scholarly journals Models of semiconductor quantum dots blinking based on spectral diffusion -=SUP=-*-=/SUP=-

2019 ◽  
Vol 126 (1) ◽  
pp. 77
Author(s):  
V.K. Busov ◽  
P.A. Frantsuzov
Keyword(s):  
Quantum Dots ◽  
Electron Transfer ◽  
Quantum Dot ◽  
Semiconductor Quantum Dots ◽  
Spectral Diffusion ◽  
The Other ◽  
Diffusion Controlled ◽  
Colloidal Quantum Dot ◽  
Marcus Model ◽  
Observed Behavior

AbstractThree models of single colloidal quantum dot emission fluctuations (blinking) based on spectral diffusion were considered analytically and numerically. It was shown that the only one of them, namely the Frantsuzov and Marcus model reproduces the key properties of the phenomenon. The other two models, the Diffusion-Controlled Electron Transfer (DCET) model and the Extended DCET model predict that after an initial blinking period, most of the QDs should become permanently bright or permanently dark which is significantly different from the experimentally observed behavior.

scholarly journals From Random Telegraph to Gaussian Stochastic Noises: Decoherence and Spectral Diffusion in a Semiconductor Quantum Dot

2010 ◽  
Vol 2010 ◽  
pp. 1-13 ◽  
Author(s):  
A. Berthelot ◽  
C. Voisin ◽  
C. Delalande ◽  
Ph. Roussignol ◽  
R. Ferreira ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Quantum Dot ◽  
Gaussian Noise ◽  
Theoretical Description ◽  
Semiconductor Quantum Dots ◽  
Spectral Diffusion ◽  
Jump Processes ◽  
Quantitative Interpretation ◽  
Semiconductor Quantum Dot ◽  
Stochastic Noises

We present a general theoretical description of the extrinsic dephasing mechanism of spectral diffusion that dominates the decoherence dynamics in semiconductor quantum dots at low temperature. We discuss the limits of random telegraph and Gaussian stochastic noises and show that the combination of both approaches in the framework of the pre-Gaussian noise theory allows a quantitative interpretation of high-resolution experiments in single semiconductor quantum dots. We emphasize the generality and the versatility of our model where the inclusion of asymmetric jump processes appears as an essential extension for the understanding of semiconductor quantum dot physics.

Optical Characterization of CdSe Colloidal Quantum Dot/ MEH-PPV Polymer Nanocomposites Spin-cast on GaAs Substrates

2006 ◽  
Vol 939 ◽  
Author(s):  
Adrienne D. Stiff-Roberts ◽  
Abhishek Gupta ◽  
Zhiya Zhao
Keyword(s):  
Quantum Dots ◽  
Quantum Dot ◽  
Optoelectronic Devices ◽  
Photogenerated Electron ◽  
Polymer Nanocomposite ◽  
Colloidal Quantum Dots ◽  
Infrared Light ◽  
Gaas Substrates ◽  
Conducting Polymer Nanocomposite ◽  
Colloidal Quantum Dot

ABSTRACTThe motivation and distinct approach for this work is the use of intraband transitions within colloidal quantum dots for the detection of mid- (3-5 μm) and/or long-wave (8-14 μm) infrared light. The CdSe colloidal quantum dot/MEH-PPV conducting polymer nanocomposite material is well-suited for this application due to the ∼1.5 eV difference between the corresponding electron affinities. Therefore, CdSe colloidal quantum dots embedded in MEH-PPV should provide electron quantum confinement such that intraband transitions can occur in the conduction band. Further, it is desirable to deposit these nanocomposites on semiconductor substrates to enable charge transfer of photogenerated electron-hole pairs from the substrate to the nanocomposite. In this way, optoelectronic devices analogous to those achieved using Stranski-Krastanow quantum dots grown by epitaxy can be realized. To date, there have been relatively few investigations of colloidal quantum dot nanocomposites deposited on GaAs substrates. However, it is crucial to develop a better understanding of the optical properties of these hybrid material systems if such heterostructures are to be used for optoelectronic devices, such as infrared photodetectors. By depositing the nanocomposites on GaAs substrates featuring different doping characteristics and measuring the corresponding Fourier transform infrared absorbance, the feasibility of these intraband transitions is demonstrated at room temperature.

Efficient and Bright Colloidal Quantum Dot Light-Emitting Diodes via Controlling the Shell Thickness of Quantum Dots

2013 ◽  
Vol 5 (22) ◽  
pp. 12011-12016 ◽  
Author(s):  
Huaibin Shen ◽  
Qinli Lin ◽  
Hongzhe Wang ◽  
Lei Qian ◽  
Yixing Yang ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Quantum Dot ◽  
Shell Thickness ◽  
Light Emitting Diodes ◽  
Light Emitting ◽  
Colloidal Quantum Dot

Quantum dot–polymer conjugates for stable luminescent displays

Nanoscale ◽  
2018 ◽  
Vol 10 (28) ◽  
pp. 13368-13374 ◽  
Author(s):  
Sushant Ghimire ◽  
Anjaly Sivadas ◽  
Ken-ichi Yuyama ◽  
Yuta Takano ◽  
Raju Francis ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Solar Cells ◽  
Quantum Dot ◽  
Semiconductor Quantum Dots ◽  
Broad Absorption ◽  
Polymer Conjugates ◽  
Absorption Of Light

The broad absorption of light in the UV-Vis-NIR region and the size-based tunable photoluminescence color of semiconductor quantum dots make these tiny crystals one of the most attractive antennae in solar cells and phosphors in electrooptical devices.

Partially pyridine-functionalized quantum dots for efficient red, green, and blue light-emitting diodes

2019 ◽  
Vol 7 (12) ◽  
pp. 3429-3435 ◽  
Author(s):  
Sukyung Choi ◽  
Jaehyun Moon ◽  
Hyunsu Cho ◽  
Byoung-Hwa Kwon ◽  
Nam Sung Cho ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Quantum Dot ◽  
Blue Light ◽  
Light Emitting Diodes ◽  
High Brightness ◽  
Light Emitting ◽  
Turn On ◽  
Colloidal Quantum Dot

Surface-exchanged, partially pyridine-functionalized colloidal quantum dot-based light-emitting diodes (QD-LEDs) exhibit a low turn-on voltage and high brightness.

Upconverting nanoparticle to quantum dot FRET for homogeneous double-nano biosensors

RSC Advances ◽  
2015 ◽  
Vol 5 (18) ◽  
pp. 13270-13277 ◽  
Author(s):  
Leena Mattsson ◽  
K. David Wegner ◽  
Niko Hildebrandt ◽  
Tero Soukka
Keyword(s):  
Quantum Dots ◽  
Quantum Dot ◽  
Near Infrared ◽  
Photophysical Properties ◽  
Semiconductor Quantum Dots ◽  
Optical Biosensing ◽  
Donor Acceptor

The unique photophysical properties of upconverting nanoparticles (UCNPs) and semiconductor quantum dots (QDs) render them an attractive donor–acceptor combination for near-infrared (NIR) excited FRET-based optical biosensing.

Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots

2000 ◽  
Vol 85 (15) ◽  
pp. 3301-3304 ◽  
Author(s):  
R. G. Neuhauser ◽  
K. T. Shimizu ◽  
W. K. Woo ◽  
S. A. Empedocles ◽  
M. G. Bawendi
Keyword(s):  
Quantum Dots ◽  
Semiconductor Quantum Dots ◽  
Spectral Diffusion ◽  
Fluorescence Intermittency
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