these assumptions that ignores the build-up and decay of the progeny on the filter paper during the sampling period, which is typically in the order of a few minutes. Of special concern is the 214Bi decay during the sampling period, since 214Po's alphas are lost during the sampling time and cannot be accounted for during the counting time. In addition, the method assumes that 214Bi activity during the counting period is constant. This inaccurate assumption can result in a smaller count rate, especially when counting times are long. Hence, underestimated working levels are expected when using Kusnetz factors without correcting for the sampling and counting times. In this technical report, exact sampling and counting time corrections to the method are provided along with the updated Kusnetz factors that correspond to common equilibrium conditions to correctly estimate the Working Level in air. Additionally, time corrections to the commonly used self-absorption correction formula and the lower level of detectability (LLD) equation used for any sample measurement are given.

Evaluating the impact of free private well testing outreach on participants' private well stewardship in New Jersey

Over 1 million people in New Jersey (NJ) are estimated to receive drinking water from private wells. The most commonly detected contaminants in NJ private well water are naturally occurring arsenic and gross alpha (8.3 and 10.9%, respectively). Between 2015 and 2018, three free and voluntary private well testing events tested a total of 571 at-risk wells and 226 (40%) were identified as having one or more contaminants exceeding drinking water standards. Participants were invited to complete a survey to evaluate household characteristics, participant experience, and private well stewardship behavior patterns. Of 529 delivered surveys, 211 (40%) participants completed surveys. Among respondents, 63% reported plans to test their private wells in the future. Among failed wells, 45% of households reported performing mitigative action in response to the event, either through the installation of water treatment system or switching to bottled water. The survey evaluation identified previous knowledge of well contamination risks and discussing test results with a third party as important factors for promoting self-reported stewardship behavior. The evaluation provides guidance for outreach organizers to develop effective testing events and further considers the private well owners' experience of the outreach events to identify information for ‘best practices’ and improvements of future programs.

Measurement of Natural Radionuclides in Drinking Water and Risk Assessment in a Volcanic Region of Italy, Campania

The physical–chemical properties of water are closely linked to the geological nature of the site where they are located. This aspect becomes even more interesting when analyzing the natural radionuclides in the drinking water of a volcanic territory such as Campania in southern Italy. This study concerned the measurement of activity concentration of gross alpha and beta, radon, and tritium to evaluate their biological impact. The measurements were carried out using alpha spectrometry for alpha emitters, proportional counter for beta emitters, the electret system for radon in water, and finally liquid scintillation for the measurement of tritium concentration. The biological impact was assessed considering the indicative dose, if applicable, and the effective annual dose of radon. Although the results show that the values are below international and national references, the radiological characterization of drinking water is of fundamental importance to optimize the radiation protection of the population.

Gross alpha and gross beta activities measurements in groundwaters using liquid scintillation counting (LSC)

In this work Authors describe the methodology of gross alpha and gross beta activities determination in water samples. The chosen method is dedicated to LSC and is based on ISO 11704:2018 and it is suitable for ground waters with low and medium salinity, especially drinking or tap waters as well as medicinal waters (with healing properties, using in health resorts). Authors describe the proper sampling, laboratory preparation including radon removal and measurements conditions. The local and European law regulations showing the limits of radioactivity of drinking waters and medicinal waters are presented. This work presents also selected data of gross alpha and gross beta activities from selected research: the highest levels is measured in Jordanian (gross alpha) and in Brazil (gross beta) and it is respectively 3.58 Bq/L and 5.22 Bq/L.

Detecting the relations between meteorological elements and alpha and beta activity concentration at Al-Tuwaitha site, Baghdad

In this study, 50 samples of air particulates collected from different places in- and outside the Al-Tuwaitha nuclear site, south of Baghdad were used to measure daily gross alpha and beta activity concentrations (AAC and BAC) for the period from 28 January 2015 to 13 April 2017. At the same time, several meteorological factors such as air temperature, wind speed, wind direction, air pressure, relative humidity, and solar radiation, were also measured. Air stability classes were also derived from wind speed and solar radiation. AAC/BAC variations in the surface air layer were discussed in relation to these factors. The results show that there are inverse relations between AAC/BAC and wind speed and temperature, linear relations between AAC/ABC and air pressure and weak relations between AAC/BAC and relative humidity and solar radiation. Lastly, AAC/BAC measurements in unstable air are as large as in neutral air.